The spin glass-antiferromagnetism competition in Kondo-lattice systems in the presence of a transverse applied magnetic field

A theory is proposed to describe the competition among antiferromagnetism (AF), spin glass (SG) and Kondo effect. The model describes two Kondo sublattices with an intrasite Kondo interaction strength $J_{K}$ and a random Gaussian interlattice interaction in the presence of a transverse field $\Gamma$. The $\Gamma$ field is introduced as a quantum mechanism to produce spin flipping and the random coupling has average $-2J_0/N$ and variance $32 J^{2}/N$. The path integral formalism with Grassmann fields is used to study this fermionic problem, in which the disorder is treated within the framework of the replica trick. The free energy and the order parameters are obtained using the static ansatz. In this many parameters problem, we choose $J_0/J \approx (J_{K}/J)^{2}$ and $\Gamma/J \approx (J_{K}/J)^{2}$ to allow a better comparison with the experimental findings. The obtained phase diagram has not only the same sequence as the experimental one for $Ce_{2}Au_{1-x}Co_{x}Si_{3}$, but mainly, it also shows a qualitative agreement concerning the behavior of the freezing temperature and the Neel temperature which decreases until a Quantum Critical Point (QCP).Comment: 4 pages, 1 figure, accepted for publication in Physica

Spin glass freezing in Kondo lattice compounds

It is presented a theory that describes a spin glass phase at finite temperatures in Kondo lattice systems with an additional RKKY interaction represented by long range, random couplings among localized spins like in the Sherrington- Kirkpatrick (SK) spin glass model. The problem is studied within the functional integral formalism where the spin operators are represented by bilinear combinations of fermionic (anticommuting) Grassmann variables. The Kondo and spin glass transitions are both described with the mean field like static ansatz that reproduces good results in the two well known limits. At high temperatures and low values of the Kondo coupling there is a paramagnetic (disordered) phase with vanishing Kondo and spin glass order parameters. By lowering the temperature a second order transition line is found at Tsg to a spin glass phase. For larger values of the Kondo coupling there is a second order transition line at roughly Tk to a Kondo ordered state. For T<Tsg the transition between the Kondo and spin glass phases becomes first order.Comment: 21 pages, 1 figure, to appear on Phys. Rev.

A van Hemmen-Kondo model for disordered strongly correlated electron systems

We present here a theoretical model in order to describe the competition between the Kondo effect and the spin glass behavior. The spin glass part of the starting Hamiltonian contains Ising spins with an intersite exchange interaction given by the local van Hemmen model, while the Kondo effect is described as usual by the intrasite exchange $J_K$. We obtain, for large $J_K$ values, a Kondo phase and, for smaller $J_K$ values, a succession, with decreasingComment: 14 pages, 4 figures, accepted for publication in Phys. Rev.

Doniach diagram for ordered, disordered and underscreened Kondo lattices

The Doniach's diagram has been originally proposed to describe the competition between the local Kondo effect and the intersite RKKY interactions in cerium compounds. Here we discuss the extension of this diagram to different variations of Kondo lattice model. We consider a) ordered cerium compounds where the competition between magnetic order and Kondo effect plays an important role, as $CeRh_2Si_2$, b) disordered cerium systems with competing spin glass phase, magnetic ordered phases and a Kondo phase, as the heavy fermion cerium alloy $CeCu_xNi_{1-x}$ and, c) uranium compounds where a coexistence between Kondo effect and ferromagnetic order has been observed, as UTe. We show that all these cases can be described by a generalized Doniach phase diagram.Comment: Presented in the Latin American Workshop on Magnetism and Magnetic Materials (LAW3M) Rio de Janeiro, Brazil, August 12-16, 2007. Proceedings to be published in JMM

Spin Glass and antiferromagnetism in Kondo lattice disordered systems

The competition between spin glass (SG), antiferromagnetism (AF) and Kondo effect is studied here in a model which consists of two Kondo sublattices with a gaussian random interaction between spins in differents sublattices with an antiferromagnetic mean Jo and standard deviation J. In the present approach there is no hopping of the conduction electrons between the sublattices and only spins in different sublattices can interact. The problem is formulated in the path integral formalism where the spin operators are expressed as bilinear combinations of Grassmann fields which can be solved at mean field level within the static approximation and the replica symmetry ansatz. The obtained phase diagram shows the sequence of phases SG, AF and Kondo state for increasing Kondo coupling. This sequence agrees qualitatively with experimental data of the Ce_{2} Au_{1-x} Co_{x} Si_{3} compound.Comment: 7 pages, 1 figure, submitted to EPJ

A theoretical study of the cluster glass-Kondo-magnetic disordered alloys

The physics of disordered alloys, such as typically the well known case of CeNi1-xCux alloys, showing an interplay among the Kondo effect, the spin glass state and a magnetic order, has been studied firstly within an average description like in the Sherrington-Kirkpatrick model. Recently, a theoretical model (PRB 74, 014427 (2006)) involving a more local description of the intersite interaction has been proposed to describe the phase diagram of CeNi1-xCux. This alloy is an example of the complex interplay between Kondo effect and frustration in which there is in particular the onset of a cluster-glass state. Although the model given in Ref. PRB 74, 014427 (2006) has reproduced the different phases relatively well, it is not able to describe the cluster-glass state. We study here the competition between the Kondo effect and a cluster glass phase within a Kondo Lattice model with an inter-cluster random Gaussian interaction. The inter-cluster term is treated within the cluster mean-field theory for spin glasses, while, inside the cluster, an exact diagonalisation is performed including inter-site ferromagnetic and intra-site Kondo interactions. The cluster glass order parameters and the Kondo correlation function are obtained for different values of the cluster size, the intra-cluster ferromagnetic coupling and the Kondo intra-site coupling. We obtain, for instance, that the increase of the Kondo coupling tends to destroy the cluster glass phase.Comment: 6 pages, 2 figures, Accepted for publication in Physica

Green nanocomposites as carriers for slow-release of tebuconazole.

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