Decay Properties of 266^{266}Bh and 262^{262}Db Produced in the 248^{248}Cm + 23^{23}Na Reaction

Decay properties of an isotope $^{266}$Bh and its daughter nucleus $^{262}$Db produced by the $^{248}$Cm($^{23}$Na, 5\textit{n}) reaction were studied by using a gas-filled recoil separator coupled with a position-sensitive semiconductor detector. $^{266}$Bh was clearly identified from the correlation of the known nuclide, $^{262}$Db. The obtained decay properties of $^{266}$Bh and $^{262}$Db are consistent with those observed in the $^{278}$113 chain, which provided further confirmation of the discovery of $^{278}$113.Comment: Accepted for publication in J. Phys. Soc. JPN., to be published in Vol.78 No.

Future of superheavy element research: Which nuclei could be synthesized within the next few years?

Low values of the fusion cross sections and very short half-lives of nuclei with Z$>$120 put obstacles in synthesis of new elements. Different nuclear reactions (fusion of stable and radioactive nuclei, multi-nucleon transfers and neutron capture), which could be used for the production of new isotopes of superheavy (SH) elements, are discussed in the paper. The gap of unknown SH nuclei, located between the isotopes which were produced earlier in the cold and hot fusion reactions, can be filled in fusion reactions of $^{48}$Ca with available lighter isotopes of Pu, Am, and Cm. Cross sections for the production of these nuclei are predicted to be rather large, and the corresponding experiments can be easily performed at existing facilities. For the first time, a narrow pathway is found to the middle of the island of stability owing to possible $\beta^+$-decay of SH isotopes which can be formed in ordinary fusion reactions of stable nuclei. Multi-nucleon transfer processes at near barrier collisions of heavy (and very heavy, U-like) ions are shown to be quite realistic reaction mechanism allowing us to produce new neutron enriched heavy nuclei located in the unexplored upper part of the nuclear map. Neutron capture reactions can be also used for the production of the long-living neutron rich SH nuclei. Strong neutron fluxes might be provided by pulsed nuclear reactors and by nuclear explosions in laboratory conditions and by supernova explosions in nature. All these possibilities are discussed in the paper.Comment: An Invited Plenary Talk given by Valeriy I. Zagrebaev at the 11th International Conference on Nucleus-Nucleus Collisions (NN2012), San Antonio, Texas, USA, May 27-June 1, 2012. To appear in the NN2012 Proceedings in Journal of Physics: Conference Series (JPCS

Observation of the competing fission modes in 178 Pt

Fragment mass distributions from fission of the excited compound nucleus 178 Pt have been deduced from the measured fragment velocities. The 178 Pt nucleus was created at the JAEA tandem facility in a complete fusion reaction 36 Ar + 142 Nd, at beam energies of 155, 170 and 180 MeV. The data are indicative of a mixture of the mass-asymmetric and mass-symmetric fission modes associated with higher and lower total kinetic energies of the fragments, respectively. The measured fragment yields are dominated by asymmetric mass splits, with the symmetric mode contributing at the level of ≈1/3. This constitutes the first observation of a multimodal fission in the sub-lead region. Most probable experimental fragment-mass split of the asymmetric mode, A L /A H ≈79/99, is well reproduced by nuclear density functional theory using the UNEDF1-HFB and D1S potentials. The symmetric mode is associated by theory with very elongated fission fragments, which is consistent with the observed total kinetic energy/fragment mass correlation

Beta-Delayed fission of 230Am

The exotic decay process of β-delayed fission (βDF) has been studied in the neutron-deficient isotope Am230. The Am230 nuclei were produced in the complete fusion reaction Pb207(Al27,4n)Am230 and separated by using the GARIS gas-filled recoil ion separator. A lower limit for the βDF probability PβDF(Am230)>0.30 was deduced, which so far is the highest value among all known βDF nuclei. The systematics of βDF in the region of Am230 will be discussed

First Direct Mass Measurements of Nuclides around Z=100 with a Multireflection Time-of-Flight Mass Spectrograph

The masses of 246Es, 251Fm, and the transfermium nuclei 249−252Md and 254No, produced by hot- and cold-fusion reactions, in the vicinity of the deformed N=152 neutron shell closure, have been directly measured using a multireflection time-of-flight mass spectrograph. The masses of 246Es and 249,250,252Md were measured for the first time. Using the masses of 249,250Md as anchor points for α decay chains, the masses of heavier nuclei, up to 261Bh and 266Mt, were determined. These new masses were compared with theoretical global mass models and demonstrated to be in good agreement with macroscopic-microscopic models in this region. The empirical shell gap parameter δ2n derived from three isotopic masses was updated with the new masses and corroborates the existence of the deformed N=152 neutron shell closure for Md and Lr

R&D status of pulse shape analysis for short-lived decay of superheavy elements in GARIS-II

To search undiscovered superheavy elements, a series of commissioning experiments for the new gas-filled separator GARIS-II at RIKEN was recently carried out. A new data acquisition method was tested to study the short-lived α decay. Both the α decay and evaporation residues were detected by the silicon detectors, and the preamplified waveforms were then directly registered by a flash ADC and analyzed by means of a pulse shape analysis. This paper describes the identification of two sequential pulses (pileup events) from short-lived α decays and the determination of their energy and time difference by the template fitting method. The performance of the present system was evaluated by using a simulated data set and was successfully employed for online experimental data such as 220Ac → 216Fr.