K-shell processes in heavy-ion collisions in solids and the local plasma approximation

We have investigated K-shell vacancy production due to ionization and electron transfer processes, in collisions of highly charged oxygen ions with various solid targets such as Cl, K, Ti, Fe, and Cu at energies between 1.5 and 6.0 MeV/u. The K-shell ionization cross sections were derived from the measured K x-ray cross sections. An ab initio theoretical model based on the local plasma approximation ͑LPA͒, which is an extension of the dielectric formalism to consider core electrons, provides an explanation of the measured data only qualitatively. In case of asymmetric collisions (Z p /Z t Ͻ0.35, Z p , Z t being the atomic numbers of the projectile and target, respectively͒ and at higher energies, the LPA model explains the data to some extent but deviates for more symmetric collision systems. On the other hand, a perturbed-stationary-state ͑PSS͒ calculation ͑ECPSSR͒, including the corrective terms due to energy ͑E͒ loss, Coulomb ͑C͒ deflection, and relativistic ͑R͒ wave functions designed for ion-atom collisions agree quite well with the data for different combinations of target and projectile elements. In addition, we have also measured the K͑target͒-K͑projectile͒ electron transfer cross sections and compared them with a model based on perturbed-stationary-state approximation

Two-Center Effect on Low-Energy Electron Emission in Collisions of 1-MeV/u Bare Ions with Atomic Hydrogen, Molecular Hydrogen, and Helium: II. H\u3csub\u3e2\u3c/sub\u3e and He

We have studied the energy and angular distributions of low-energy electron emission in collisions of bare carbon ions of 1-MeV/u energy with He and H2 targets. The double-differential cross sections (DDCS’s) are measured for electrons with energies between 0.5 and 300 eV emitted within an angular range of 15° to 160°. The large forward-backward asymmetry observed in the angular distributions is explained in terms of the two-center effect. Single differential cross sections (SDCS’s) and total cross sections are also derived by integrating the DDCS’s over emission angles and energies. The data are compared with different theoretical calculations based on the first Born, CDW (continuum-distorted-wave), and CDW-EIS (eikonal-initial-state) approximations. The angular distributions of DDCS’s and SDCS’s are shown to deviate largely from the predictions of the B1 calculations, and are in much better agreement with both the continuum distorted-wave models. The CDW approximation provides a better agreement with the data compared to the CDW-EIS approximation, especially at higher electron energies. The total ionization cross sections for all three targets are shown to follow a scaling rule approximately

Two-Center Effect on Low-Energy Electron Emission in Collisions of 1-MeV/u Bare Ions with Atomic Hydrogen, Molecular Hydrogen, and Helium: II. H\u3csub\u3e2\u3c/sub\u3e and He

We have studied the energy and angular distributions of low-energy electron emission in collisions of bare carbon ions of 1-MeV/u energy with He and H2 targets. The double-differential cross sections (DDCS’s) are measured for electrons with energies between 0.5 and 300 eV emitted within an angular range of 15° to 160°. The large forward-backward asymmetry observed in the angular distributions is explained in terms of the two-center effect. Single differential cross sections (SDCS’s) and total cross sections are also derived by integrating the DDCS’s over emission angles and energies. The data are compared with different theoretical calculations based on the first Born, CDW (continuum-distorted-wave), and CDW-EIS (eikonal-initial-state) approximations. The angular distributions of DDCS’s and SDCS’s are shown to deviate largely from the predictions of the B1 calculations, and are in much better agreement with both the continuum distorted-wave models. The CDW approximation provides a better agreement with the data compared to the CDW-EIS approximation, especially at higher electron energies. The total ionization cross sections for all three targets are shown to follow a scaling rule approximately

Two-Center Effect on Low-Energy Electron Emission in Collisions of 1-MeV/u Bare Ions with Atomic Hydrogen, Molecular Hydrogen, and Helium. I. Atomic Hydrogen

