A microscopic model for solidification

We present a novel picture of a non isothermal solidification process starting from a molecular level, where the microscopic origin of the basic mechanisms and of the instabilities characterizing the approach to equilibrium is rendered more apparent than in existing approaches based on coarse grained free energy functionals \`a la Landau. The system is composed by a lattice of Potts spins, which change their state according to the stochastic dynamics proposed some time ago by Creutz. Such a method is extended to include the presence of latent heat and thermal conduction. Not only the model agrees with previous continuum treatments, but it allows to introduce in a consistent fashion the microscopic stochastic fluctuations. These play an important role in nucleating the growing solid phase in the melt. The approach is also very satisfactory from the quantitative point of view since the relevant growth regimes are fully characterized in terms of scaling exponents.Comment: 7 pages Latex +3 figures.p

Evidence of a pressure-induced metallization process in monoclinic VO2_2

Raman and combined trasmission and reflectivity mid infrared measurements have been carried out on monoclinic VO$_2$ at room temperature over the 0-19 GPa and 0-14 GPa pressure ranges, respectively. The pressure dependence obtained for both lattice dynamics and optical gap shows a remarkable stability of the system up to P*$\sim$10 GPa. Evidence of subtle modifications of V ion arrangements within the monoclinic lattice together with the onset of a metallization process via band gap filling are observed for P$>$P*. Differently from ambient pressure, where the VO$_2$ metal phase is found only in conjunction with the rutile structure above 340 K, a new room temperature metallic phase coupled to a monoclinic structure appears accessible in the high pressure regime, thus opening to new important queries on the physics of VO$_2$.Comment: 5 pages, 3 figure

Anisotropic excitonic effects in the energy loss function of hexagonal boron nitride

We demonstrate that the valence energy-loss function of hexagonal boron nitride (hBN) displays a strong anisotropy in shape, excitation energy and dispersion for momentum transfer q parallel or perpendicular to the hBN layers. This is manifested by e.g. an energy shift of 0.7 eV that cannot be captured by single-particle approaches and is a demonstration of a strong anisotropy in the two-body electron-hole interaction. Furthermore, for in-plane directions of q we observe a splitting of the -plasmon in the M direction that is absent in the K direction and this can be traced back to band-structure effects.Comment: 10 pages, 4 figure

Anomalous Aharonov--Bohm gap oscillations in carbon nanotubes

The gap oscillations caused by a magnetic flux penetrating a carbon nanotube represent one of the most spectacular observation of the Aharonov-Bohm effect at the nano--scale. Our understanding of this effect is, however, based on the assumption that the electrons are strictly confined on the tube surface, on trajectories that are not modified by curvature effects. Using an ab-initio approach based on Density Functional Theory we show that this assumption fails at the nano-scale inducing important corrections to the physics of the Aharonov-Bohm effect. Curvature effects and electronic density spilled out of the nanotube surface are shown to break the periodicity of the gap oscillations. We predict the key phenomenological features of this anomalous Aharonov-Bohm effect in semi-conductive and metallic tubes and the existence of a large metallic phase in the low flux regime of Multi-walled nanotubes, also suggesting possible experiments to validate our results.Comment: 7 figure

Fluctuation-Induced Casimir Forces in Granular Fluids

We have numerically investigated the behavior of driven non-cohesive granular media and found that two fixed large intruder particles, immersed in a sea of small particles, experience, in addition to a short range depletion force, a long range repulsive force. The observed long range interaction is fluctuation-induced and we propose a mechanism similar to the Casimir effect that generates it: the hydrodynamic fluctuations are geometrically confined between the intruders, producing an unbalanced renormalized pressure. An estimation based on computing the possible Fourier modes explains the repulsive force and is in qualitative agreement with the simulations.Comment: 4 pages, 3 figures. Accepted in Phys. Rev. Letter

Sequential fissions of heavy nuclear systems

In Xe+Sn central collisions from 12 to 20 MeV/A measured with the INDRA 4$\pi$ multidetector, the three-fragment exit channel occurs with a significant cross section. In this contribution, we show that these fragments arise from two successive binary splittings of a heavy composite system. Strong Coulomb proximity effects are observed in the three-fragment final state. By comparison with Coulomb trajectory calculations, we show that the time scale between the consecutive break-ups decreases with increasing bombarding energy, becoming compatible with quasi-simultaneous multifragmentation above 18 MeV/A.Comment: 6 pages, 5 figures, contribution to conference proceedings of the Fifth International Workshop on Nuclear fission and Fission-Product Spectroscop

Pharmacokinetic and clinical considerations for monitoring asparaginase activity levels during pegaspargase therapy

Peer Reviewedhttp://deepblue.lib.umich.edu/bitstream/2027.42/111166/1/pbc25426.pd

Experimental determination of the quasi-projectile mass with measured neutrons

The investigation of the isospin dependence of multifragmentation reactions relies on precise reconstruction of the fragmenting source. The criteria used to assign free emitted neutrons, detected with the TAMU Neutron Ball, to the quasi-projectile source are investigated in the framework of two different simulation codes. Overall and source-specific detection efficiencies for multifragmentation events are found to be model independent. The equivalence of the two different methods used to assign experimentally detected charged particles and neutrons to the emitting source is shown. The method used experimentally to determine quasi-projectile emitted free neutron multiplicity is found to be reasonably accurate and sufficiently precise as to allow for the study of well-defined quasi-projectile sources.Comment: 10 pages, 8 figures. To be submitted to Nucl. Instr. and Meth.