Charge-Density-Wave Ordering in the Metal-Insulator Transition Compound PrRu4P12

X-ray and electron diffraction measurements on the metal-insulator (M-I) transition compound PrRu$_4$P$_{12}$ have revealed the emergence of a periodic ordering of charge density around the Pr atoms. It is found that the ordering is associated with the onset of a low temperature insulator phase. These conclusions are supported by the facts that the space group of the crystal structure transforms from Im$\bar{3}$ to Pm$\bar{3}$ below the M-I transition temperature and also that the temperature dependence of the superlattice peaks in the insulator phase follows the squared BCS function. The M-I transition could be originated from the perfect nesting of the Fermi surface and/or the instability of the $f$ electrons.Comment: 4 pages, 5 figures, Phys. Rev. B (2004) (in press

Thin Ice Target for 16^{16}O(p,p') experiment

A windowless and self-supporting ice target is described. An ice sheet with a thickness of 29.7 mg/cm$^2$ cooled by liquid nitrogen was placed at the target position of a magnetic spectrometer and worked stably in the $^{16}$O$(p,p')$ experiment at $E_{p}=392$ MeV. Background-free spectra were obtained.Comment: 14 pages, 4 figures, Nucl. Instr. & Meth. A (in press

Complete set of polarization transfer coefficients for the 3He(p,n){}^{3}{\rm He}(p,n) reaction at 346 MeV and 0 degrees

We report measurements of the cross-section and a complete set of polarization transfer coefficients for the ${}^{3}{\rm He}(p,n)$ reaction at a bombarding energy $T_p$ = 346 MeV and a reaction angle $\theta_{\rm lab}$ = $0^{\circ}$. The data are compared with the corresponding free nucleon-nucleon values on the basis of the predominance of quasi-elastic scattering processes. Significant discrepancies have been observed in the polarization transfer $D_{LL}(0^{\circ})$, which are presumably the result of the three-proton $T$ = 3/2 resonance. The spin--parity of the resonance is estimated to be $1/2^-$, and the distribution is consistent with previous results obtained for the same reaction at $T_p$ = 48.8 MeV.Comment: 4 figures, Accepted for publication in Physical Review

Recent Surface Studies Using Biassed Secondary Electron Imaging

The growth and surface diffusion of Cs on Si(100) and Ag on Fe(110) have been studied using biassed secondary electron imaging (b-SEI) and Auger electron spectroscopy (AES). The b-SEI technique was found capable of detecting Cs on the Si surface with a 0.5% ML sensitivity. Unusual diffusion profiles containing linear sections were obtained for coverages (θ) \u3c 1/2 ML. The general form of these profiles were reproduced using a 2-phase model, where Cs chains act as sources of mobile adatoms, in conjunction with a diffusion coefficient of the form D ~ θ (1- Cθ). This form of D, obtained from Boltzmann-Matano analysis, is consistent with diffusion theory including strongly repulsive Cs-Cs interactions. An adatom diffusion energy, Ed, = 0.47 ± 0.05 eV was found to be consistent with measurements of the diffusion coefficient made in the temperature range 333 ≤ T ≤ 363K. The growth mode for Ag on Fe(110) was determined by AES and b-SEI to be Stranski-Krastanov, with islands growing on top of two intermediate layers. Diffusion experiments conducted on finite Ag patches show that following annealing, adatoms dissociate from the islands and second monolayer and contribute to the observed expansion of the first monolayer. The diffusion results also indicate that while islands are still present, there is a competition between adatoms entering and leaving the second monolayer

Tight-binding parameters and exchange integrals of Ba_2Cu_3O_4Cl_2

Band structure calculations for Ba_2Cu_3O_4Cl_2 within the local density approximation (LDA) are presented. The investigated compound is similar to the antiferromagnetic parent compounds of cuprate superconductors but contains additional Cu_B atoms in the planes. Within the LDA, metallic behavior is found with two bands crossing the Fermi surface (FS). These bands are built mainly from Cu 3d_{x^2-y^2} and O 2p_{x,y} orbitals, and a corresponding tight-binding (TB) model has been parameterized. All orbitals can be subdivided in two sets corresponding to the A- and B-subsystems, respectively, the coupling between which is found to be small. To describe the experimentally observed antiferromagnetic insulating state, we propose an extended Hubbard model with the derived TB parameters and local correlation terms characteristic for cuprates. Using the derived parameter set we calculate the exchange integrals for the Cu_3O_4 plane. The results are in quite reasonable agreement with the experimental values for the isostructural compound Sr_2Cu_3O_4Cl_2.Comment: 5 pages (2 tables included), 4 ps-figure

