197 research outputs found
Simultaneous estimation of groundwater recharge and hydrodynamic parameters for groundwater flow modeling
International audienc
First identification of large electric monopole strength in well-deformed rare earth nuclei
Excited states in the well-deformed rare earth isotopes Sm and
Er were populated via ``safe'' Coulomb excitation at the Munich MLL
Tandem accelerator. Conversion electrons were registered in a cooled Si(Li)
detector in conjunction with a magnetic transport and filter system, the
Mini-Orange spectrometer. For the first excited state in Sm at
1099 keV a large value of the monopole strength for the transition to the
ground state of could be extracted. This confirms the interpretation of the lowest
excited state in Sm as the collective -vibrational
excitation of the ground state. In Er the measured large electric
monopole strength of clearly identifies the state at 1934 keV to be the
-vibrational excitation of the ground state.Comment: submitted to Physics Letters
Study of bound states in 12Be through low-energy 11Be(d,p)-transfer reactions
The bound states of 12Be have been studied through a 11Be(d,p)12Be transfer
reaction experiment in inverse kinematics. A 2.8 MeV/u beam of 11Be was
produced using the REX-ISOLDE facility at CERN. The outgoing protons were
detected with the T-REX silicon detector array. The MINIBALL germanium array
was used to detect gamma rays from the excited states in 12Be. The gamma-ray
detection enabled a clear identification of the four known bound states in
12Be, and each of the states has been studied individually. Differential cross
sections over a large angular range have been extracted. Spectroscopic factors
for each of the states have been determined from DWBA calculations and have
been compared to previous experimental and theoretical results
First Results on In-Beam gamma Spectroscopy of Neutron-Rich Na and Mg Isotopes at REX-ISOLDE
After the successful commissioning of the radioactive beam experiment at
ISOLDE (REX-ISOLDE) - an accelerator for exotic nuclei produced by ISOLDE -
first physics experiments using these beams were performed. Initial experiments
focused on the region of deformation in the vicinity of the neutron-rich Na and
Mg isotopes. Preliminary results show the high potential and physics
opportunities offered by the exotic isotope accelerator REX in conjunction with
the modern Germanium gamma spectrometer MINIBALL.Comment: 7 pages, RNB6 conference contributio
Design of a 2-D Cementation Experiment in Porous Medium Using Numerical Simulation
International audienceThe validation and qualification of reactive transport simulation tools has motivated the design and simulation, at a laboratory scale, of an experiment in which flow, advective/dispersive transport of solutes and physicochemical transformation affecting a porous medium are strongly coupled. Several possible experimental setups (or designs) have been evaluated using numerical simulation. The selected experimental design involves the successive precipitation and perforation of a clogging obstacle composed of calcium oxalate. Before an experiment can actually be conducted, this problem is proposed as a numerical benchmark for reactive transport codes and simulated using the coupled reactive transport code Hytec (CIG-École des mines, France)
Approaches to Modeling Coupled Flow and Reaction in a 2-D Cementation Experiment
Porosity evolution at reactive interfaces is a key process that governs the evolution and performances of many engineered systems that have important applications in earth and environmental sciences. This is the case, for example, at the interface between cement structures and clays in deep geological nuclear waste disposals. Although in a different transport regime, similar questions arise for permeable reactive barriers used for biogeochemical remediation in surface environments. The COMEDIE project aims at investigating the coupling between transport, hydrodynamics and chemistry when significant variations of porosity occur. The present work focuses on a numerical benchmark used as a design exercise for the future COMEDIE-2D experiment. The use of reactive transport simulation tools like Hytec and Crunch provides predictions of the physico-chemical evolutions that are expected during the future experiments in laboratory. Focus is given in this paper on the evolution during the simulated experiment of precipitate, permeability and porosity fields. A first case is considered in which the porosity is constant. Results obtained with Crunch and Hytec are in relatively good agreement. Differences are attributable to the models of reactive surface area taken into account for dissolution/precipitation processes. Crunch and Hytec simulations taking into account porosity variations are then presented and compared. Results given by the two codes are in qualitative agreement, with differences attributable in part to the models of reactive surface area for dissolution/precipitation processes. As a consequence, the localization of secondary precipitates predicted by Crunch leads to lower local porosities than for predictions obtained by Hytec and thus to a stronger coupling between flow and chemistry. This benchmark highlights the importance of the surface area model employed to describe systems in which strong porosity variations occur as a result of dissolution/precipitation. The simulation of highly non-linear reactive transport systems is also shown to be partly dependent on specific numerical approaches