We have investigated ionization mechanisms in fast ion-atom collisions by measuring the low-energy electron emission cross sections in a pure three-body collision involving bare carbon ions (v=6.35 a.u.) colliding with atomic hydrogen targets. The measurements have also been extended to molecular hydrogen and helium targets. In this paper we provide the energy and angular distributions of double differential cross sections of low-energy electron emission for atomic hydrogen targets. The Slevin rf source with a high degree of dissociation was used to produce the atomic H target. It is found that the two-center effect has a major influence on the observed large forward-backward angular asymmetry. A detailed comparison is presented with calculations based on the continuum distorted-wave (CDW) and CDW-EIS (eikonal initial-state) approximations. Both the continuum distorted-wave calculations provide a very good understanding of the data, whereas the first Born calculation predicts almost symmetric forward-backward distributions that do not agree with the data. The two-center effect is slightly better represented by the CDW calculations compared to the CDW-EIS calculation. The total cross sections are, however, in good agreement with the theories used. The results for molecular hydrogen and helium will be discussed in the following paper

Impact ionization of molecular oxygen by 3.5-MeV/u bare carbon ions

We have measured the absolute double-differential cross sections (DDCSs) for electron emission in ionization of O2 molecules under the impact of 3.5-MeV/u C6+ ions. The data were collected between 10 and 600 eV, in an angular range of 30◦ to 150◦. The single-differential cross sections (SDCSs) in emission angle and electron energy are deduced from the electron DDCS spectra. Also, the total cross section has been obtained from the SDCS spectra. The DDCS spectra as well as the SDCS spectra are compared with continuum distorted-wave eikonal initial-state calculations which employ molecular wave functions built as linear combinations of atomic orbitals. The DDCS ratio i.e. σO2/2σO, derived by dividing the experimental DDCS for molecular oxygen with the theoretical DDCS for atomic oxygen, does not show any primary or secondary oscillations arising from Young-type interference, which is apparently in contrast to what has been observed earlier for H2 and in agreement with the model calculation. Similarly, the forward-backward angular asymmetry increases monotonically with the velocity of the emitted electrons. However, the results on the DDCSs, SDCSs, the asymmetry parameter, and the nonexistence of oscillations are in qualitative agreement with the predictions of the model usedOne of the authors (F.M.) acknowledges the financial support from the MICINN Projects No. FIS2010-15127 and No. CSD 2007- 00010. C.A.T., R.D.R., and F.M. acknowledge the Programa de Cooperación Interuniversitaria e Investigación Científica entre España e Iberoamérica AECID Project No. A2/039631/1

Doubly Differential Cross Sections of Low-Energy Electrons Emitted in the Ionization of Molecular Hydrogen by Bare Carbon Ions

We have measured the double differential cross sections (DDCS) (d2σ/dεedΩe) of low-energy electron emission in the ionization of H2 bombarded by bare carbon ions of energy 30 MeV. The energy and angular distributions of the electron DDCS have been obtained for 12 different emission angles and for electron energies varying between 0.1 and 300 eV. We have also deduced the single differential and total ionization cross section from the measured DDCS. The data have been compared with the predictions of first Born approximations and the CDW-EIS (continuum distorted wave–eikonal initial state) model. The CDW-EIS model provides an excellent agreement with the data. [S1050-2947~96!10109-8

Electron Capture by Proton Beam in Collisions with Water Vapor

In low energy ion-molecule collisions, electron capture is one of the most important channels. A new experimental setup was developed to study the electron capture process using low-energy ion beams extracted from an electron cyclotron resonance (ECR) plasma-based ion accelerator. Experiments were carried out with the proton beam colliding with water vapor in the energy range of 70–300 keV. Capture events were detected using a position-sensitive detection system comprising micro channel plates (MCPs) and a delay line detector (DLD). These e-capture events can be a result of pure capture reactions as well as transfer ionization. The capture cross section was found to decrease sharply with the beam energy and agreed well with previous measurements. The setup was also used to detect the events that gave rise to the single and multiple e-capture (integrated over all recoil-ion charge states) of C4+ ions. The capture cross-sections for one, two, three, and four electrons were measured for 100 keV C4+ ions. The ratio of multielectron capture yield to that for single e-capture decreased with the number of captured electrons