Magnetic relaxation and magnetization field dependence measurements in La0.5Ca0.5MnO3

We reported a systematic change in the average magnetic relaxation rate, after the application and removal of a 5 T magnetic field, in a polycrystalline sample of La0.5Ca0.5MnO3. Magnetic relaxation measurements and magnetization versus field curves were taken from 10 K to 160 K. The long time behavior of the relaxation curves was approximately logarithmic in all cases. Keywords: Charge Ordering, Relaxation, Magnetic measurementsComment: 2 figures, accepted to be presented in the International Conference on Magnetism 2000 in Recife, also submitted to Journal of Magnetism and Magnetic Material

Experimental investigation of the flow evolution in the tributary of a 90° open channel confluence

Open channel and river confluences have received a lot of attention in hydraulic literature, because of the interesting flow phenomena observed. Features such as flow acceleration, curvature, separation, mixing and recovery are combined in the confluence area into a complex 3D flow pattern. Typically, the analysis of these features is started at the upstream corner of the confluence area, and the upstream main and tributary branches are considered to be the (uniform) upstream boundary conditions. However, several indications in literature suggest the existence of flow features upstream of the confluence corner. This paper confirms, by means of measurements in a laboratory, 90° confluence flume, considerable streamline curvature in the tributary branch, upstream of the confluence. Furthermore, it shows and quantifies velocity redistribution as well as local water surface super-elevation and depression in the tributary branch. Consequently, flow fea-ture analysis in confluences should start a considerable distance upstream of the confluence

Fabrication of Microstructure Arrays on Photosensitive Glass by Femtosecond Laser

A maskless technique for the fabrication of U-shaped microstructure arrays on the surface of photosensitive glass by femtosecond laser-induced modification is developed. This technique is followed by heat treatment to crystallize the modified area, and the specimen is then placed in acid solution for chemical etching. The surface roughness of the microstructures is further improved by a secondary annealing process. The fabricated photosensitive glass is used as a mold template, and replicated plano-convex cylindrical arrays by UV-replica are also presented. The focusing ability of the microlens arrays on the glass mold and replicate is demonstrated. DOI: 10.2961/jlmn.2012.01.002

Nonperturbative Corrections to One Gluon Exchange Quark Potentials

The leading nonperturbative QCD corrections to the one gluon exchange quark-quark, quark-antiquark and $q \bar{q}$ pair-excitation potentials are derived by using a covariant form of nonlocal two-quark and two-gluon vacuum expectation values. Our numerical calculation indicates that the correction of quark and gluon condensates to the quark-antiquark potential improves the heavy quarkonium spectra to some degree.Comment: LaTex, 16 pages, three figures, to appear in Nucl. Phys.

Imperfections and their passivation in halide perovskite solar cells

All highly-efficient organic–inorganic halide perovskite (OIHP) solar cells to date are made of polycrystalline perovskite films which contain a high density of defects, including point and extended imperfections. The imperfections in OIHP materials play an important role in the process of charge recombination and ion migration in perovskite solar cells (PSC), which heavily influences the resulting device energy conversion efficiency and stability. Here we review the recent advances in passivation of imperfections and suppressing ion migration to achieve improved efficiency and highly stable perovskite solar cells. Due to the ionic nature of OIHP materials, the defects in the photoactive films are inevitably electrically charged. The deep level traps induced by particular charged defects in OIHP films are major non-radiative recombination centers; passivation by coordinate bonding, ionic bonding, or chemical conversion have proven effective in mitigating the negative impacts of these deep traps. Shallow level charge traps themselves may contribute little to non-radiative recombination, but the migration of charged shallow level traps in OIHP films results in unfavorable band bending, interfacial reactions, and phase segregation, influencing the carrier extraction efficiency. Finally, the impact of defects and ion migration on the stability of perovskite solar cells is described

