1,106 research outputs found
Lifetimes of antiferromagnetic magnons in two and three dimensions: experiment, theory, and numerics
A high-resolution neutron spectroscopic technique is used to measure
momentum-resolved magnon lifetimes in the prototypical two- and
three-dimensional antiferromagnets Rb2MnF4 and MnF2, over the full Brillouin
zone and a wide range of temperatures. We rederived theories of the lifetime
resulting from magnon-magnon scattering, thereby broadening their applicability
beyond asymptotically small regions of wavevector and temperature.
Corresponding computations, combined with a small contribution reflecting
collisions with domain boundaries, yield excellent quantitative agreement with
the data.Comment: 5 pages, 4 figure
Electronic structure, magnetic and dielectric properties of the edge-sharing copper-oxide chain compound NaCuO
We report an experimental study of \nco, a Mott insulator containing chains
of edge-sharing CuO plaquettes, by polarized x-ray absorption spectroscopy
(XAS), resonant magnetic x-ray scattering (RMXS), magnetic susceptibility, and
pyroelectric current measurements. The XAS data show that the valence holes
reside exclusively on the Cu sites within the copper-oxide spin chains
and populate a -orbital polarized within the CuO plaquettes. The RMXS
measurements confirm the presence of incommensurate magnetic order below a
N\'eel temperature of K, which was previously inferred from
neutron powder diffraction and nuclear magnetic resonance data. In conjunction
with the magnetic susceptibility and XAS data, they also demonstrate a new
"orbital" selection rule for RMXS that is of general relevance for magnetic
structure determinations by this technique. Dielectric property measurements
reveal the absence of significant ferroelectric polarization below , which
is in striking contrast to corresponding observations on the isostructural
compound \lco. The results are discussed in the context of current theories of
multiferroicity.Comment: 7 pages, 7 figure
Hard x-ray spectroscopy in NaxCoO2 and superconducting NaxCoO2 - yH2O: A view on the bulk Co electronic properties
The electronic properties of Co in bulk Na0.7CoO2 and the superconducting
hydrated compound Na0.35CoO2 - y H2O have been investigated by x-ray absorption
spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS) using hard
x-rays. The XAS spectra at the Co K-edge were measured in both compounds with
two different polarization directions. The changes in the XAS spectra upon
hydration and their polarization dependence are well accounted for by linear
muffin- tin orbital calculations in the local density approximation. The
underlying electronic structure indicates the strong hybridization between the
Co 3d and O 2p states in both compounds, while the electron localization is
enhanced in the hydrated compound due to the increase of the Co-Co interplanar
distance. The Co K pre-edge further highlights the splitting of the d band as a
result of the crystal field effect and demonstrates the Co valency increase
when Na0.7CoO2 is hydrated. The RIXS spectra measured at the Co K-edge show an
energy loss feature around 10 eV in both compounds in fair agreement with the
calculated dynamical structure factor. The RIXS feature is associated to a
damped plasmon excitation.Comment: 8 page
Teaching powerful geographical knowledge : a matter of social justice : initial findings from the GeoCapabilities 3 project
GeoCapabilities offers an approach for unlocking powerful disciplinary knowledge (PDK) for children. In phase three of the project, we are exploring how far GeoCapabilities ‘works’ for teachers serving communities in challenging socio-economic circumstances. We connect GeoCapabilities to social justice in education, theoretically. Then, using the topic of migration, we discuss initial empirical findings of how teachers understand PDK and their challenges for teaching PDK. Collaborative work between teachers and academics suggests that the social justice dimension of GeoCapabilities could be realised, with appropriate support for teachers. We conclude with a set of principles to inform the future work of GeoCapabilities
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Scalable High Performance Message Passing over InfiniBand for Open MPI
InfiniBand (IB) is a popular network technology for modern high-performance computing systems. MPI implementations traditionally support IB using a reliable, connection-oriented (RC) transport. However, per-process resource usage that grows linearly with the number of processes, makes this approach prohibitive for large-scale systems. IB provides an alternative in the form of a connectionless unreliable datagram transport (UD), which allows for near-constant resource usage and initialization overhead as the process count increases. This paper describes a UD-based implementation for IB in Open MPI as a scalable alternative to existing RC-based schemes. We use the software reliability capabilities of Open MPI to provide the guaranteed delivery semantics required by MPI. Results show that UD not only requires fewer resources at scale, but also allows for shorter MPI startup times. A connectionless model also improves performance for applications that tend to send small messages to many different processes
Football and dementia: A qualitative investigation of a community based sports group for men with early onset dementia
This study investigates the impact of a weekly group providing sport and physical activities for men with early onset dementia established by Notts County Football in the Community (NCFC). There were three aims: investigate the effect of early onset dementia on individuals with the condition and their carers; examine perceptions of current levels of service provision for people with early onset dementia; and analyse the impact of the group. Men with dementia (n=5) attending the sessions, their carers (n=5), NCFC coaching staff (n=5) and people organising/facilitating the sessions (n=5), were interviewed. Semi-structured interviews explored the participants’ experiences of dementia, their opinions on current service provisions and on the sessions. Data were analysed using thematic analysis. Four main themes were found: loss related to the condition of dementia and its impact on relationships (‘Loss’); lack of age-appropriate services for people with early onset dementia (‘Lack of Resources’); enjoyment and positive anticipation related to the group for all involved (‘Enjoyment and Anticipation’); and ‘the Notts County Effect’ which attributed the success of the sessions to the strong brand of the football club, and to personalised service in a “dementia-free” environment. The NCFC sessions provided a safe low-cost intervention with positive effects upon quality of life for both people with early onset dementia, their carers and the staff involved. This suggests that the service may be valuable to a wider range of people living in different area
Exploitative Strategies: Consequences for Individual Behavior, Social Structure, and Design of Institutions
Entanglement Measures for Single- and Multi-Reference Correlation Effects
Electron correlation effects are essential for an accurate ab initio
description of molecules. A quantitative a priori knowledge of the single- or
multi-reference nature of electronic structures as well as of the dominant
contributions to the correlation energy can facilitate the decision regarding
the optimum quantum chemical method of choice. We propose concepts from quantum
information theory as orbital entanglement measures that allow us to evaluate
the single- and multi-reference character of any molecular structure in a given
orbital basis set. By studying these measures we can detect possible artifacts
of small active spaces.Comment: 14 pages, 4 figure
Ground state properties of heavy alkali halides
We extend previous work on alkali halides by calculations for the heavy-atom
species RbF, RbCl, LiBr, NaBr, KBr, RbBr, LiI, NaI, KI, and RbI. Relativistic
effects are included by means of energy-consistent pseudopotentials,
correlations are treated at the coupled-cluster level. A striking deficiency of
the Hartree-Fock approach are lattice constants deviating by up to 7.5 % from
experimental values which is reduced to a maximum error of 2.4 % by taking into
account electron correlation. Besides, we provide ab-initio data for in-crystal
polarizabilities and van der Waals coefficients.Comment: accepted by Phys. Rev.
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