Polymer Electret Improves the Performance of the Oxygen-Doped Organic Field-Effect Transistors

Chemical doping is widely used in the electronic devices. In p-type semiconductor thin films, oxygen doping fills the hole traps and increases hole concentrations, improving the performance of the organic field-effect transistors (OFETs). Due to the low ionization potential for p-type semiconductors, the superfluous holes induced by the oxygen doping degrades the OFETs off-state leakage performance. On the other hand, for p-type semiconductors with high ionization potential (up to 5.5-6.0 eV), the limited oxidation of oxygen is hard to achieve satisfactory doping concentrations to fill the trap states. This refers to the well-known intrinsic incompatibility between the oxygen doping and high-performance OFETs. Herein, a novel strategy is introduced to overcome the incompatibility and achieve high-performance OFETs by using the structural polymer electret. That is, moderate hole concentrations induced by low-pressure (30 Pa) oxygen plasma fill the hole traps within semiconductor. And the built-in field resulted from polymer electret accumulates the holes inside semiconductor near the semiconductor/electret interface, thus improving the OFETs performance. Using a model organic semiconductor with high ionization potential-2,7-didodecyl[1]benzothieno [3,2-b][1]benzothiophene (C12-BTBT) as an example, the high-performance OFETs with field-effect mobility (μFET) of 3.5 cm 2 V -1 s -1 , subthreshold-swing (SS) of 110 mV decade -1 , on-off ratio of 10 4 , and widely-tunable threshold voltage (V t ) are realized at a low voltage below 2 V in the open air

Reticulation is a Risk Factor of Progressive Subpleural non-Fibrotic Interstitial Lung Abnormalities

Rationale: Interstitial lung abnormalities (ILAs) are being increasingly identified in clinical practice. In particular for subpleural non-fibrotic ILAs, the risk of progression over time and the risk factors for progressive behavior are still largely unknown. Objectives: To determine the age band prevalence of ILAs and the risk of radiological progression of subpleural non-fibrotic ILAs over time in a large health check-up population, and to identify how reticulation contributes to the risk of radiological progression. Methods: Based on ILAs definition by the Fleischner Society, low-dose chest CT images from community-dwelling population undergone health check-up were evaluated for ILAs. Multivariable logistic regression was used to assess the risk of radiological progression. Measurements and Main Results: Among 155,539 individuals, 3,300 (2.1%) were confirmed to have ILAs: the vast majority (81.7%) were defined as subpleural non-fibrotic ILAs. The prevalence of ILAs increased linearly with age (P for trend<0.0001). Of 454 individuals with subpleural non-fibrotic ILAs, 198 (43.6%) had radiological progression over 4 years. The presence of reticulation on initial imaging was an independent predictor of radiological progression (OR 1.9; 95%CI 1.2-3.0, P=0.0040). No difference in radiological progression was identified between subpleural non-fibrotic ILAs with extensive reticulation and subpleural fibrotic ILAs (73.0% vs. 68.8%, P=0.7626). Conclusions: The prevalence of ILAs increases linearly with age. Nearly half of subpleural non-fibrotic ILAs progress radiologically over 4 years. The presence of reticulation is a risk factor for radiological progression. Subpleural non-fibrotic ILAs with extensive reticulation are likely to be a feature of subpleural fibrotic ILAs

Data-Driven Modeling of Systemic Air Traffic Delay Propagation: An Epidemic Model Approach

To better understand the mechanism of air traffic delay propagation at the system level, an efficient modeling approach based on the epidemic model for delay propagation in airport networks is developed. The normal release rate (NRR) and average flight delay (AFD) are considered to measure airport delay. Through fluctuation analysis of the average flight delay based on complex network theory, we find that the long-term dynamic of airport delay is dominated by the propagation factor (PF), which reveals that the long-term dynamic of airport delay should be studied from the perspective of propagation. An integrated airport-based Susceptible-Infected-Recovered-Susceptible (ASIRS) epidemic model for air traffic delay propagation is developed from the network-level perspective, to create a simulator for reproducing the delay propagation in airport networks. The evolution of airport delay propagation is obtained by analyzing the phase trajectory of the model. The simulator is run using the empirical data of China. The simulation results show that the model can reproduce the evolution of the delay propagation in the long term and its accuracy for predicting the number of delayed airports in the short term is much higher than the probabilistic prediction method. The model can thus help managers as a tool to effectively predict the temporal and spatial evolution of air traffic delay

Distribution, Genesis, and Human Health Risks of Groundwater Heavy Metals Impacted by the Typical Setting of Songnen Plain of NE China

Heavy metals pollution in groundwater and the resulting health risks have always been an environmental research hotspot. However, the available information regarding this topic and associated methods is still limited. This study collected 98 groundwater samples from a typical agricultural area of Songnen Plain in different seasons. The pollution status and sources of ten heavy metals (As, Ba, Cd, Co, Cr (VI), Cu, Fe, Mn, Ni, Pb, and Zn) were then analyzed and compared. In addition, the human health risks assessment (HHRA) model was used to calculate human health risks caused by heavy metals in groundwater. The results revealed that heavy metals were mainly distributed in the northwest of the study area and along the upper reaches of the Lalin river and that the concentrations of heavy metals were higher during the wet season than the dry season. Industrial and agricultural activities and natural leaching are the main sources, and each kind of heavy metal may have different sources. Fe and Mn are the primary pollutants, mainly caused by the native environment and agricultural activities. The exceeding standard rates are 71.74% and 61.54%, respectively based on the Class III of Quality Standard for Groundwater of China (GB/T 14848-2017). The maximum exceeding multiple are 91.45 and 32.05, respectively. The health risks of heavy metals borne by different groups of people were as follows: child > elder > young > adult. Carcinogenic heavy metals contribute to the main risks, and the largest risks sources are Cr and As. Therefore, the government should appropriately restrict the use of pesticides and fertilizers, strictly manage the discharge of enterprises, and control man-made heavy metals from the source. In addition, centralized water supply and treatment facilities shall be established to prevent the harm of native heavy metals