b-physics signals of the lightest CP-odd Higgs in the NMSSM at large tan beta

We investigate the low energy phenomenology of the lighter pseudoscalar $A_1^0$ in the NMSSM. The $A_1^0$ mass can naturally be small due to a global $U(1)_R$ symmetry of the Higgs potential, which is only broken by trilinear soft terms. The $A_1^0$ mass is further protected from renormalization group effects in the large $\tan \beta$ limit. We calculate the $b \to s A_1^0$ amplitude at leading order in $\tan \beta$ and work out the contributions to rare $K$, $B$ and radiative $\Upsilon$-decays and $B -\bar B$ mixing. We obtain constraints on the $A_1^0$ mass and couplings and show that masses down to ${\cal{O}}(10)$ MeV are allowed. The $b$-physics phenomenology of the NMSSM differs from the MSSM in the appearance of sizeable renormalization effects from neutral Higgses to the photon and gluon dipole operators and the breakdown of the MSSM correlation between the $B_s \to \mu^+ \mu^-$ branching ratio and $B_s - \bar B_s$ mixing. For $A_1^0$ masses above the tau threshold the $A_1^0$ can be searched for in $b \to s \tau^+ \tau^-$ processes with branching ratios \lsim 10^{-3}.Comment: 18 pages, 3 figures; references adde

Synergistic Effect of Elevated Device Temperature and Excess Charge Carriers on the Rapid Light-Induced Degradation of Perovskite Solar Cells

With power conversion efficiencies now reaching 24.2%, the major factor limiting efficient electricity generation using perovskite solar cells (PSCs) is their long‐term stability. In particular, PSCs have demonstrated rapid degradation under illumination, the driving mechanism of which is yet to be understood. It is shown that elevated device temperature coupled with excess charge carriers due to constant illumination is the dominant force in the rapid degradation of encapsulated perovskite solar cells under illumination. Cooling the device to 20 °C and operating at the maximum power point improves the stability of CH3NH3PbI3 solar cells over 100× compared to operation under open circuit conditions at 60 °C. Light‐induced strain originating from photothermal‐induced expansion is also observed in CH3NH3PbI3, which excludes other light‐induced‐strain mechanisms. However, strain and electric field do not appear to play any role in the initial rapid degradation of CH3NH3PbI3 solar cells under illumination. It is revealed that the formation of additional recombination centers in PSCs facilitated by elevated temperature and excess charge carriers ultimately results in rapid light‐induced degradation. Guidance on the best methods for measuring the stability of PSCs is also given

Interplay among critical temperature, hole content, and pressure in the cuprate superconductors

Within a BCS-type mean-field approach to the extended Hubbard model, a nontrivial dependence of T_c on the hole content per unit CuO_2 is recovered, in good agreement with the celebrated non-monotonic universal behaviour at normal pressure. Evaluation of T_c at higher pressures is then made possible by the introduction of an explicit dependence of the tight-binding band and of the carrier concentration on pressure P. Comparison with the known experimental data for underdoped Bi2212 allows to single out an `intrinsic' contribution to d T_c / d P from that due to the carrier concentration, and provides a remarkable estimate of the dependence of the inter-site coupling strength on the lattice scale.Comment: REVTeX 8 pages, including 5 embedded PostScript figures; other required macros included; to be published in Phys. Rev. B (vol. 54

Ultrafast Exciton Transport with a Long Diffusion Length in Layered Perovskites with Organic Cation Functionalization

Layered perovskites have been employed for various optoelectronic devices including solar cells and light-emitting diodes for improved stability, which need exciton transport along both the in-plane and the out-of-plane directions. However, it is not clear yet what determines the exciton transport along the in-plane direction, which is important to understand its impact toward electronic devices. Here, by employing both steady-state and transient photoluminescence mapping, it is found that in-plane exciton diffusivities in layered perovskites are sensitive to both the number of layers and organic cations. Apart from exciton–phonon coupling, the octahedral distortion is revealed to significantly affect the exciton diffusion process, determined by temperature-dependent photoluminescence, light-intensity-dependent time-resolved photoluminescence, and density function theory calculations. A simple fluorine substitution to phenethylammonium for the organic cations to tune the structural rigidity and octahedral distortion yields a record exciton diffusivity of 1.91 cm2 s−1 and a diffusion length of 405 nm along the in-plane direction. This study provides guidance to manipulate exciton diffusion by modifying organic cations in layered perovskites

Pathogenesis of non-alcoholic fatty liver disease

Non-alcoholic fatty liver disease (NAFLD) represents a spectrum of disease ranging from hepatocellular steatosis through steatohepatitis to fibrosis and irreversible cirrhosis. The prevalence of NAFLD has risen rapidly in parallel with the dramatic rise in obesity and diabetes, and is rapidly becoming the most common cause of liver disease in Western countries. Indeed, NAFLD is now recognized to be the aetiology in many cases previously labelled as cryptogenic cirrhosis