Giant isotope effect in the incoherent tunneling specific heat of the molecular nanomagnet Fe8

Time-dependent specific heat experiments on the molecular nanomagnet Fe8 and the isotopic enriched analogue 57Fe8 are presented. The inclusion of the 57Fe nuclear spins leads to a huge enhancement of the specific heat below 1 K, ascribed to a strong increase in the spin-lattice relaxation rate Gamma arising from incoherent, nuclear-spin-mediated magnetic quantum tunneling in the ground-doublet. Since Gamma is found comparable to the expected tunneling rate, the latter process has to be inelastic. A model for the coupling of the tunneling levels to the lattice is presented. Under transverse field, a crossover from nuclear-spin-mediated to phonon-induced tunneling is observed.Comment: Replaced with version accepted for publication in Physical Review Letter

Quantum dot dephasing by edge states

We calculate the dephasing rate of an electron state in a pinched quantum dot, due to Coulomb interactions between the electron in the dot and electrons in a nearby voltage biased ballistic nanostructure. The dephasing is caused by nonequilibrium time fluctuations of the electron density in the nanostructure, which create random electric fields in the dot. As a result, the electron level in the dot fluctuates in time, and the coherent part of the resonant transmission through the dot is suppressed

Quantized adiabatic quantum pumping due to interference

Recent theoretical calculations, demonstrating that quantized charge transfer due to adiabatically modulated potentials in mesoscopic devices can result purely from the interference of the electron wave functions (without invoking electron-electron interactions) are reviewed: (1) A new formula is derived for the pumped charge Q (per period); It reproduces the Brouwer formula without a bias, and also yields the effect of the modulating potential on the Landauer formula in the presence of a bias. (2) For a turnstile geometry, with time-dependent gate voltages V_L(t) and V_R(t), the magnitude and sign of Q are determined by the relative position and orientation of the closed contour traversed by the system in the {V_L-V_R} plane, relative to the transmission resonances in that plane. Integer values of Q (in units of e) are achieved when a transmission peak falls inside the contour, and are given by the winding number of the contour. (3) When the modulating potential is due to surface acoustic waves, Q exhibits a staircase structure, with integer values, reminiscent of experimental observations.Comment: Invited talk, Localization, Tokyo, August 200

Acoustoelectric current and pumping in a ballistic quantum point contact

The acoustoelectric current induced by a surface acoustic wave (SAW) in a ballistic quantum point contact is considered using a quantum approach. We find that the current is of the "pumping" type and is not related to drag, i.e. to the momentum transfer from the wave to the electron gas. At gate voltages corresponding to the plateaus of the quantized conductance the current is small. It is peaked at the conductance step voltages. The peak current oscillates and decays with increasing SAW wavenumber for short wavelengths. These results contradict previous calculations, based on the classical Boltzmann equation.Comment: 4 pages, 1 figur

Book Reviews

When considered as an installment in the unfolding of Friedmann\u27s views, based on his earlier writings, the conclusion to the book under review is to be cherished. When considered, on the other hand, solely in context of the contributed chapters of the same volume, the conclusion does not emerge as Friedmann at his most forceful or persuasive. To find the best of Friedmann, we need only sample his prolific contributions to the law reviews, whether on the United States involvement in the Vietnam conflict, the judgment of the International Court in the South West Africa cases, the risks to humanity arising from genetic engineering, or the relationship between law and mankind\u27s sense of justice

BOOK REVIEWS: Ethics at the Edges of Life / Samuel Johnson

Professor Paul Ramsey,\u27 writing as a Christian ethicist, has revised, extended, and updated the Bampton Lectures in America that he delivered in 1975 at Columbia University. The resulting book is Ethics at the Edges of Life: Medical and Legal Intersections. A substantial portion of the book is devoted to critical analysis of a number of landmark court decisions, all of which were rendered after his delivery of the Bampton lectures--Planned Parenthood v. Danforth, on abortion; Commonwealth v. Edelin, on the treatment of a fetus during or immediately after an abortion; In re Quinlan, on the termination of life support; and Superintendent of Belchertown State School v. Saikewicz,\u27 on the decision not to provide life-prolonging treatment. The book also analyzes a statutory post-Bampton development-the 1976 California Natural Death Act.\u27 - - - - - - - - - - - - - - - - - - - - - - - With the observation that Samuel Johnson has fascinated more people than any other writer except Shakespeare, Professor W. Jackson Bate of Harvard University opens this profound biography. Now available to readers for more than three years, with the immediate excitement of its publication well-passed, the book clearly stands out as the quintessential presentation of the life of Johnson and as a monument of its genre. The force of Bate\u27s book results from his ability to combine research and literary talents.From a vast amount of material, Professor Bate has ferreted out the essential data for the composition of a portrait that depicts Johnson as the whole man, his eccentricity and greatness blended to perfection. Moreover, Bate has compiled his findings in a manner both pleasant and instructive that makes his presentation an independent work of art