"Safe" Coulomb Excitation of 30Mg
We report on the first radioactive beam experiment performed at the recently
commissioned REX-ISOLDE facility at CERN in conjunction with the highly
efficient gamma spectrometer MINIBALL. Using 30Mg ions accelerated to an energy
of 2.25 MeV/u together with a thin nat-Ni target, Coulomb excitation of the
first excited 2+ states of the projectile and target nuclei well below the
Coulomb barrier was observed. From the measured relative de-excitation gamma
ray yields the B(E2; 0+ -> 2+) value of 30Mg was determined to be 241(31)
e2fm4. Our result is lower than values obtained at projectile fragmentation
facilities using the intermediate-energy Coulomb excitation method, and
confirms the theoretical conjecture that the neutron-rich magnesium isotope
30Mg lies still outside the ``island of inversion''
Spectroscopy of Na: shell evolution toward the drip line
Excited states in Na have been studied using the -decay of
implanted Ne ions at GANIL/LISE as well as the in-beam -ray
spectroscopy at the NSCL/S800 facility. New states of positive
(J=3,4) and negative (J=1-5) parity are proposed. The
former arise from the coupling between 0d protons and a 0d
neutron, while the latter are due to couplings with 1p or 0f
neutrons. While the relative energies between the J=1-4 states are
well reproduced with the USDA interaction in the N=17 isotones, a progressive
shift in the ground state binding energy (by about 500 keV) is observed between
F and Al. This points to a possible change in the proton-neutron
0d-0d effective interaction when moving from stability to the
drip line. The presence of J=1-4 negative parity states around 1.5
MeV as well as of a candidate for a J=5 state around 2.5 MeV give
further support to the collapse of the N=20 gap and to the inversion between
the 0f and 1p levels below Z=12. These features are discussed
in the framework of Shell Model and EDF calculations, leading to predicted
negative parity states in the low energy spectra of the F and O
nuclei.Comment: Exp\'erience GANIL/LISE et NSCL/S80
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Characterization and Source Term Assessments of Radioactive Particles from Marshall Islands Using Non-Destructive Analytical Techniques
A considerable fraction of radioactivity entering the environment from different nuclear events is associated with particles. The impact of these events can only be fully assessed where there is some knowledge about the mobility of particle bound radionuclides entering the environment. The behavior of particulate radionuclides is dependent on several factors, including the physical, chemical and redox state of the environment, the characteristics of the particles (e.g., the chemical composition, crystallinity and particle size) and on the oxidative state of radionuclides contained in the particles. Six plutonium-containing particles stemming from Runit Island soil (Marshall Islands) were characterized using non-destructive analytical and microanalytical methods. By determining the activity of {sup 239,240}Pu and {sup 241}Am isotopes from their gamma peaks structural information related to Pu matrix was obtained, and the source term was revealed. Composition and elemental distribution in the particles were studied with synchrotron radiation based micro X-ray fluorescence (SR-{mu}-XRF) spectrometry. Scanning electron microscope equipped with energy dispersive X-ray detector (SEMEDX) and secondary ion mass spectrometer (SIMS) were used to examine particle surfaces. Based on the elemental composition the particles were divided into two groups; particles with plain Pu matrix, and particles where the plutonium is included in Si/O-rich matrix being more heterogeneously distributed. All of the particles were identified as fragments of initial weapons material. As containing plutonium with low {sup 240}Pu/{sup 239}Pu atomic ratio, {approx}2-6%, which corresponds to weapons grade plutonium, the source term was identified to be among the safety tests conducted in the history of Runit Island
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