273 research outputs found
Time dependence of Bragg forward scattering and self-seeding of hard x-ray free-electron lasers
Free-electron lasers (FELs) can now generate temporally short, high power
x-ray pulses of unprecedented brightness, even though their longitudinal
coherence is relatively poor. The longitudinal coherence can be potentially
improved by employing narrow bandwidth x-ray crystal optics, in which case one
must also understand how the crystal affects the field profile in time and
space. We frame the dynamical theory of x-ray diffraction as a set of coupled
waves in order to derive analytic expressions for the spatiotemporal response
of Bragg scattering from temporally short incident pulses. We compute the
profiles of both the reflected and forward scattered x-ray pulses, showing that
the time delay of the wave is linked to its transverse spatial shift
through the simple relationship , where
is the grazing angle of incidence to the diffracting planes. Finally,
we apply our findings to obtain an analytic description of Bragg forward
scattering relevant to monochromatically seed hard x-ray FELs.Comment: 11 pages, 6 figure
Focusing of a tabletop soft-x-ray laser beam and laser ablation
Includes bibliographical references (page 1716).We focused the beam of a high-repetition-rate capillary-discharge tabletop laser operating at a wavelength of 46.9 nm, using a spherical Si/Sc multilayer mirror. The energy densities significantly exceeded the thresholds for the ablation of metals. Single-shot laser ablation patterns were used in combination with ray-tracing computations to characterize the focused beam. The radiation intensity within the 2-μm-diameter central region of the focal spot was estimated to be ≈1011 W/cm2, with a corresponding energy density of ~100 J/cm2
Interaction of the Electromagnetic p-Waves with Thin Metal Films
For the first time it is shown that for thin metallic films thickness of
which not exceed thickness of skin-layer, the problem allows analytical
solution for arbitrary boundary value problems. The analysis of dependence of
coefficients of transmission, reflection and absorbtion on angle incidence,
thickness of films and coefficient of specular reflection is carried out.Comment: 15 pages, 9 figure
Comparison of oxidizing agents for the oxidative coupling of methane over state-of-the-art catalysts
The synthesis of selected state-of-the-art catalysts providing high performances in the oxidative coupling of methane (OCM) with O2 was reproduced according to the respective recipes reported in literature. A reference material with identical stoichiometric composition was further synthesized by applying the cellulose templating method. This method increases the surface area and affects the phase composition and crystallite size of the catalysts as determined by N2-physisoprtion, X-ray diffraction and scanning electron microscopy. This, however, is in most cases detrimental to the catalytic OCM performance due to enhanced global activity resulting in hot spots in the catalyst bed. Catalysts were tested in the OCM under variation of temperature (973–1073 K), GHSV (3600–100,000 h−1) and oxidizing agent (O2 and N2O). In general, conversions of CH4 when using N2O are lower than in the presence of O2, however, the selectivities to C2 products ethane and ethylene are higher even at a similar level of CH4 conversion. This confirms the presence of different oxygen species formed by activation of these oxidizing agents
Efficiency of productivity potential realization of different-age sites of a trunk of grades of columnar type apple-trees
Received: April 15th, 2022 ; Accepted: May 15th, 2022 ; Published: May 17th, 2022 ; Correspondence: [email protected] article provides information about buds organogenesis in plants of columnar apple
cultivars in the Forest-Steppe of Ukraine (Kyiv), which allows to establish the features of this
process in complex fruit formations of different ages, and their productivity and longevity. We
recommend studying of apple trees productivity in the process of its formation by analyzing of
rudimentary organs formation and their consistent development into vegetative and generative
organs, which are elements of productivity. Studies of organogenesis different-age fruit
formations of columnar apple cultivars were conducted in the northern part of the Forest-Steppe
of Ukraine during 2016–2020. It was established that separate age sections of columnar apple
trees trunk formed different initial productivity potential. In plants of all studied varieties and age
groups, the laying of generative buds, the implementation of reproductive elements in V–IX and
X–XI stages of organogenesis were more effective in older age areas of the trunk. Complex fruit
formations, regardless of the trunk age where they are placed, form a high potential for
productivity, which is effectively realized. The dependence of the formation and productivity
potential realization on the stages of organogenesis and meteorological factors is established
Science Requirements and Conceptual Design for a Polarized Medium Energy Electron-Ion Collider at Jefferson Lab
This report presents a brief summary of the science opportunities and program
of a polarized medium energy electron-ion collider at Jefferson Lab and a
comprehensive description of the conceptual design of such a collider based on
the CEBAF electron accelerator facility.Comment: 160 pages, ~93 figures This work was supported by the U.S. Department
of Energy, Office of Nuclear Physics, under Contract No. DE-AC05-06OR23177,
DE-AC02-06CH11357, DE-AC05-060R23177, and DESC0005823. The U.S. Government
retains a non-exclusive, paid-up, irrevocable, world-wide license to publish
or reproduce this manuscript for U.S. Government purpose
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Forty years of temporal analysis of products
A detailed understanding of reaction mechanisms and kinetics is required in order to develop and optimize catalysts and catalytic processes. While steady-state investigations are known to give a global view of the catalytic system, transient studies are invaluable since they can provide more comprehensive insight into elementary steps. For almost forty years temporal analysis of products (TAP) has been successfully utilized for transient studies of gas phase heterogeneous reactions, and there have been a number of advances in instrumentation and numerical modeling methods in that time. Since TAP is a complex methodology it is often viewed as a niche specialty. With the purpose to make TAP more relevant and approachable to a wider segment of the catalytic research community, part of the intention of this work is to highlight the significant contributions TAP has made to elucidating mechanistic and kinetic aspects of complex, multi-step heterogeneous reactions. With this in mind, an outlook is also disclosed for the technique in terms of what is needed to revitalize the field and make it more applicable to the recent advances in catalyst characterization (e.g. operando modes)
Updated Report Acceleration of Polarized Protons to 120-150 GeV/c at Fermilab
The SPIN@FERMI collaboration has updated its 1991-95 Reports on the
acceleration of polarized protons in Fermilab's Main Injector, which was
commissioned by Fermilab. This Updated Report summarizes some updated Physics
Goals for a 120-150 GeV/c polarized proton beam. It also contains an updated
discussion of the Modifications and Hardware needed for a polarized beam in the
Main Injector, along with an updated Schedule and Budget.Comment: 30 pages, 12 figure
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