Carbide coated fibers in graphite-aluminum composites

The NASA-supported program at the Los Alamos Scientific Laboratory (LASL) to develop carbon fiber-aluminum matrix composites is described. Chemical vapor deposition (CVD) was used to uniformly deposit thin, smooth, continuous coats of TiC on the fibers of graphite tows. Wet chemical coating of fibers, followed by high-temperature treatment, was also used, but showed little promise as an alternative coating method. Strength measurements on CVD coated fiber tows showed that thin carbide coats can add to fiber strength. The ability of aluminum alloys to wet TiC was successfully demonstrated using TiC-coated graphite surfaces. Pressure-infiltration of TiC- and ZrC-coated fiber tows with aluminum alloys was only partially successful. Experiments were performed to evaluate the effectiveness of carbide coats on carbon as barriers to prevent reaction between alluminum alloys and carbon. Initial results indicate that composites of aluminum and carbide-coated graphite are stable for long periods of time at temperatures near the alloy solidus

Carbide coated fibers in graphites-aluminum composites

Research activities are described for a NASA-supported program at the Los Alamos Scientific Laboratory to develop graphite fiber-aluminum matrix composites. A chemical vapor deposition apparatus was constructed for continuously coating graphite fibers with TiC. As much as 150 meters of continuously coated fibers were produced. Deposition temperatures were varied from 1365 K to about 1750 K, and deposition time from 6 to 150 seconds. The 6 sec deposition time corresponded to a fiber feed rate of 2.54 m/min through the coater. Thin, uniform, adherent TiC coats, with thicknesses up to approximately 0.1 micrometer were produced on the individual fibers of Thornel 50 graphite yarns without affecting fiber strength. Although coat properties were fairly uniform throughout a given batch, more work is needed to improve the batch-to-batch reproducibility. Samples of TiC-coated Thornel 50 fibers were infiltrated with an aluminum alloy and hot-pressed in vacuum to produce small composite bars for flexure testing. Strengths as high as 90% of the rule-of-mixtures strength were achieved. Results of the examination of the fracture surfaces indicate that the bonding between the aluminum and the TiC-coated fibers is better than that achieved in a similar, commercially infiltrated material made with fibers having no observable surface coats. Several samples of Al-infiltrated, TiC-coated Thornel 50 graphite yarns, together with samples of the commercially infiltrated, uncoated fibers, were heated for 100 hours at temperatures near the alloy solidus. The TiC-coated samples appear to undergo less reaction than do the uncoated samples. Photomicrographs are shown

Carbide coated fibers in graphite-aluminum composites

The study of protective-coupling layers of refractory metal carbides on the graphite fibers prior to their incorporation into composites is presented. Such layers should be directly wettable by liquid aluminum and should act as diffusion barriers to prevent the formation of aluminum carbide. Chemical vapor deposition was used to uniformly deposit thin, smooth, continuous coats of ZrC on the carbon fibers of tows derived from both rayon and polyacrylonitrile. A wet chemical coating of the fibers, followed by high-temperature treatment, was used, and showed promise as an alternative coating method. Experiments were performed to demonstrate the ability of aluminum alloys to wet carbide surfaces. Titanium carbide, zirconium carbide and carbide-coated graphite surfaces were successfully wetted. Results indicate that initial attempts to wet surfaces of ZrC-coated carbon fibers appear successful

Adiabatic transport in nanostructures

A confined system of non-interacting electrons, subject to the combined effect of a time-dependent potential and different external chemical-potentials, is considered. The current flowing through such a system is obtained for arbitrary strengths of the modulating potential, using the adiabatic approximation in an iterative manner. A new formula is derived for the charge pumped through an un-biased system (all external chemical potentials are kept at the same value); It reproduces the Brouwer formula for a two-terminal nanostructure. The formalism presented yields the effect of the chemical potential bias on the pumped charge on one hand, and the modification of the Landauer formula (which gives the current in response to a constant chemical-potential difference) brought about by the modulating potential on the other. Corrections to the adiabatic approximation are derived and discussed.Comment: 8 pages, 2 figure