Study of nuclear correlation effects via 12C(p,n)12N(g.s.,1+) at 296 MeV

We report measurements of the cross section and a complete set of polarization observables for the Gamow--Teller ${}^{12}{\rm C}(\vec{p},\vec{n}){}^{12}{\rm N}({\rm g.s.},1^+)$ reaction at a bombarding energy of 296 MeV. The data are compared with distorted wave impulse approximation calculations employing transition form factors normalized to reproduce the observed beta-decay $ft$ value. The cross section is significantly under-predicted by the calculations at momentum transfers $q \gtrsim$ 0.5 ${\rm fm^{-1}}$. The discrepancy is partly resolved by considering the non-locality of the nuclear mean field. However, the calculations still under-predict the cross section at large momentum transfers of $q$ $\simeq$ 1.6 ${\rm fm^{-1}}$. We also performed calculations employing random phase approximation response functions and found that the observed enhancement can be attributed in part to pionic correlations in nuclei.Comment: 5 figures, submitted to Phys. Lett.

Three-Dimensional Simulations of Mixing Instabilities in Supernova Explosions

We present the first three-dimensional (3D) simulations of the large-scale mixing that takes place in the shock-heated stellar layers ejected in the explosion of a 15.5 solar-mass blue supergiant star. The outgoing supernova shock is followed from its launch by neutrino heating until it breaks out from the stellar surface more than two hours after the core collapse. Violent convective overturn in the post-shock layer causes the explosion to start with significant asphericity, which triggers the growth of Rayleigh-Taylor (RT) instabilities at the composition interfaces of the exploding star. Deep inward mixing of hydrogen (H) is found as well as fast-moving, metal-rich clumps penetrating with high velocities far into the H-envelope of the star as observed, e.g., in the case of SN 1987A. Also individual clumps containing a sizeable fraction of the ejected iron-group elements (up to several 0.001 solar masses) are obtained in some models. The metal core of the progenitor is partially turned over with Ni-dominated fingers overtaking oxygen-rich bullets and both Ni and O moving well ahead of the material from the carbon layer. Comparing with corresponding 2D (axially symmetric) calculations, we determine the growth of the RT fingers to be faster, the deceleration of the dense metal-carrying clumps in the He and H layers to be reduced, the asymptotic clump velocities in the H-shell to be higher (up to ~4500 km/s for the considered progenitor and an explosion energy of 10^{51} ergs, instead of <2000 km/s in 2D), and the outward radial mixing of heavy elements and inward mixing of hydrogen to be more efficient in 3D than in 2D. We present a simple argument that explains these results as a consequence of the different action of drag forces on moving objects in the two geometries. (abridged)Comment: 15 pages, 8 figures, 30 eps files; significantly extended and more figures added after referee comments; accepted by The Astrophysical Journa

Anomalous Spin Dynamics observed by High Frequency ESR in Honeycomb Lattice Antiferromagnet InCu2/3V1/3O3

High-frequency ESR results on the S=1/2 Heisenberg hexagonal antiferromagnet InCu2/3V1/3O3 are reported. This compound appears to be a rare model substance for the honeycomb lattice antiferromagnet with very weak interlayer couplings. The high-temperature magnetic susceptibility can be interpreted by the S=1/2 honeycomb lattice antiferromagnet, and it shows a magnetic-order-like anomaly at TN=38 K. Although, the resonance field of our high-frequency ESR shows the typical behavior of the antiferromagnetic resonance, the linewidth of our high-frequency ESR continues to increase below TN, while it tends to decrease as the temperature in a conventional three-dimensional antiferromagnet decreases. In general, a honeycomb lattice antiferromagnet is expected to show a simple antiferromagnetic order similar to that of a square lattice antiferromagnet theoretically because both antiferromagnets are bipartite lattices. However, we suggest that the observed anomalous spin dynamics below TN is the peculiar feature of the honeycomb lattice antiferromagnet that is not observed in the square lattice antiferromagnet.Comment: 5 pages, 5 figure

Hard-core Yukawa model for two-dimensional charge stabilized colloids

The hyper-netted chain (HNC) and Percus-Yevick (PY) approximations are used to study the phase diagram of a simple hard-core Yukawa model of charge-stabilized colloidal particles in a two-dimensional system. We calculate the static structure factor and the pair distribution function over a wide range of parameters. Using the statics correlation functions we present an estimate for the liquid-solid phase diagram for the wide range of the parameters.Comment: 7 pages, 9figure