4,213 research outputs found
How droplets nucleate and grow on liquids and liquid impregnated surfaces
Condensation on liquids has been studied extensively in context of breath figure templating, materials synthesis and enhancing heat transfer using liquid impregnated surfaces. However, the mechanics of nucleation and growth on liquids remains unclear, especially on liquids that spread on the condensate. By examining the energy barriers of nucleation, we provide a framework to choose liquids that can lead to enhanced nucleation. We show that due to limits of vapor sorption within a liquid, nucleation is most favoured at the liquid–air interface and demonstrate that on spreading liquids, droplet submergence within the liquid occurs thereafter. We provide a direct visualization of the thin liquid profile that cloaks the condensed droplet on a liquid impregnated surface and elucidate the vapour transport mechanism in the liquid films. Finally, we show that although the viscosity of the liquid does not affect droplet nucleation, it plays a crucial role in droplet growth.MIT Energy InitiativeMasdar Institute of Science and Technology (Grant 69238330
Radiative electron capture in the first forbidden unique decay of 81Kr
The photon spectrum accompanying the orbital K-electron capture in the first
forbidden unique decay of 81Kr was measured. The total radiation intensity for
the photon energies larger than 50 keV was found to be 1.47(6) x 10^{-4} per
K-capture. Both the shape of the spectrum and its intensity relative to the
ordinary, non-radiative capture rate, are compared to theoretical predictions.
The best agreement is found for the recently developed model which employs the
length gauge for the electromagnetic field.Comment: 7 pages, 6 figure
Gamow-Teller Strength in the Region of Sn
New calculations are presented for Gamow-Teller beta decay of nuclei near
Sn. Essentially all of the Sn Gamow-Teller decay strength is
predicted to go to a single state at an excitation energy of 1.8 MeV in
In. The first calculations are presented for the decays of neighboring
odd-even and odd-odd nuclei which show, in contrast to Sn, surprisingly
complex and broad Gamow-Teller strength distributions. The results are compared
to existing experimental data and the resulting hindrance factors are
discussed.Comment: 12 pages (latex) and 2 figures available on reques
Decay Rate of Triaxially-Deformed Proton Emitters
The decay rate of a triaxially-deformed proton emitter is calculated in a
particle-rotor model, which is based on a deformed Woods-Saxon potential and
includes a deformed spin-orbit interaction. The wave function of the
ground state of the deformed proton emitter Ho is obtained
in the adiabatic limit, and a Green's function technique is used to calculate
the decay rate and branching ratio to the first excited 2 state of the
daughter nucleus. Only for values of the triaxial angle
is good agreement obtained for both the total decay rate and the 2
branching ratio.Comment: 19 pages, 4 figure
Penning trap mass measurements on (99-109)$Cd with ISOLTRAP and implications on the rp process
Penning trap mass measurements on neutron-deficient Cd isotopes (99-109)Cd
have been performed with the ISOLTRAP mass spectrometer at ISOLDE/CERN, all
with relative mass uncertainties below 3*10^8. A new mass evaluation has been
performed. The mass of 99Cd has been determined for the first time which
extends the region of accurately known mass values towards the doubly magic
nucleus 100Sn. The implication of the results on the reaction path of the rp
process in stellar X-ray bursts is discussed. In particular, the uncertainty of
the abundance and the overproduction created by the rp-process for the mass A =
99 is demonstrated by reducing the uncertainty of the proton-separation energy
of 100In Sp(100In) by a factor of 2.5.Comment: 14 pages, 9 figure
Orbital dependent nucleonic pairing in the lightest known isotopes of tin
By studying the 109Xe-->105Te-->101Sn superallowed alpha-decay chain, we
observe low-lying states in 101Sn, the one-neutron system outside doubly magic
100Sn. We find that the spins of the ground state (J = 7=2) and first excited
state (J = 5=2) in 101Sn are reversed with respect to the traditional level
ordering postulated for 103Sn and the heavier tin isotopes. Through simple
arguments and state-of-the-art shell model calculations we explain this
unexpected switch in terms of a transition from the single-particle regime to
the collective mode in which orbital-dependent pairing correlations, dominate.Comment: 5 pages 3 figure
Beta decay of 71,73Co; probing single particle states approaching doubly magic 78Ni
Low-energy excited states in 71,73Ni populated via the {\beta} decay of
71,73Co were investigated in an experiment performed at the National
Superconducting Cyclotron Laboratory (NSCL) at Michigan State University (MSU).
Detailed analysis led to the construction of level schemes of 71,73Ni, which
are interpreted using systematics and analyzed using shell model calculations.
The 5/2- states attributed to the the f5/2 orbital and positive parity 5/2+ and
7/2+ states from the g9/2 orbital have been identified in both 71,73Ni. In 71Ni
the location of a 1/2- {\beta}-decaying isomer is proposed and limits are
suggested as to the location of the isomer in 73Ni. The location of positive
parity cluster states are also identified in 71,73Ni. Beta-delayed neutron
branching ratios obtained from this data are given for both 71,73Co.Comment: Accepted for publication in PR
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