254 research outputs found

    Study of intercalation and deintercalation of Na_xCoO_2 yH_2O single crystals

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    Single crystals of NaxCoO2 with beta-phase (x=0.55, 0.60 and 0.65), alpha'-phase (x=0.75) and alpha-phase (x=0.9, 1.0) have been grown by the floating zone technique. The Na-extraction and hydration were carried out for the alpha'-sample to get superconducting phase of NaxCoO2.yH2O (x~0.3, y~1.3). Hydrated single crystals exhibit cracked layers perpendicular to the c-axis due to a large expansion when the water is inserted into the structure. A study of intercalation/deintercalation was performed to determine the stability of the hydrated phase and effects of hydration on the structure of the compound. X-ray diffraction and Thermogravimetric experiments are used to monitor the process of water molecules accommodated in and removed from the crystal lattice. The initial intercalation process takes place with two-water molecules corresponding to y=0.6) inserted in a formula unit, followed by a group of four (y=1.3) to form a cluster of Na(H2O)4. Thermogravimetric analysis suggests that the deintercalation occurs with the removal of the water molecules one by one from the hydrated cluster at elevated temperatures of approximately 50, 100, 200 and 300 C, respectively. Our investigations reveal that the hydration process is dynamic and that water molecule inter- and deintercalation follow different reaction paths in an irreversible way.Comment: 15 pages, 6 figures, figures with higher resolution by email request from the corresponding autho

    A Review of Multi- Compartment Infectious Disease Models

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    Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/156488/2/insr12402.pdfhttp://deepblue.lib.umich.edu/bitstream/2027.42/156488/1/insr12402_am.pd

    The Periodic Instability of Diameter of ZnO Nanowires via a Self-oscillatory Mechanism

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    ZnO nanowires with a periodic instability of diameter were successfully prepared by a thermal physical vapor deposition method. The morphology of ZnO nanowires was investigated by SEM. SEM shows ZnO possess periodic bead-like structure. The instability only appears when the diameter of ZnO nanowires is small. The kinetics and mechanism of Instability was discussed at length. The appearance of the instability is due to negative feed-back mechanism under certain experimental conditions (crystallization temperature, vapor supersaturation, etc)

    Observational constraint on generalized Chaplygin gas model

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    We investigate observational constraints on the generalized Chaplygin gas (GCG) model as the unification of dark matter and dark energy from the latest observational data: the Union SNe Ia data, the observational Hubble data, the SDSS baryon acoustic peak and the five-year WMAP shift parameter. It is obtained that the best fit values of the GCG model parameters with their confidence level are As=0.730.06+0.06A_{s}=0.73^{+0.06}_{-0.06} (1σ1\sigma) 0.09+0.09^{+0.09}_{-0.09} (2σ)(2\sigma), α=0.090.12+0.15\alpha=-0.09^{+0.15}_{-0.12} (1σ1\sigma) 0.19+0.26^{+0.26}_{-0.19} (2σ)(2\sigma). Furthermore in this model, we can see that the evolution of equation of state (EOS) for dark energy is similar to quiessence, and its current best-fit value is w0de=0.96w_{0de}=-0.96 with the 1σ1\sigma confidence level 0.91w0de1.00-0.91\geq w_{0de}\geq-1.00.Comment: 9 pages, 5 figure

    Simulating Poynting Flux Acceleration in the Laboratory with Colliding Laser Pulses

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    We review recent PIC simulation results which show that double-sided irradiation of a thin over-dense plasma slab with ultra-intense laser pulses from both sides can lead to sustained comoving Poynting flux acceleration of electrons to energies much higher than the conventional ponderomotive limit. The result is a robust power-law electron momentum spectrum similar to astrophysical sources. We discuss future ultra-intense laser experiments that may be used to simulate astrophysical particle acceleration.Comment: Paper accepted for publication in the Astrophysics and Space Science, Volume for HEDLA06 conference proceedings, edited by G. Kyrala, in pres

    Combined constraints on modified Chaplygin gas model from cosmological observed data: Markov Chain Monte Carlo approach

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    We use the Markov Chain Monte Carlo method to investigate a global constraints on the modified Chaplygin gas (MCG) model as the unification of dark matter and dark energy from the latest observational data: the Union2 dataset of type supernovae Ia (SNIa), the observational Hubble data (OHD), the cluster X-ray gas mass fraction, the baryon acoustic oscillation (BAO), and the cosmic microwave background (CMB) data. In a flat universe, the constraint results for MCG model are, Ωbh2=0.022630.00162+0.00184\Omega_{b}h^{2}=0.02263^{+0.00184}_{-0.00162} (1σ1\sigma) 0.00195+0.00213^{+0.00213}_{-0.00195} (2σ)(2\sigma), Bs=0.77880.0723+0.0736B_{s}=0.7788^{+0.0736}_{-0.0723} (1σ1\sigma) 0.0904+0.0918^{+0.0918}_{-0.0904} (2σ)(2\sigma), α=0.10790.2539+0.3397\alpha=0.1079^{+0.3397}_{-0.2539} (1σ1\sigma) 0.2911+0.4678^{+0.4678}_{-0.2911} (2σ)(2\sigma), B=0.001890.00756+0.00583B=0.00189^{+0.00583}_{-0.00756} (1σ1\sigma) 0.00915+0.00660^{+0.00660}_{-0.00915} (2σ)(2\sigma), and H0=70.7113.142+4.188H_{0}=70.711^{+4.188}_{-3.142} (1σ1\sigma) 4.149+5.281^{+5.281}_{-4.149} (2σ)(2\sigma).Comment: 12 pages, 1figur

    Prevalence of Type 2 Diabetes among Newly Detected Pulmonary Tuberculosis Patients in China: A Community Based Cohort Study

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    Background: Patients with type 2 diabetes (DM) have a higher risk of developing pulmonary tuberculosis (PTB); moreover, DM co-morbidity in PTB is associated with poor PTB treatment outcomes. Community based prevalence data on DM and prediabetes (pre-DM) among TB patients is lacking, particularly from the developing world. Therefore we conducted a prospective study to investigate the prevalence of DM and pre-DM and evaluated the risk factors for the presence of DM among newly detected PTB patients in rural areas of China. Methods and Findings: In a prospective community based study carried out from 2010 to 2012, a representative sample of 6382 newly detected PTB patients from 7 TB clinics in Linyi were tested for DM. A population of 6674 non-TB controls from the same community was similarly tested as well. The prevalence of DM in TB patients (6.3%) was higher than that in non-TB controls (4.7%, p = 10000 RMB yuan) were positively associated and frequent outdoor activity was negatively associated with DM in PTB patients. Conclusions: The prevalence of DM in PTB patients was higher than in non-TB controls with a 3 fold higher adjusted odds ratio of having DM. Given the increasing DM prevalence and still high burden of TB in China, this association may represent a new public health challenge concerning the prevention and treatment of both diseases
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