Characterization of Cs vapor cell coated with octadecyltrichlorosilane using coherent population trapping spectroscopy

We report the realization and characterization using coherent population trapping (CPT) spectroscopy of an octadecyltrichlorosilane (OTS)-coated centimeter-scale Cs vapor cell. The dual-structure of the resonance lineshape, with presence of a narrow structure line at the top of a Doppler-broadened structure, is clearly observed. The linewidth of the narrow resonance is compared to the linewidth of an evacuated Cs cell and of a buffer gas Cs cell of similar size. The Cs-OTS adsorption energy is measured to be (0.42 $\pm$ 0.03) eV, leading to a clock frequency shift rate of $2.7\times10^{-9}/$K in fractional unit. A hyperfine population lifetime, $T_1$, and a microwave coherence lifetime, $T_2$, of 1.6 and 0.5 ms are reported, corresponding to about 37 and 12 useful bounces, respectively. Atomic-motion induced Ramsey narrowing of dark resonances is observed in Cs-OTS cells by reducing the optical beam diameter. Ramsey CPT fringes are detected using a pulsed CPT interrogation scheme. Potential applications of the Cs-OTS cell to the development of a vapor cell atomic clock are discussed.Comment: 33 pages, 13 figure

Sub-Doppler spectroscopy of the near-UV Cs atom 6S1/2_{1/2}-7P1/2_{1/2} transition in a microfabricated vapor cell

We report on the characterization of sub-Doppler resonances detected by probing the 6S$_{1/2}$-7P$_{1/2}$ transition of Cs atom at 459 nm in a microfabricated vapor cell. The dependence of the sub-Doppler resonance (linewidth, amplitude) on some key experimental parameters, including the laser intensity and the cell temperature, is investigated. These narrow atomic resonances are of interest for high-resolution spectroscopy, instrumentation, and may constitute the basis of a near-UV microcell optical standard

Investigations for a Miniature Optical Frequency Reference Based on High-Contrast Sub-Doppler Resonance in a MEMS Cesium Vapor Cell

International audienceMany of modern quantum technologies require the development of high-performance and low-power consumption miniaturized devices such as laser systems, atomic clocks, magnetometers and other quantum sensors. These instruments are to date often based on the use of chip-size diode lasers and microfabricated (MEMS) cells filled with alkali atoms [1]. An interesting challenge concerns the development of miniaturized optical frequency references (OFR). Different approaches have been engaged in this direction. One of the most successful example is a rubidium microcell-based OFR, involving the two-photon spectroscopy technique. This approach has recently demonstrated a remarkable frequency stability level of 4.4×10–12 at 1 s [2]. The present study is focused on a simple alternative approach based on sub-Doppler spectroscopy (SDS) with counter-propagating light beams. We propose to use dual-frequency light beams with orthogonal linear polarizations and frequency difference w1–w2 = Dhfs, with Dhfs the frequency of the atom ground-state hyper-fine splitting. First dual-frequency sub-Doppler spectroscopy (DF SDS) experiments have been performed with cmscale cells [3,4]. In the present study, we present preliminary spectroscopy and frequency stability results of alaser stabilized using DF SDS with a Cs vapor microfabricated cell [5] (Fig.1a). An extended-cavity diode laser (ECDL) source and a Mach-Zehnder intensity EOM are used to obtain the dual-frequency light field. A forward beam goes through the cell and is then reflected by a mirror to create the backward beam

On the reduction of gas permeation through the glass windows of micromachined vapor cells using Al2_{2}O3_{3} coatings

Stability and precision of atomic devices are closely tied to the quality and stability of the internal atmosphere of the atomic vapor cells on which they rely. Such atmosphere can be stabilized by building the cell with low permeation materials such as sapphire, or aluminosilicate glass in microfabricated devices. Recently, we showed that permeation barriers made of Al$_{2}$O$_{3}$ thin-film coatings deposited on standard borosilicate glass could be an alternative for buffer gas pressure stabilization. In this study, we hence investigate how helium permeation is influenced by the thickness, ranging from 5 to 40 nm, of such Al$_{2}$O$_{3}$ thin-films coated by atomic layer deposition. Permeation rates are derived from long-term measurements of the pressure-shifted transition frequency of a coherent population trapping (CPT) atomic clock. From thicknesses of 20 nm onward, a significant enhancement of the cell hermeticity is experienced, corresponding to two orders of magnitude lower helium permeation rate. In addition, we test cesium vapor cells filled with neon as a buffer gas and whose windows are coated with 20 nm of Al$_{2}$O$_{3}$. As for helium, the permeation rate of neon is significantly reduced thanks to alumina coatings, leading to a fractional frequency stability of 4x10$^{-12}$ at 1 day when the cell is used in a CPT clock. These features outperform the typical performances of uncoated Cs-Ne borosilicate cells and highlight the significance of Al$_{2}$O$_{3}$ coatings for buffer gas pressure stabilization.Comment: 6 pages, 4 figure

Laser light routing in an elongated micromachined vapor cell with diffraction gratings for atomic clock applications

International audienceThis paper reports on an original architecture of microfabricated alkali vapor cell designed for miniature atomic clocks. The cell combines diffraction gratings with anisotropically etched single-crystalline silicon sidewalls to route a normally-incident beam in a cavity oriented along the substrate plane. Gratings have been specifically designed to diffract circularly polarized light in the first order, the latter having an angle of diffraction matching the (111) sidewalls orientation. Then, the length of the cavity where light interacts with alkali atoms can be extended. We demonstrate that a longer cell allows to reduce the beam diameter, while preserving the clock performances. As the cavity depth and the beam diameter are reduced, collimation can be performed in a tighter space. This solution relaxes the constraints on the device packaging and is suitable for wafer-level assembly. Several cells have been fabricated and characterized in a clock setup using coherent population trapping spectroscopy. The measured signals exhibit null power linewidths down to 2.23 kHz and high transmission contrasts up to 17%. A high contrast-to-linewidth ratio is found at a linewidth of 4.17 kHz and a contrast of 5.2% in a 7-mm-long cell despite a beam diameter reduced to 600 μm

Utilisation d'éléments optiques diffractifs binaires pour la mise en forme et l'amélioration des performances des lasers solides

CAEN-BU Sciences et STAPS (141182103) / SudocSudocFranceF

Microfabrication of axicons by glass blowing at a wafer-level

International audienceThis Letter reports on the generation of glass-based axicons realized at the wafer level by means of microfabrication. The technique is based on micro glass blowing allowing parallel fabrication of numerous components at a time. Blowing is achieved due to cavities containing a gas that expands when the wafer stack is introduced in a furnace. Such cavities, generated in a silicon wafer and sealed by a bonded glass wafer, act as pistons pushing locally the other side of the glass wafer where the micro-optical component profile emerges. After cavities’ removal by polishing, it is shown that such a component produces nondiffracting Bessel beams

Preliminary studies of Rb microfabricated cells for a two-photon Rb optical frequency reference

International audienceDoppler-free two-photon absorption spectroscopy is employed to characterize the purity of rubidium vapor micro-fabricated cells. The observed broadening suggests the presence of impurities and contaminants in the cell