19,401 research outputs found
All-optical generation and detection of sub-picosecond ac spin current pulses in GaAs
Sub-picosecond ac spin current pulses are generated optically in GaAs bulk
and quantum wells at room temperature and 90K through quantum interference
between one-photon and two-photon absorptions driven by two phase-locked
ultrafast laser pulses that are both circularly polarized. The dynamics of the
current pulses are detected optically by monitoring in real time and real space
nanoscale motion of electrons with high-resolution pump-probe techniques.Comment: 5 pages, 5 figure
CW and pulsed electrically detected magnetic resonance spectroscopy at 263 GHz/12 T on operating amorphous silicon solar cells
Here we describe a new high frequency/high field continuous wave and pulsed
electrically detected magnetic resonance (CW EDMR and pEDMR) setup, operating
at 263 GHz and resonance fields between 0 and 12 T. Spin dependent transport in
illuminated hydrogenated amorphous silicon p-i-n solar cells at 5 K and 90 K
was studied by in operando 263 GHz CW and pEDMR alongside with complementary
X-band CW EDMR. Benefiting from the superior resolution at 263 GHz, we were
able to better resolve EDMR signals originating from spin dependent hopping and
recombination processes. 5 K EDMR spectra were found to be dominated by
conduction and valence band tale states involved in spin dependent hopping,
with additional contributions from triplet exciton states. 90 K EDMR spectra
could be assigned to spin pair recombination involving conduction band tail
states and dangling bonds as dominating spin dependent transport process, with
additional contributions from valence band tail and triplet exciton states.Comment: 8 pages, 4 figure
Eigenvalue spectrum for single particle in a spheroidal cavity: A Semiclassical approach
Following the semiclassical formalism of Strutinsky et al., we have obtained
the complete eigenvalue spectrum for a particle enclosed in an infinitely high
spheroidal cavity. Our spheroidal trace formula also reproduces the results of
a spherical billiard in the limit . Inclusion of repetition of each
family of the orbits with reference to the largest one significantly improves
the eigenvalues of sphere and an exact comparison with the quantum mechanical
results is observed upto the second decimal place for . The
contributions of the equatorial, the planar (in the axis of symmetry plane) and
the non-planar(3-Dimensional) orbits are obtained from the same trace formula
by using the appropriate conditions. The resulting eigenvalues compare very
well with the quantum mechanical eigenvalues at normal deformation. It is
interesting that the partial sum of equatorial orbits leads to eigenvalues with
maximum angular momentum projection, while the summing of planar orbits leads
to eigenvalues with except for L=1. The remaining quantum mechanical
eigenvalues are observed to arise from the 3-dimensional(3D) orbits. Very few
spurious eigenvalues arise in these partial sums. This result establishes the
important role of 3D orbits even at normal deformations.Comment: 17 pages, 7 ps figure
Structure of a Complete ATP Synthase Dimer Reveals the Molecular Basis of Inner Mitochondrial Membrane Morphology
We determined the structure of a complete, dimeric F1Fo-ATP synthase from yeast Yarrowia lipolytica mitochondria by a combination of cryo-EM and X-ray crystallography. The final structure resolves 58 of the 60 dimer subunits. Horizontal helices of subunit a in Fo wrap around the c-ring rotor, and a total of six vertical helices assigned to subunits a, b, f, i, and 8 span the membrane. Subunit 8 (A6L in human) is an evolutionary derivative of the bacterial b subunit. On the lumenal membrane surface, subunit f establishes direct contact between the two monomers. Comparison with a cryo-EM map of the F1Fo monomer identifies subunits e and g at the lateral dimer interface. They do not form dimer contacts but enable dimer formation by inducing a strong membrane curvature of ∼100°. Our structure explains the structural basis of cristae formation in mitochondria, a landmark signature of eukaryotic cell morphology
Trapped ion mobility spectrometry and PASEF enable in-depth lipidomics from minimal sample amounts
A comprehensive characterization of the lipidome from limited starting material remains very challenging. Here we report a high-sensitivity lipidomics workflow based on nanoflow liquid chromatography and trapped ion mobility spectrometry (TIMS). Taking advantage of parallel accumulation-serial fragmentation (PASEF), we fragment on average 15 precursors in each of 100 ms TIMS scans, while maintaining the full mobility resolution of co-eluting isomers. The acquisition speed of over 100 Hz allows us to obtain MS/MS spectra of the vast majority of isotope patterns. Analyzing 1 mu L of human plasma, PASEF increases the number of identified lipids more than three times over standard TIMS-MS/MS, achieving attomole sensitivity. Building on high intra- and inter-laboratory precision and accuracy of TIMS collisional cross sections (CCS), we compile 1856 lipid CCS values from plasma, liver and cancer cells. Our study establishes PASEF in lipid analysis and paves the way for sensitive, ion mobility-enhanced lipidomics in four dimensions
Electrical spin injection from an organic-based ferrimagnet in a hybrid organic/inorganic heterostructure
We report the successful extraction of spin polarized current from the
organic-based room temperature ferrimagnetic semiconductor V[TCNE]x (x~2, TCNE:
tetracyanoethylene; TC ~ 400 K, EG ~ 0.5 eV, s ~ 10-2 S/cm) and its subsequent
injection into a GaAs/AlGaAs light-emitting diode (LED). The spin current
tracks the magnetization of V[TCNE]x~2, is weakly temperature dependent, and
exhibits heavy hole / light hole asymmetry. This result has implications for
room temperature spintronics and the use of inorganic materials to probe spin
physics in organic and molecular systems
Local dynamics of topological magnetic defects in the itinerant helimagnet FeGe
Chiral magnetic interactions induce complex spin textures including helical
and conical spin waves, as well as particle-like objects such as magnetic
skyrmions and merons. These spin textures are the basis for innovative device
paradigms and give rise to exotic topological phenomena, thus being of interest
for both applied and fundamental sciences. Present key questions address the
dynamics of the spin system and emergent topological defects. Here we analyze
the micromagnetic dynamics in the helimagnetic phase of FeGe. By combining
magnetic force microscopy, single-spin magnetometry, and
Landau-Lifschitz-Gilbert simulations we show that the nanoscale dynamics are
governed by the depinning and subsequent motion of magnetic edge dislocations.
The motion of these topologically stable objects triggers perturbations that
can propagate over mesoscopic length scales. The observation of stochastic
instabilities in the micromagnetic structure provides new insight to the
spatio-temporal dynamics of itinerant helimagnets and topological defects, and
discloses novel challenges regarding their technological usage
Two-dimensional imaging of the spin-orbit effective magnetic field
We report on spatially resolved measurements of the spin-orbit effective
magnetic field in a GaAs/InGaAs quantum-well. Biased gate electrodes lead to an
electric-field distribution in which the quantum-well electrons move according
to the local orientation and magnitude of the electric field. This motion
induces Rashba and Dresselhaus effective magnetic fields. The projection of the
sum of these fields onto an external magnetic field is monitored locally by
measuring the electron spin-precession frequency using time-resolved Faraday
rotation. A comparison with simulations shows good agreement with the
experimental data.Comment: 6 pages, 4 figure
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