Electron Paramagnetic Resonance of Single Magnetic Moment on a Surface

We address electron spin resonance of single magnetic moments in a tunnel junction using time-dependent electric fields and spin-polarized current. We show that the tunneling current directly depends on the local magnetic moment and that the frequency of the external electric field mixes with the characteristic Larmor frequency of the local spin. The importance of the spin-polarized current induced anisotropy fields acting on the local spin moment is, moreover, demonstrated. Our proposed model thus explains the absence of an electron spin resonance for a half integer spin, in contrast with the strong signal observed for an integer spin.Comment: 6 pages, 2 figures, as publishe

Spin Inelastic Electron Tunneling Spectroscopy on Local Magnetic Moment Embedded in Josephson Junction

Recent experimental conductance measurements performed on paramagnetic molecular adsorbates on a superconducting surface, using superconducting scanning tunneling microscopy techniques, are theoretically investigated. For low temperatures, we demonstrate that tunneling current assisted excitations of the local magnetic moment cannot occur for voltage biases smaller than the superconducting gap of the scanning tunneling microscope. The magnetic moment is only excited for voltages corresponding to the sum of the superconducting gap and the spin excitation energies. In excellent agreement with experiment, we show that pumping into higher excitations give additional current signatures by accumulation of density in the lower ones. Using external magnetic fields, we Zeeman split possible degeneracy and thereby resolve all excitations comprised in the magnetic moment.Comment: 6 pages, 4 figures, submitte

The X-ray and radio emission from SN 2002ap: The importance of Compton scattering

The radio and X-ray observations of the Type Ic supernova SN 2002ap are modeled. We find that inverse Compton cooling by photospheric photons explains the observed steep radio spectrum, and also the X-ray flux observed by XMM. Thermal emission from the shock is insufficient to explain the X-ray flux. The radio emitting region expands with a velocity of, roughly, 70,000 km/s. From the ratio of X-ray to radio emission we find that the energy densities of magnetic fields and relativistic electrons are close to equipartion.Comment: 15 pages, 2 figures, ApJ accepte

Theory of spin inelastic tunneling spectroscopy for superconductor-superconductor and superconductor-metal junctions

We address the tunneling conductance and spin inelastic tunneling spectroscopy of localized paramagnetic moments in a superconducting environment, pertaining to recent measurements on Fe-octaethylporphyrin-chloride using superconducting scanning tunneling microscopy. We demonstrate that the Cooper pair correlations in the tip and substrate generate a finite uniaxial anisotropy field acting on the local spin moment, and we argue that this field may be a source for the observed changes in the conductance spectrum for decreasing distance between the scanning tunneling tip and the local magnetic moment. We make a side-by-side comparison between the superconductor-superconductor junction and normal-metal--superconductor junction, and find qualitative agreement between the two setups while quantitative differences become explicit. When simulating the effects of electron pumping, we obtain additional peaks in the conductance spectrum that can be attributed to excitations between higher-energy spin states. The transverse anisotropy field couples basis states of the local spin which opens for transitions between spin states that are otherwise forbidden by conservation of angular momentum. Finally, we explore the influences of temperature, which tend to enable in-gap transitions, and an external magnetic field, which enables deeper studies of the spin excitation spectrum. We especially notice the appearance of a low and high excitation peak on each side of the main coherence peak as an imprint of transitions between the Zeeman split ground states.Comment: 14 pages, 8 figure

