A structural evaluation of the tungsten isotopes via thermal neutron capture

Total radiative thermal neutron-capture $\gamma$-ray cross sections for the $^{182,183,184,186}$W isotopes were measured using guided neutron beams from the Budapest Research Reactor to induce prompt and delayed $\gamma$ rays from elemental and isotopically-enriched tungsten targets. These cross sections were determined from the sum of measured $\gamma$-ray cross sections feeding the ground state from low-lying levels below a cutoff energy, E$_{\rm crit}$, where the level scheme is completely known, and continuum $\gamma$ rays from levels above E$_{\rm crit}$, calculated using the Monte Carlo statistical-decay code DICEBOX. The new cross sections determined in this work for the tungsten nuclides are: $\sigma_{0}(^{182}{\rm W}) = 20.5(14)$ b and $\sigma_{11/2^{+}}(^{183}{\rm W}^{m}, 5.2 {\rm s}) = 0.177(18)$ b; $\sigma_{0}(^{183}{\rm W}) = 9.37(38)$ b and $\sigma_{5^{-}}(^{184}{\rm W}^{m}, 8.33 \mu{\rm s}) = 0.0247(55)$ b; $\sigma_{0}(^{184}{\rm W}) = 1.43(10)$ b and $\sigma_{11/2^{+}}(^{185}{\rm W}^{m}, 1.67 {\rm min}) = 0.0062(16)$ b; and, $\sigma_{0}(^{186}{\rm W}) = 33.33(62)$ b and $\sigma_{9/2^{+}}(^{187}{\rm W}^{m}, 1.38 \mu{\rm s}) = 0.400(16)$ b. These results are consistent with earlier measurements in the literature. The $^{186}$W cross section was also independently confirmed from an activation measurement, following the decay of $^{187}$W, yielding values for $\sigma_{0}(^{186}{\rm W})$ that are consistent with our prompt $\gamma$-ray measurement. The cross-section measurements were found to be insensitive to choice of level density or photon strength model, and only weakly dependent on E$_{\rm crit}$. Total radiative-capture widths calculated with DICEBOX showed much greater model dependence, however, the recommended values could be reproduced with selected model choices. The decay schemes for all tungsten isotopes were improved in these analyses.Comment: 25 pages, 15 figures, 15 table

Measurement of cross sections for alpha-induced reactions on 197Au and thick-target yields for the ((alpha),(gamma)) process on 64Zn and 63Cu

We have measured the cross sections for the {sup 197}Au({alpha},{gamma}){sup 201}Tl and {sup 197}Au({alpha},2n){sup 199}Tl reactions in the 17.9- to 23.9-MeV energy range, and {sup 197}Au({alpha},n){sup 200}Tl reaction in the 13.4- to 23.9-MeV energy range using an activation technique. Thick-target yields for the {sup 64}Zn({alpha},{gamma}){sup 68}Ge (7- to 14-MeV) and {sup 63}Cu({alpha},{gamma}){sup 67}Ga (7-MeV) reactions were measured. For all measurements, natural elements were bombarded with He{sup +} beams from the 88'' Cyclotron at the Lawrence Berkeley National Laboratory (LBNL). Irradiated samples were counted using a g-spectrometry system at LBNL's Low Background Facility. Measured {sup 197}Au({alpha},{gamma}){sup 201}Tl cross-sections were compared with the NON-SMOKER theoretical values. The thick-target yields for the {sup 64}Zn({alpha},{gamma}){sup 68}Ge and {sup 63}Cu({alpha},{gamma}){sup 67}Ga reactions are also compared with the theoretical yield, calculated numerically using the energy dependent NON-SMOKER cross section data. In both cases, measured values are found to follow a trend of overlapping the predicted value near the alpha nucleus barrier height and fall below with a slowly widening difference between them in the sub barrier energy points

Properties of the 5- state at 839 keV in 176Lu and the s-process branching at A = 176

The s-process branching at mass number A = 176 depends on the coupling between the high-K ground state and a low-lying low-K isomer in 176Lu. This coupling is based on electromagnetic transitions via intermediate states at higher energies. The properties of the lowest experimentally confirmed intermediate state at 839 keV are reviewed, and the transition rate between low-K and high-K states under stellar conditions is calculated on the basis of new experimental data for the 839 keV state. Properties of further candidates for intermediate states are briefly analyzed. It is found that the coupling between the high-K ground state and the low-K isomer in 176Lu is at least one order of magnitude stronger than previously assumed leading to crucial consequences for the interpretation of the 176Lu/176Hf pair as an s-process thermometer.Comment: 11 pages, 4 figures accepted for publication in Phys. Rev.

