A quantum photonics model for non-classical light generation using integrated nanoplasmonic cavity-emitter systems

The implementation of non-classical light sources is becoming increasingly important for various quantum applications. A particularly interesting approach is to integrate such functionalities on a single chip as this could pave the way towards fully scalable quantum photonic devices. Several approaches using dielectric systems have been investigated in the past. However, it is still not understood how on-chip nanoplasmonic antennas, interacting with a single quantum emitter, affect the quantum statistics of photons reflected or transmitted in the guided mode of a waveguide. Here we investigate a quantum photonic platform consisting of an evanescently coupled nanoplasmonic cavity-emitter system and discuss the requirements for non-classical light generation. We develop an analytical model that incorporates quenching due to the nanoplasmonic cavity to predict the quantum statistics of the transmitted and reflected guided waveguide light under weak coherent pumping. The analytical predictions match numerical simulations based on a master equation approach. It is moreover shown that for resonant excitation the degree of anti-bunching in transmission is maximized for an optimal cavity modal volume $V_{c}$ and cavity-emitter distance $s$. In reflection, perfectly anti-bunched light can only be obtained for specific $(V_{c},s)$ combinations. Finally, our model also applies to dielectric cavities and as such can guide future efforts in the design and development of on-chip non-classical light sources using dielectric and nanoplasmonic cavity-emitter systems

Enhanced spontaneous raman signal collected evanescently by silicon nitride slot waveguides

We investigate the effect of waveguide geometry on the conversion efficiency of Raman signals collected by integrated photonic waveguides. Compared to strip-type photonic wires, we report a six-fold increase in conversion efficiency for silicon-nitride slot-waveguides

Integration of Single Photon Emitters in 2D Layered Materials with a Silicon Nitride Photonic Chip

Photonic integrated circuits (PICs) enable miniaturization of optical quantum circuits because several optic and electronic functionalities can be added on the same chip. Single photon emitters (SPEs) are central building blocks for such quantum circuits and several approaches have been developed to interface PICs with a host material containing SPEs. SPEs embedded in 2D transition metal dichalcogenides have unique properties that make them particularly appealing as PIC-integrated SPEs. They can be easily interfaced with PICs and stacked together to create complex heterostructures. Since the emitters are embedded in a monolayer there is no total internal reflection, enabling very high light extraction efficiencies without the need of any additional processing to allow efficient single photon transfer between the host and the underlying PIC. Arrays of 2D-based SPEs can moreover be fabricated deterministically through STEM patterning or strain engineering. Finally, 2D materials grown with high wafer-scale uniformity are becoming more readily available, such that they can be matched at the wafer level with underlying PICs. Here we report on the integration of a WSe$_{2}$ monolayer onto a Silicon Nitride (SiN) chip. We demonstrate the coupling of SPEs with the guided mode of a SiN waveguide and study how the on-chip single photon extraction can be maximized by interfacing the 2D-SPE with an integrated dielectric cavity. Our approach allows the use of optimized PIC platforms without the need for additional processing in the host material. In combination with improved wafer-scale CVD growth of 2D materials, this approach provides a promising route towards scalable quantum photonic chips

Enhancement of raman scattering efficiency by a metallic nano-antenna on top of a high index contrast waveguide

We theoretically study coupling of dipole radiation into integrated Si3N4 strip waveguides functionalized with a nanoplasmonic antenna. This structure enables efficient coupling of enhanced Raman signals into the fundamental TE-mode of the waveguide

Surface enhanced Raman spectroscopy using a single mode nanophotonic-plasmonic platform

Surface Enhanced Raman Spectroscopy (SERS) is a well-established technique for enhancing Raman signals. Recently photonic integrated circuits have been used, as an alternative to microscopy based excitation and collection, to probe SERS signals from external metallic nanoparticles. However, in order to develop quantitative on-chip SERS sensors, integration of dedicated nanoplasmonic antennas and waveguides is desirable. Here we bridge this gap by demonstrating for the first time the generation of SERS signals from integrated bowtie nanoantennas, excited and collected by a single mode waveguide, and rigorously quantify the enhancement process. The guided Raman power generated by a 4-Nitrothiophenol coated bowtie antenna shows an 8 x 10^6 enhancement compared to the free-space Raman scattering. An excellent correspondence is obtained between the theoretically predicted and observed absolute Raman power. This work paves the way towards fully integrated lab-on-a-chip systems where the single mode SERS-probe can be combined with other photonic, fluidic or biological functionalities.Comment: Submitted to Nature Photonic

Surface enhanced Raman spectroscopy on single mode nanophotonic-plasmonic waveguides

We analyze the generation of Surface Enhanced Raman Spectroscopy signals from integrated bowtie antennas, excited and collected by a single mode silicon nitride waveguide, and discuss strategies to enhance the Signal-to-Noise Ratio

On-chip enhanced raman spectroscopy using metal slot waveguide

info:eu-repo/semantics/publishe

Nanophotonic waveguide enhanced Raman spectroscopy of biological submonolayers

Characterizing a monolayer of biological molecules has been a major challenge. We demonstrate nanophotonic wave-guide enhanced Raman spectroscopy (NWERS) of monolayers in the near-infrared region, enabling real-time measurements of the hybridization of DNA strands and the density of sub-monolayers of biotin-streptavidin complex immobilized on top of a photonics chip. NWERS is based on enhanced evanescent excitation and collection of spontaneous Raman scattering near nanophotonic waveguides, which for a one centimeter silicon nitride waveguide delivers a signal that is more than four orders of magnitude higher in comparison to a confocal Raman microscope. The reduced acquisition time and specificity of the signal allows for a quantitative and real-time characterization of surface species, hitherto not possible using Raman spectroscopy. NWERS provides a direct analytic tool for monolayer research and also opens a route to compact microscope-less lab-on-a-chip devices with integrated sources, spectrometers and detectors fabricated using a mass-producible CMOS technology platform