249 research outputs found
Extensive reduction of surface UV radiation since 1750 in world's populated regions
Human activity influences a wide range of components that affect the surface UV radiation levels, among them ozone at high latitudes. We calculate the effect of human-induced changes in the surface erythemally weighted ultra-violet radiation (UV-E) since 1750. We compare results from a radiative transfer model to surface UV-E radiation for year 2000 derived by satellite observations (from Total Ozone Mapping Spectroradiometer) and to ground based measurements at 14 sites. The model correlates well with the observations; the correlation coefficients are 0.97 and 0.98 for satellite and ground based measurements, respectively. In addition to the effect of changes in ozone, we also investigate the effect of changes in SO<sub>2</sub>, NO<sub>2</sub>, the direct and indirect effects of aerosols, albedo changes and aviation-induced contrails and cirrus. The results show an increase of surface UV-E in polar regions, most strongly in the Southern Hemisphere. Furthermore, our study also shows an extensive surface UV-E reduction over most land areas; a reduction up to 20% since 1750 is found in some industrialized regions. This reduction in UV-E over the industrial period is particularly large in highly populated regions
Optical properties in the UV and visible spectral region of organic acids relevant to tropospheric aerosols
International audienceRefractive and absorption indices in the UV and visible region of selected aqueous organic acids relevant to tropospheric aerosols are reported. The acids investigated are the aliphatic dicarboxylic acids oxalic, malonic, tartronic, succinic and glutaric acid. In addition we report data for pyruvic, pinonic, benzoic and phthalic acid. To cover a wide range of conditions we have investigated the aqueous organic acids at different concentrations spanning from highly diluted samples to concentrations close to saturation. The density of the investigated samples is reported and a parameterisation of the absorption and refractive index that allows the calculation of the optical constants of mixed aqueous organic acids at different concentrations is presented. The single scattering albedo is calculated for two size distributions using measured and a synthetic set of optical constants. The results show that tropospheric aerosols consisting of only these organic acids and water have a pure scattering effect
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Emerging Asian aerosol patterns
Anthropogenic aerosol emissions over Asia are changing rapidly, both in composition and spatial distribution1. The Shared Socioeconomic Pathways (SSPs), potential narratives of development used by the Intergovernmental Panel for Climate Change in future projections, span a range of influences of aerosols on climate over the next decades. Several of these narratives project the continuation of a trend manifested in observations since 2010, with a clear dipole between South and East Asia.
The patterns of radiative forcing that result from these distributions of aerosols will differ from those of the late 20th century. They may instigate large-scale atmospheric responses that could have wide ranging impacts on climate and society well beyond the aerosol source regions. South and East Asia are particularly vulnerable to climate change because of strong seasonal variations in precipitation, high average temperature, and very high population density. Therefore, any aerosol impacts on the strength or seasonal variations in monsoon rainfall, freshwater availability, or climate extremes, will incur large societal costs. We urge the scientific community to make definite progress towards understanding and quantifying the impacts of Asian aerosols and to tackle the potentially large regional and hemispheric implications of these emerging trends
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Halfway to doubling of CO2 radiative forcing
The “double CO2” experiment has become a standard experiment in climate science, and a convenient way of comparing the sensitivity of different climate models. Double CO2 was first used by Arrhenius in the 19th century and in the classic paper by Manabe and Wetherald, published 50 years ago, which marked the start of the modern era of climate modeling. Doubling CO2 now has an iconic role in climate research. The equilibrium climate sensitivity (ECS) is defined as the global-mean surface temperature change resulting from a doubling of CO2, which is a headline result in Intergovernmental Panel on Climate Change (IPCC) assessments. In its most recent assessment IPCC concluded that the ECS “is likely in the range 1.5 to 4.5oC”. We show that we are now halfway to doubling of CO2 since pre-industrial times in terms of radiative forcing, but not in concentration
Clinical and Histopathological Prognostic Factors in Chondrosarcomas
Purpose. In an attempt to identify clinical and histopathological factors of prognostic
importance in chondrosarcomas, 115 cases of malignant and borderline chondromatous tumours were reviewed
Land cover change in low-warming scenarios may enhance the climate role of secondary organic aerosols
Most socioeconomic pathways compatible with the aims of the Paris Agreement include large changes to land use and land cover. The associated vegetation changes can interact with the atmosphere and climate through numerous mechanisms. One of these is emissions of biogenic volatile organic compounds (BVOCs), which may lead to the formation of secondary organic aerosols (SOAs) and atmospheric chemistry changes. Here, we use a modeling framework to explore potential future global and regional changes in SOA and tropospheric ozone following idealized, large-scale vegetation perturbations, and their resulting radiative forcing (RF). Guided by projections in low-warming scenarios, we modify crop and forest cover, separately, and in concurrence with changes in anthropogenic emissions and CO2 level. We estimate that increasing global forest cover by 30% gives a 37% higher global SOA burden, with a resulting forcing of −0.13 W m−2. The effect on tropospheric ozone is relatively small. Large SOA burden changes of up to 48% are simulated for South America and Sub-Saharan Africa. Conversely, increasing crop cover at the expense of tropical forest, yields similar changes but of opposite sign. The magnitude of these changes is strongly affected by the concurrent evolution of anthropogenic emissions. Our land cover perturbations are representative of energy crop expansion and afforestation, two key mitigation measures in 1.5 °C compatible scenarios. Our results hence indicate that depending on the role of these two in the underlying mitigation strategies, scenarios with similar long-term global temperature levels could lead to opposite effects on SOA. Combined with the complexity of factors that control SOA, this highlights the importance of including BVOC effects in further studies and assessments of climate and air quality mitigation involving the land surface
A Retrospective Clinicopathological Study of 37 Patients With Chordoma: A Danish National Series
Purpose. There are, in general, few published series on chordoma. It is a rare disease and further data are still needed
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Multi-model simulations of aerosol and ozone radiative forcing due to anthropogenic emission changes during the period 1990-2015
Over the past few decades, the geographical distribution of emissions of substances that alter the atmospheric energy balance has changed due to economic growth and air pollution regulations. Here, we show the resulting changes to aerosol and ozone abundances and their radiative forcing, using recently updated emission data for the period 1990-2015, as simulated by seven global atmospheric composition models. The models broadly reproduce large-scale changes in surface aerosol and ozone based on observations (e.g., -1 to -3%/yr in aerosols over 30 the US and Europe). The global mean radiative forcing due to ozone and aerosol changes over the 1990-2015 period increased by +0.17 ±0.08 Wm-2, with approximately 1/3 due to ozone. This increase is more strongly positive than that reported in IPCC AR5. The main reasons for the increased positive radiative forcing of aerosols over this period are the substantial reduction of global mean SO2 emissions, which is stronger in the new emission inventory compared to that used in the IPCC analysis, and higher black carbon emissions
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