Microscopic Theory for Coupled Atomistic Magnetization and Lattice Dynamics

A coupled atomistic spin and lattice dynamics approach is developed which merges the dynamics of these two degrees of freedom into a single set of coupled equations of motion. The underlying microscopic model comprises local exchange interactions between the electron spin and magnetic moment and the local couplings between the electronic charge and lattice displacements. An effective action for the spin and lattice variables is constructed in which the interactions among the spin and lattice components are determined by the underlying electronic structure. In this way, expressions are obtained for the electronically mediated couplings between the spin and lattice degrees of freedom, besides the well known inter-atomic force constants and spin-spin interactions. These former susceptibilities provide an atomistic ab initio description for the coupled spin and lattice dynamics. It is important to notice that this theory is strictly bilinear in the spin and lattice variables and provides a minimal model for the coupled dynamics of these subsystems and that the two subsystems are treated on the same footing. Questions concerning time-reversal and inversion symmetry are rigorously addressed and it is shown how these aspects are absorbed in the tensor structure of the interaction fields. By means of these results regarding the spin-lattice coupling, simple explanations of ionic dimerization in double anti-ferromagnetic materials, as well as, charge density waves induced by a non-uniform spin structure are given. In the final parts, a set of coupled equations of motion for the combined spin and lattice dynamics are constructed, which subsequently can be reduced to a form which is analogous to the Landau-Lifshitz-Gilbert equations for spin dynamics and damped driven mechanical oscillator for the ...Comment: 22 pages, including 7 pages of Appendix and references, 6 figure

Theory of spin-polarized scanning tunneling microscopy applied to local spins

We provide a theory for scanning tunneling microscopy and spectroscopy using a spin-polarized tip. It it shown that the tunneling conductance can be partitioned into three separate contributions, a background conductance which is independent of the local spin, a dynamical conductance which is proportional to the local spin moment, and a conductance which is proportional to the noise spectrum of the local spin interactions. The presented theory is applicable to setups with magnetic tip and substrate in non-collinear arrangement, as well as for non-magnetic situations. The partitioning of the tunneling current suggests a possibility to extract the total spin moment of the local spin from the dynamical conductance. The dynamical conductance suggests a possibility to generate very high frequency spin-dependent ac currents and/or voltages. We also propose a measurement of the dynamical conductance that can be used to determine the character of the effective exchange interaction between individual spins in clusters. The third contribution to the tunneling current is associated with the spin-spin correlations induced by the exchange interaction between the local spin moment and the tunneling electrons. We demonstrate how this term can be used in the analysis of spin excitations recorded in conductance measurements. Finally, we propose to use spin-polarized scanning tunneling microscopy for detailed studies of the spin excitation spectrum.Comment: 12 pages, 4 figure, updated to match the published version, to appear in the Phys. Rev.

Signatures of band-like tunnelling in granular nanowires

We explore the problem of tunneling through disorderd nanowires, comprised of a random distribution of metallic grains, by means of a many-body model that captures the essential physics of the system. The random configuration of grains gives rise to a smooth band-like set of states, which mediates current flow through the nanowire. Analytical and numerical calculations show the characteristic signature of this unusual band-like transport to be a quadratic variation of the current as a function of the applied voltage (i.e. $I\sim V^2$), a variation that is clearly observed in experimental studies of Pt/C composite nanowires.Comment: 4 pages, 3 figures. submitted to the Physcal Review

Simultaneous XMM-Newton and ESO VLT observations of SN 1995N: probing the wind/ejecta interaction

We present the results of the first {\it XMM-Newton} observation of the interacting type IIn supernova 1995N, performed in July 2003. We find that the 0.2--10.0 keV unabsorbed flux dropped at a value of $\simeq 1.8 \times 10^{-13}$ erg cm$^{-2}$ s$^{-1}$, almost one order of magnitude lower than that of a previous {\it ASCA} observation of January 1998. From all the available X-ray measurements, an interesting scenario emerges where the X-ray light emission may be produced by a two-phase (clumpy/smooth) circumstellar medium. The X-ray spectral analysis shows statistically significant evidence for the presence of two distinct components, that can be modeled with emission from optically thin, thermal plasmas at different temperatures. The exponent of the ejecta density distribution inferred from these temperatures is $n\simeq 6.4$. From the fluxes of the two spectral components we derive an estimate of the mass loss rate of the supernova progenitor, ${\dot M} \sim 2 \times 10^{-4} M_\odot {\rm yr}^{-1}$, at the upper end of the interval exhibited by red super-giants. Coordinated optical and infrared observations allow us to reconstruct the simultaneous infrared to X-ray flux distribution of SN 1995N. We find that, at $\sim$ 9 years after explosion, the direct X-ray thermal emission due to the wind/ejecta interaction is $\sim 5$ times larger than the total reprocessed IR/optical flux.Comment: 11 pages, 7 figures, MNRAS, in pres