15,231 research outputs found

    Spectroscopy of PTCDA attached to rare gas samples: clusters vs. bulk matrices. I. Absorption spectroscopy

    Get PDF
    The interaction between PTCDA (3,4,9,10-perylene-tetracarboxylic-dianhydride) and rare gas or para-hydrogen samples is studied by means of laser-induced fluorescence excitation spectroscopy. The comparison between spectra of PTCDA embedded in a neon matrix and spectra attached to large neon clusters shows that these large organic molecules reside on the surface of the clusters when doped by the pick-up technique. PTCDA molecules can adopt different conformations when attached to argon, neon and para-hydrogen clusters which implies that the surface of such clusters has a well-defined structure and has not liquid or fluxional properties. Moreover, a precise analysis of the doping process of these clusters reveals that the mobility of large molecules on the cluster surface is quenched, preventing agglomeration and complex formation

    Electronic properties of disordered corner-sharing tetrahedral lattices

    Full text link
    We have examined the behaviour of noninteracting electrons moving on a corner-sharing tetrahedral lattice into which we introduce a uniform (box) distribution, of width W, of random on-site energies. We have used both the relative localization length and the spectral rigidity to analyze the nature of the eigenstates, and have determined both the mobility edge trajectories as a function of W, and the critical disorder, Wc, beyond which all states are localized. We find (i) that the mobility edge trajectories (energies Ec vs. disorder W) are qualitatively different from those found for a simple cubic lattice, and (ii) that the spectral rigidity is scale invariant at Wc and thus provides a reliable method of estimating this quantity -- we find Wc/t=14.5. We discuss our results in the context of the metal-to-insulator transition undergone by LiAlyTi{2-y}O4 in a quantum site percolation model that also includes the above-mentioned Anderson disorder, and show that the effects produced by Anderson disorder are far less important than those produced by quantum site percolation, at least in the determination of the doping concentration at which the metal-to-insulator transition is predicted to occur

    New method for reducing the contribution of the beam position in the quadrupole signal

    Get PDF

    Quantum rainbow scattering at tunable velocities

    Full text link
    Elastic scattering cross sections are measured for lithium atoms colliding with rare gas atoms and SF6 molecules at tunable relative velocities down to ~50 m/s. Our scattering apparatus combines a velocity-tunable molecular beam with a magneto-optic trap that provides an ultracold cloud of lithium atoms as a scattering target. Comparison with theory reveals the quantum nature of the collision dynamics in the studied regime, including both rainbows as well as orbiting resonances

    Spin Diffusion in Classical Heisenberg Magnets with Uniform, Alternating, and Random Exchange

    Get PDF
    We have carried out an extensive simulation study for the spin autocorrelation function at T=∞ of the one‐dimensional classical Heisenberg model with four different types of isotropic bilinear nearest‐neighbor coupling: uniform exchange, alternating exchange, and two kinds of random exchange. For the long‐time tails of all but one case, the simulation data seem incompatible with the simple ∼t −1/2 leading term predicted by spin diffusion phenomenology

    UD Information Services Announces Appointment and Promotion

    Get PDF
    News release announces that Patricia Rooney has been promoted to Assignment Editor and Pamela Blumsheid has been appointed Public Affairs Coordinator

    Experimental and computational analyses reveal that environmental restrictions shape HIV-1 spread in 3D cultures

    No full text
    Here, using an integrative experimental and computational approach, Imle et al. show how cell motility and density affect HIV cell-associated transmission in a three-dimensional tissue-like culture system of CD4+ T cells and collagen, and how different collagen matrices restrict infection by cell-free virions

    Hanle effect in coherent backscattering

    Get PDF
    We study the shape of the coherent backscattering (CBS) cone obtained when resonant light illuminates a thick cloud of laser-cooled rubidium atoms in presence of a homogenous magnetic field. We observe new magnetic field-dependent anisotropies in the CBS signal. We show that the observed behavior is due to the modification of the atomic radiation pattern by the magnetic field (Hanle effect in the excited state).Comment: 4 pages, 3 figure
    corecore