284 research outputs found
Spin-orbit excitations of quantum wells
Confinement asymmetry effects on the photoabsorption of a quantum well are
discussed by means of a sum-rules approach using a Hamiltonian including a
Rashba spin-orbt coupling. We show that while the strength of the excitation is
zero when the spin-orbit coupling is neglected, the inclusion of the spin-orbit
interaction gives rise to a non zero strength and mean excitation energy in the
far-infrared region. A simple expression for these quantities up to the second
order in the Rashba parameter was derived. The effect of two-body Coulomb
interaction is then studied by means of a Quantum Monte Carlo calculation,
showing that electron-electron correlations induce only a small deviation from
the independent particle model result
Spin-orbit effects on the Larmor dispersion relation in GaAs quantum wells
We have studied the relevance of spin-orbit coupling to the dispersion 00009
relation of the Larmor resonance observed in inelastic light scattering and
electron-spin resonance experiments on GaAs quantum wells. We show that the
spin-orbit interaction, here described by a sum of Dresselhaus and
Bychkov-Rashba terms, couples Zeeman and spin-density excitations. We have
evaluated its contribution to the spin splitting as a function of the magnetic
field , and have found that in the small limit, the spin-orbit
interaction does not contribute to the spin splitting, whereas at high magnetic
fields it yields a independent contribution to the spin splitting given by
, with being the intensity of the
Bychkov-Rashba and Dresselhaus spin-orbit terms.Comment: To be published in Physical Review
Orbital current mode in elliptical quantum dots
An orbital current mode peculiar to deformed quantum dots is theoretically
investigated; first by using a simple model that allows to interpret
analytically its main characteristics, and second, by numerically solving the
microscopic equations of time evolution after an initial perturbation within
the time-dependent local-spin-density approximation. Results for different
deformations and sizes are shown.Comment: 4 REVTEX pages, 4 PDF figures, accepted in PRB:R
Spin and density longitudinal response of quantum dots in time-dependent local-spin-density approximation
The longitudinal dipole response of a quantum dot has been calculated in the
far-infrared regime using local spin density functional theory. We have studied
the coupling between the collective spin and density modes as a function of the
magnetic field. We have found that the spin dipole mode and single particle
excitations have a sizeable overlap, and that the magnetoplasmon modes can be
excited by the dipole spin operator if the dot is spin polarized. The frequency
of the dipole spin edge mode presents an oscillation which is clearly filling
factor () related. We have found that the spin dipole mode is especially
soft for even values, becoming unstable for magnetic fields in the region
. Results for selected number of electrons and confining
potentials are discussed. An analytical model which reproduces the main
features of the microscopic spectra has been developed.Comment: We have added some new references and minor changes on the mnuscript
have been mad
Structure and far-infrared edge modes of quantum antidots at zero magnetic field
We have investigated edge modes of different multipolarity sustained by
quantum antidots at zero magnetic field. The ground state of the antidot is
described within a local density functional formalism. Two sum rules, which are
exact within this formalism, have been derived and used to evaluate the energy
of edge collective modes as a function of the surface density and the size of
the antidot.Comment: Typeset using Revtex, 8 pages and 6 Postscript figure
Optical response of two-dimensional few-electron concentric double quantum rings: A local-spin-density-functional theory study
We have investigated the dipole charge- and spin-density response of
few-electron two-dimensional concentric nanorings as a function of the
intensity of a perpendicularly applied magnetic field. We show that the dipole
response displays signatures associated with the localization of electron
states in the inner and outer ring favored by the perpendicularly applied
magnetic field. Electron localization produces a more fragmented spectrum due
to the appearance of additional edge excitations in the inner and outer ring.Comment: To be published in Physical Review
Effective Field Theory for the Quantum Electrodynamics of a Graphene Wire
We study the low-energy quantum electrodynamics of electrons and holes, in a
thin graphene wire. We develop an effective field theory (EFT) based on an
expansion in p/p_T, where p_T is the typical momentum of electrons and holes in
the transverse direction, while p are the momenta in the longitudinal
direction. We show that, to the lowest-order in (p/p_T), our EFT theory is
formally equivalent to the exactly solvable Schwinger model. By exploiting such
an analogy, we find that the ground state of the quantum wire contains a
condensate of electron-hole pairs. The excitation spectrum is saturated by
electron-hole collective bound-states, and we calculate the dispersion law of
such modes. We also compute the DC conductivity per unit length at zero
chemical potential and find g_s =e^2/h, where g_s=4 is the degeneracy factor.Comment: 7 pages, 2 figures. Definitive version, accepted for publication on
Phys. Rev.
An enhanced sampling QM/AMOEBA approach: The case of the excited state intramolecular proton transfer in solvated 3-hydroxyflavone
We present an extension of the polarizable quantum mechanical (QM)/AMOEBA approach to enhanced sampling techniques. This is achieved by connecting the enhanced sampling PLUMED library to the machinery based on the interface of Gaussian and Tinker to perform QM/AMOEBA molecular dynamics. As an application, we study the excited state intramolecular proton transfer of 3-hydroxyflavone in two solvents: methanol and methylcyclohexane. By using a combination of molecular dynamics and umbrella sampling, we find an ultrafast component of the transfer, which is common to the two solvents, and a much slower component, which is active in the protic solvent only. The mechanisms of the two components are explained in terms of intramolecular vibrational redistribution and intermolecular hydrogen-bonding, respectively. Ground and excited state free energies along an effective reaction coordinate are finally obtained allowing for a detailed analysis of the solvent mediated mechanism
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