272 research outputs found
Millikelvin magnetic relaxation measurements of alpha-Fe2O3 antiferromagnetic particles
In this paper we report magnetic relaxation data for antiferromagnetic
alpha-Fe2O3 particles of 5 nm mean diameter in the temperature range 0.1 K to
25 K. The average spin value of these particles S=124 and the uniaxial
anisotropy constant D=1.6x10^-2 K have been estimated from the experimental
values of the blocking temperature and anisotropy field. The observed plateau
in the magnetic viscosity from 3 K down to 100 mK agrees with the occurrence of
spin tunneling from the ground state Sz = S. However, the scaling M vs Tln(nu
t) is broken below 5 K, suggesting the occurrence of tunneling from excited
states below this temperature.Comment: 4 pages (two columns), 4 figure
How to distinguish between interacting and noninteracting molecules in tunnel junctions
Recent experiments demonstrate a temperature control of the electric
conduction through a ferrocene-based molecular junction. Here we examine the
results in view of determining means to distinguish between transport through
single-particle molecular levels or via transport channels split by Coulomb
repulsion. Both transport mechanisms are similar in molecular junctions given
the similarities between molecular intralevel energies and the charging energy.
We propose an experimentally testable way to identify the main transport
process. By applying a magnetic field to the molecule, we observe that an
interacting theory predicts a shift of the conductance resonances of the
molecule whereas in the noninteracting case each resonance is split into two
peaks. The interaction model works well in explaining our experimental results
obtained in a ferrocene-based single-molecule junction, where the charge
degeneracy peaks shift (but do not split) under the action of an applied
7-Tesla magnetic field. This method is useful for a proper characterization of
the transport properties of molecular tunnel junctions.Comment: Main text: 7 pages, 5 figures; SI: 2 pages, 2 figures. Accepted to
RSC Nanoscal
Low temperature microwave emission from molecular clusters
We investigate the experimental detection of the electromagnetic radiation
generated in the fast magnetization reversal in Mn12-acetate at low
temperatures. In our experiments we used large single crystals and assemblies
of several small single crystals of Mn12-acetate placed inside a cylindrical
stainless steel waveguide in which an InSb hot electron device was also placed
to detect the radiation. All this was set inside a SQUID magnetometer that
allowed to change the magnetic field and measure the magnetic moment and the
temperature of the sample as the InSb detected simultaneously the radiation
emitted from the molecular magnets. Our data show a sequential process in which
the fast inversion of the magnetic moment first occurs, then the radiation is
detected by the InSb device, and finally the temperature of the sample
increases during 15 ms to subsequently recover its original value in several
hundreds of milliseconds.Comment: changed conten
Electrostatic Control over Temperature-Dependent Tunneling across a Single Molecule Junction
Understanding how the mechanism of charge transport through molecular tunnel
junctions depends on temperature is crucial to control electronic function in
molecular electronic devices. With just a few systems investigated as a
function of bias and temperature so far, thermal effects in molecular tunnel
junctions remain poorly understood. Here we report a detailed charge transport
study of an individual redox-active ferrocene-based molecule over a wide range
of temperatures and applied potentials. The results show the temperature
dependence of the current to vary strongly as a function of the gate voltage.
Specifically, the current across the molecule exponentially increases in the
Coulomb blockade regime and decreases at the charge degeneracy points, while
remaining temperature-independent at resonance. Our observations can be well
accounted for by a formal single-level tunneling model where the temperature
dependence relies on the thermal broadening of the Fermi distributions of the
electrons in the leads.Comment: 37 pages, 13 figure
High frequency resonant experiments in Fe molecular clusters
Precise resonant experiments on Fe magnetic clusters have been
conducted down to 1.2 K at various tranverse magnetic fields, using a
cylindrical resonator cavity with 40 different frequencies between 37 GHz and
110 GHz. All the observed resonances for both single crystal and oriented
powder, have been fitted by the eigenstates of the hamiltonian . We have identified the
resonances corresponding to the coherent quantum oscillations for different
orientations of spin S = 10.Comment: to appear in Phys.Rev. B (August 2000
Incommensurate Transverse Anisotropy Induced by Disorder and Spin-Orbit-Vibron Coupling in Mn12-acetate
It has been shown within density-functional theory that in Mn-acetate
there are effects due to disorder by solvent molecules and a coupling between
vibrational and electronic degrees of freedom. We calculate the in-plane
principal axes of the second-order anisotropy caused by the second effect and
compare them with those of the fourth-order anisotropy due to the first effect.
We find that the two types of the principal axes are not commensurate with each
other, which results in a complete quenching of the tunnel-splitting
oscillation as a function of an applied transverse field.Comment: Will be presented at MMM conference 200
Dynamical spin injection at a quasi-one-dimensional ferromagnet-graphene interface
We present a study of dynamical spin injection from a three-dimensional ferromagnet into two-dimensional single-layer graphene. Comparative ferromagnetic resonance (FMR) studies of ferromagnet/graphene strips buried underneath the central line of a coplanar waveguide show that the FMR linewidth broadening is the largest when the graphene layer protrudes laterally away from the ferromagnetic strip, indicating that the spin current is injected into the graphene areas away from the area directly underneath the ferromagnet being excited. Our results confirm that the observed damping is indeed a signature of dynamical spin injection, wherein a pure spin current is pumped into the single-layer graphene from the precessing magnetization of the ferromagnet. The observed spin pumping efficiency is difficult to reconcile with the expected backflow of spins according to the standard spin pumping theory and the characteristics of graphene, and constitutes an enigma for spin pumping in two-dimensional structures
Relaxation and Landau-Zener experiments down to 100 mK in ferritin
Temperature-independent magnetic viscosity in ferritin has been observed from
2 K down to 100 mK, proving that quantum tunneling plays the main role in these
particles at low temperature. Magnetic relaxation has also been studied using
the Landau-Zener method making the system crossing zero resonant field at
different rates, alpha=dH/dt, ranging from 10^{-5} to 10^{-3} T/s, and at
different temperatures, from 150 mK up to the blocking temperature. We propose
a new Tln(Delta H_{eff}/tau_0 alpha) scaling law for the Landau-Zener
probability in a system distributed in volumes, where Delta H_{eff} is the
effective width of the zero field resonance.Comment: 13 pages, 4 postscript figure
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