1,705 research outputs found
Superconductivity in a Molecular Metal Cluster Compound
Compelling evidence for band-type conductivity and even bulk
superconductivity below K has been found in
Ga-NMR experiments in crystalline ordered, giant Ga
cluster-compounds. This material appears to represent the first realization of
a theoretical model proposed by Friedel in 1992 for superconductivity in
ordered arrays of weakly coupled, identical metal nanoparticles.Comment: 5 pages, 4 figure
Magnetic Properties of a Quantum Ferrimagnet: NiCu(pba)(D_2O)_3 . 2D_2O
We report the results of magnetic measurements on a powder sample of
NiCu(pba)(D_2O)_3 \cdot 2D_2OS\chi\chi TT\chi TJ/k_B=121
K^{2+}^{2+}g_{Ni}g_{Cu}\chi T$ at low temperatures
is reproduced fairly well by the calculation for the same ferrimagnetic model.Comment: 7pages, 4 postscript figures, usues REVTEX. appear in J. Phys. Soc.
Jpn vol 67 No.7 (1998
Perceived changes in quality of life in trauma patients:A focus group study
Quality of life (QoL) following a physical trauma is still insufficiently known from a patient perspective. The aim of this study was to qualitatively report perceived changes in QoL after trauma. Focus groups were conducted. Patients admitted to the hospital were eligible for inclusion if they had a lower extremity trauma, severe injuries, or severe traumatic brain injury (TBI). Patients 75 years or older were invited. To analyze the perceived changes in QoL, open coding was used. Patients ( n = 20, M = 55 years) reported comparable consequences. In the first month posttrauma, physical limitations, independency, pain, and anxiety predominated. Later, patients experienced problems with acceptance. The patients’ feelings of the need to have control over their own situation, their own expectations, and a social network were related to QoL. Compared with the other patient groups, TBI patients reported more psychosocial consequences, and elderly patients reported more difficulties in performing (social) activities. Quality of health care was considered an important aspect in the patients’ perceived QoL, and adequate aftercare was missed according to the patients. The impact of a trauma influences QoL in different health domains. Further improving the quality of aftercare may positively influence trauma patients’ perceived QoL. These results indicated that TBI patients and elderly patients deserve specific attention regarding QoL
Spin Stiffness in the Hubbard model
The spin stiffness of the repulsive Hubbard model that occurs
in the hydrodynamic theory of antiferromagnetic spin waves is shown to be the
same as the thermodynamically defined stiffness involved in twisting the order
parameter. New expressions for are derived, which enable easier
interpretation, and connections with superconducting weight and gauge
invariance are discussed.Comment: 21 Pages LaTeX2e, to be published in Journal of Physics
Magnetic long-range order induced by quantum relaxation in single-molecule magnets
Can magnetic interactions between single-molecule magnets (SMMs) in a crystal
establish long-range magnetic order at low temperatures deep in the quantum
regime, where the only electron spin-fluctuations are due to incoherent
magnetic quantum tunneling (MQT)? Put inversely: can MQT provide the
temperature dependent fluctuations needed to destroy the ordered state above
some finite Tc, although it should basically itself be a T-independent process?
Our experiments on two novel Mn4 SMMs provide a positive answer to the above,
showing at the same time that MQT in the SMMs has to involve spin-lattice
coupling at a relaxation rate equaling that predicted and observed recently for
nuclear spin-mediated quantum relaxation.Comment: 4 pages, 3 figure
UvA-DARE (Digital Academic Repository) Self-perceived halitosis influences social interactions
UvA-DARE (Digital Academic Repository) Usefulness of a trauma-focused treatment approach for travel phobia
Giant isotope effect in the incoherent tunneling specific heat of the molecular nanomagnet Fe8
Time-dependent specific heat experiments on the molecular nanomagnet Fe8 and
the isotopic enriched analogue 57Fe8 are presented. The inclusion of the 57Fe
nuclear spins leads to a huge enhancement of the specific heat below 1 K,
ascribed to a strong increase in the spin-lattice relaxation rate Gamma arising
from incoherent, nuclear-spin-mediated magnetic quantum tunneling in the
ground-doublet. Since Gamma is found comparable to the expected tunneling rate,
the latter process has to be inelastic. A model for the coupling of the
tunneling levels to the lattice is presented. Under transverse field, a
crossover from nuclear-spin-mediated to phonon-induced tunneling is observed.Comment: Replaced with version accepted for publication in Physical Review
Letter
Dynamics and thermalization of the nuclear spin bath in the single-molecule magnet Mn12-ac: test for the theory of spin tunneling
The description of the tunneling of a macroscopic variable in the presence of
a bath of localized spins is a subject of great fundamental and practical
interest, and is relevant for many solid-state qubit designs. Instead of
focusing on the the "central spin" (as is most often done), here we present a
detailed study of the dynamics of the nuclear spin bath in the Mn12-ac
single-molecule magnet, probed by NMR experiments down to very low temperatures
(T = 20 mK). We find that the longitudinal relaxation rate of the 55Mn nuclei
in Mn12-ac becomes roughly T-independent below T = 0.8 K, and can be strongly
suppressed with a longitudinal magnetic field. This is consistent with the
nuclear relaxation being caused by quantum tunneling of the molecular spin, and
we attribute the tunneling fluctuations to the minority of fast-relaxing
molecules present in the sample. The transverse nuclear relaxation is also
T-independent for T < 0.8 K, and can be explained qualitatively and
quantitatively by the dipolar coupling between like nuclei in neighboring
molecules. We also show that the isotopic substitution of 1H by 2H leads to a
slower nuclear longitudinal relaxation, consistent with the decreased tunneling
probability of the molecular spin. Finally, we demonstrate that, even at the
lowest temperatures, the nuclear spins remain in thermal equilibrium with the
lattice phonons, and we investigate the timescale for their thermal
equilibration. After a review of the theory of macroscopic spin tunneling in
the presence of a spin bath, we argue that most of our experimental results are
consistent with that theory, but the thermalization of the nuclear spins is
not.Comment: 24 pages, 18 figures. Experimental study of the spin bath dynamics in
quantum nanomagnets, plus an extensive review and application of the theor
Heat Capacity and Magnetic Phase Diagram of the Low-Dimensional Antiferromagnet YBaCuO
A study by specific heat of a polycrystalline sample of the low-dimensional
magnetic system YBaCuO is presented. Magnetic fields up to 14 T are
applied and permit to extract the (,) phase diagram. Below
T, the N\'eel temperature, associated with a
three-dimensional antiferromagnetic long-range ordering, is constant and equals
K. Above , increases linearly with and a
field-induced increase of the entropy at is related to the presence of an
isosbestic point at K, where all the specific heat curves cross.
A comparison is made between YBaCuO and the quasi-two-dimensional
magnetic systems BaNiVO, SrCuOCl, and
PrCuO, for which very similar phase diagrams have been reported. An
effective field-induced magnetic anisotropy is proposed to explain these phase
diagrams.Comment: 14 pages, 7 figure
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