Excitation functions and isomeric cross-section ratios of (d,xn) reactions on 86Sr

Excitation functions of the 86Sr(d,n)87m,87gY, 86Sr(d,2n)86m,86gY and 86Sr(d,3n)85m,85gY reactions on enriched 86Sr target were measured by the activation technique up to deuteron energies of 49 MeV. The isomeric cross-section ratios as a function of projectile energy were deduced from the measured data for 87mY, 87gY(cum), 86mY, 86gY(cum), 85mY and 85gY pairs for the same energy range. All measurements are reported for the first time. The experimental data were compared with the data from the TENDL library which is based on TALYS calculation with default parameters. No satisfactory agreement was observed. Nuclear model calculations were then performed using the codes TALYS and EMPIRE with some parameter adjustments, and compared with the experimental data. The quality of the agreement between experimental data and model calculations was numerically quantified. In general, the data as well as the isomeric cross-section ratios are partially reproduced by the model calculations, provided the input model parameters are properly chosen and the level structure of the product nucleus is thoughtfully considered

To the Continuum and Beyond: Structure of U Nuclei

An experiment was performed at the 88-inch cyclotron at LBNL to investigate the structure of uranium isotopes and concurrently test the so-called surrogate ratio method. A 28 MeV proton beam was used to bombard 236U and 238U targets and the outgoing light ions were detected using the STARS silicon telescope allowing isotopic assignments and the excitation energy of the compound nucleus to be measured. A fission detector was placed at backward angles to give particle-fission coincidences, while the six clover germanium detectors of the LIBERACE array were used for particle-γ coincidences. The (p,d) reaction channels on 236U and 238U targets were used as a surrogate to measure the σ(234U(n,f))/σ(236U(n,f)) cross section ratio. The results give reasonable agreement with literature values over an equivalent neutron energy range between 0 MeV and 6 MeV. Structure results in 235U include a new (3/2−) level at 1035 keV, that is tentatively assigned as the 3/2−[501] Nilsson state. The analogue 3/2−[501] state in 237U may be associated with a previously observed level at 1201 keV, whose spin/parity is restricted to Jπ = 3/2− on the basis of newly observed decays to the ground band

Utilizing (\u3cem\u3ep,d\u3c/em\u3e) and (\u3cem\u3ep,t\u3c/em\u3e) Reactions to Obtain (\u3cem\u3en,f\u3c/em\u3e) Cross Sections in Uranium Nuclei Via the Surrogate-Ratio Method

The surrogate ratio method has been tested for (p,d) and (p,t) reactions on uranium nuclei. 236U and 238U targets were bombarded with 28-MeV protons and the light ion recoils and fission fragments were detected using the Silicon Telescope Array for Reaction Studies detector array at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory. The (p,df) reaction channels on 236U and 238U targets were used as a surrogate to determine the σ[236U(n,f)]/σ[234U(n,f)] cross-section ratio. The (p,tf) reaction channels were also measured with the same targets as a surrogate for the σ[235U(n,f)]/σ[(233U(n,f)] ratio. For the (p,df) and (p,tf) surrogate measurements, there is good agreement with accepted (n,f) values over equivalent neutron energy ranges of En=0–7 MeV and En=0–5.5 MeV, respectively. An internal surrogate ratio method comparing the (p,d) and (p,t) reaction channels on a single target is also discussed. The σ[234U(n,f)]/σ[233U(n,f)] and σ[236U(n,f)]/σ[235U(n,f)] cross-section ratios are extracted using this method for the 236U and 238U targets, respectively. The resulting fission cross-section ratios show relatively good agreement with accepted values up to En∼5 MeV

Statistical \u3cem\u3eγ\u3c/em\u3e Rays in the Analysis of Surrogate Nuclear Reactions

The surrogate nuclear reaction method is being applied in many efforts to indirectly determine neutron-induced reaction cross sections on short-lived isotopes. This technique aims to extract accurate (n,γ) cross sections from measured decay properties of the compound nucleus of interest (created using a different reaction). The advantages and limitations of a method that identifies the γ-ray decay channel by detecting any high-energy (“statistical”) γ ray emitted during the relaxation of the compound nucleus were investigated. Data collected using the Silicon Telescope Array for Reaction Studies and Livermore-Berkeley Array for Collaborative Experiments silicon and germanium detector arrays were used to study the decay of excited gadolinium nuclei following inelastic proton scattering. In many cases, this method of identifying the γ-ray decay channel can simplify the experimental data collection and greatly improve the detection efficiency for γ-ray cascades. The results show sensitivity to angular-momentum differences between the surrogate reaction and the desired (n,γ) reaction similar to an analysis performed using low-lying discrete transitions even when ratios of cross sections are considered

Remnants of Spherical Shell Structures in Deformed Nuclei: The Impact of an \u3cem\u3eN\u3c/em\u3e = 64 Neutron Subshell Closure on the Structure of \u3cem\u3eN\u3c/em\u3e ≈ 90 Gadolinium Nuclei

Odd-mass gadolinium isotopes around N = 90 were populated by the (p,d) reaction, utilizing 25-MeV protons, resulting in population of low-spin quasineutron states at energies near and below the Fermi surface. Systematics of the single quasineutron levels populated are presented. A large excitation energy gap is observed between levels originating from the 2d3/2, 1h11/2, and 3s1/2 spherical parents (above the N = 64 gap), and the 2d5/2 (below the gap), indicating that the spherical shell model level spacing is maintained at least to moderate deformations