Advances in mineral processing technologies related to iron, magnesium, and lithium

Exploitation and utilization of mineral resources have played a vital role in China's rapid economic developments. Although the history of mineral processing is quite long, technologies in this field have varied with the changes of market demands. This is particularly the case for minerals whose high-grade deposits are depleting. The aim of this review is to present our recent efforts on developing new routes for the utilization of low-grade minerals, such as iron ores and brine-containing lithium. The emphasis on the two minerals lies in the fact that iron plays a vital role in modern-day civilization and lithium is a key component in electric vehicles for transportation. Furthermore, the utilization of magnesium chloride reserves, one of the largest wastes in western China, as raw materials for fabrication of functional materials is also included in this review

Influence of Pore Structure and Solid Bitumen on the Development of Deep Carbonate Gas Reservoirs: A Case Study of the Longwangmiao Reservoir in Gaoshiti–Longnusi Area, Sichuan Basin, SW China

A variable sedimentary environment and accumulation process leads to a complex pore structure in deep carbonate gas reservoirs, and the physical properties are quite different between layers. Moreover, some pores and throats are filled with solid bitumen (SB), which not only interferes with reservoir analysis, but also affects efficient development. However, previous studies on SB mainly focused on the accumulation process and reservoir analysis, and there are few reports about the influence on development. In this paper, through scanning electron microscope analysis, SB extraction, gas flow experiments and depletion experiments, and a similar transformation between experimental results and reservoir production, the production characteristics of carbonate gas reservoirs with different pore structures were studied, and the influence of SB on pore structure, reservoir analysis and development were systematically analyzed. The results show that permeability is one of the key factors affecting gas production rate and recovery, and the production is mainly contributed by high-permeability layers. Although the reserves are abundant, the gas production rate and recovery of layers with a low permeability are relatively low. The SB reduces the pore and throat radius, resulting in porosity and permeability being decreased by 4.73–6.28% and 36.02–3.70%, respectively. With the increase in original permeability, the permeability loss rate decreases. During development, the loss rate of gas production rate is much higher than that of permeability. Increasing the production pressure difference is conducive to reducing the influence. SB also reduces the recovery, which leads to the loss rate of gas production being much higher than that of porosity. For reservoirs with a high permeability, the loss rates of gas production rate and the amount produced are close to those of permeability and porosity. Therefore, in the reservoir analysis and development of carbonate gas reservoirs bearing SB, it is necessary and significant to analyze the influence of reservoir types

Data_Sheet_1_Low-host double MDA workflow for uncultured ASFV positive blood and serum sample sequencing.DOCX

African swine fever (ASF) is a highly lethal and contagious disease caused by African swine fever virus (ASFV). Whole-genome sequencing of ASFV is necessary to study its mutation, recombination, and trace its transmission. Uncultured samples have a considerable amount of background DNA, which causes waste of sequencing throughput, storage space, and computing resources. Sequencing methods attempted for uncultured samples have various drawbacks. In this study, we improved C18 spacer MDA (Multiple Displacement Amplification)-combined host DNA exhaustion strategy to remove background DNA and fit NGS and TGS sequencing. Using this workflow, we successfully sequenced two uncultured ASFV positive samples. The results show that this method can significantly reduce the percentage of background DNA. We also developed software that can perform real-time base call and analyses in set intervals of ASFV TGS sequencing reads on a cloud server.</p

Gelatin and catechol-modified quaternary chitosan cotton dressings with rapid hemostasis and high-efficiency antimicrobial capacity to manage severe bleeding wounds

The development of functional wound dressings capable of both rapid hemostasis and high-efficiency antimicrobial is essential for the management of severe bleeding wounds. Cotton dressings are widely used in clinical practice; however, few dressings can simultaneously achieve rapid hemostasis and high-efficacy antimicrobial. Herein, a versatile cotton dressing (GCQCNF-5) was masterly developed by sequentially deposition catechol modified quaternary chitosan (CQCS) and gelatin onto a cotton nonwoven fabric (NF) surface. Because of the presence of a gelatin sponge layer with suitable thickness and porosity on its surface, GCQCNF-5 exhibits a notably enhanced hemostatic effect compared to NF both in vitro and in vivo, which is even slightly superior to that of MHS (a commercial gelatin hemostatic sponge). Moreover, after exerting a rapid hemostasis effect, GCQCNF-5 can further exploit CQCS to exert excellent immediate antimicrobial and long-lasting bacteriostatic effects. In vivo wound healing experiments further indicated that GCQCNF-5 could significantly promote rapid healing of infected wounds by effectively sterilizing, absorbing exudates, and providing moist healing environments. This study clearly demonstrated that GCQCNF-5 is a versatile wound dressing that can achieve simultaneously rapid hemostasis, high-efficiency antimicrobial, and promote rapid healing of infected wounds, with great application potential for the treatment of severe bleeding wounds