62,732 research outputs found

    Enhanced secondary organic aerosol formation due to water uptake by fine particles

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    This study characterizes the partitioning behavior of a significant fraction of the ambient organic aerosol through simultaneous measurements of gas and particle watersoluble organic carbon (WSOC). During the summer in Atlanta, WSOC gas/particle partitioning showed a strong RH dependence that was attributed to particulate liquid water. At elevated RH levels (\u3e70%) a significant increase in WSOC partitioning to the particle phase was observed and followed the predicted water uptake by fine particles. The enhancement in particle-phase partitioning translated to increased median particle WSOC concentrations ranging from 0.3 –0.9 mgCm3 . The results provide a detailed overview of the WSOC partitioning behavior in the summertime in an urban region dominated by biogenic emissions, and indicate that secondary organic aerosol formation involving partitioning to liquid water may be a significant aerosol formation route that is generally not considered. Citation: Hennigan, C. J., M. H. Bergin, J. E. Dibb, and R. J. Weber (2008), Enhanced secondary organic aerosol formation due to water uptake by fine particles, Geophys. Res. Lett., 35, L18801, doi:10.1029/2008GL035046

    Disorder effects on the superconducting properties of BaFe1.8_{1.8}Co0.2_{0.2}As2_2 single crystals

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    Single crystals of superconducting BaFe1.8_{1.8}Co0.2_{0.2}As2_2 were exposed to neutron irradiation in a fission reactor. The introduced defects decrease the superconducting transition temperature (by about 0.3 K) and the upper critical field anisotropy (e.g. from 2.8 to 2.5 at 22 K) and enhance the critical current densities by a factor of up to about 3. These changes are discussed in the context of similar experiments on other superconducting materials

    Coarse Grained Liouville Dynamics of piecewise linear discontinuous maps

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    We compute the spectrum of the classical and quantum mechanical coarse-grained propagators for a piecewise linear discontinuous map. We analyze the quantum - classical correspondence and the evolution of the spectrum with increasing resolution. Our results are compared to the ones obtained for a mixed system.Comment: 11 pages, 8 figure

    1/f noise of Josephson-junction-embedded microwave resonators at single photon energies and millikelvin temperatures

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    We present measurements of 1/f frequency noise in both linear and Josephson-junction-embedded superconducting aluminum resonators in the low power, low temperature regime - typical operating conditions for superconducting qubits. The addition of the Josephson junction does not result in additional frequency noise, thereby placing an upper limit for fractional critical current fluctuations of 10−810^{-8} (Hz−1/2^{-1/2}) at 1 Hz for sub-micron, shadow evaporated junctions. These values imply a minimum dephasing time for a superconducting qubit due to critical current noise of 40 -- 1400 μ\mus depending on qubit architecture. Occasionally, at temperatures above 50 mK, we observe the activation of individual fluctuators which increase the level of noise significantly and exhibit Lorentzian spectra

    Proton Structure Functions from Chiral Dynamics and QCD Constraints

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    The spin fractions and deep inelastic structure functions of the proton are analyzed using chiral field theory involving Goldstone bosons. A detailed comparison with recent chiral models sheds light on their successful description of the spin fractions of the proton as being due to neglecting helicity non-flip chiral transitions. This approximation is valid for zero mass quarks but not for constituent quarks. Since the chiral spin fraction models with the pure spin-flip approximation reproduce the measured spin fractions of the proton, axialvector constituent-quark-Goldstone boson coupling is found to be inconsistent with the proton spin data. Initial quark valence distributions are then constructed using quark counting constraints at Bjorken x→1x \to 1 and Regge behavior at x→0x \to 0. Sea quark distributions predicted by chiral field theory on this basis have correct order of magnitude and shape. The spin fractions agree with the data.Comment: 30 pages, 2 tables, 10 figure-ps files, LaTex. Accepted by Int. J. Mod. Phys. A. More details added on polarized chiral splitting function

    Charge dynamics in the half-metallic ferromagnet CrO\u3csub\u3e2\u3c/sub\u3e

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    Infrared spectroscopy is used to investigate the electronic structure and charge carrier relaxation in crystalline films of CrO2 which is the simplest of all half-metallic ferromagnets. Chromium dioxide is a bad metal at room temperature but it has a remarkably low residual resistivity (\u3c5 \u3eμΩ cm) despite the small spectral weight associated with free carrier absorption. The infrared measurements show that low residual resistivity is due to the collapse of the scattering rate at ω\u3c2000 \u3ecm-1. The blocking of the relaxation channels at low v and T can be attributed to the unique electronic structure of a half-metallic ferromagnet. In contrast to other ferromagnetic oxides, the intraband spectral weight is constant below the Curie temperature
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