72 research outputs found
Global simulations of aerosol processing in clouds
An explicit and detailed representation of in-droplet and in-crystal aerosol particles in stratiform clouds has been introduced in the global aerosol-climate model ECHAM5-HAM. The new scheme allows an evaluation of the cloud cycling of aerosols and an estimation of the relative contributions of nucleation and collision scavenging, as opposed to evaporation of hydrometeors in the global aerosol processing by clouds. On average an aerosol particle is cycled through stratiform clouds 0.5 times. The new scheme leads to important changes in the simulated fraction of aerosol scavenged in clouds, and consequently in the aerosol wet deposition. In general, less aerosol is scavenged into clouds with the new prognostic treatment than what is prescribed in standard ECHAM5-HAM. Aerosol concentrations, size distributions, scavenged fractions and cloud droplet concentrations are evaluated and compared to different observations. While the scavenged fraction and the aerosol number concentrations in the marine boundary layer are well represented in the new model, aerosol optical thickness, cloud droplet number concentrations in the marine boundary layer and the aerosol volume in the accumulation and coarse modes over the oceans are overestimated. Sensitivity studies suggest that a better representation of below-cloud scavenging, higher in-cloud collision coefficients, or a reduced water uptake by seasalt aerosols could reduce these biases
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Time varying arctic climate change amplification
During the past 130 years the global mean surface air temperature has risen by about 0.75 K. Due to feedbacks -- including the snow/ice albedo feedback -- the warming in the Arctic is expected to proceed at a faster rate than the global average. Climate model simulations suggest that this Arctic amplification produces warming that is two to three times larger than the global mean. Understanding the Arctic amplification is essential for projections of future Arctic climate including sea ice extent and melting of the Greenland ice sheet. We use the temperature records from the Arctic stations to show that (a) the Arctic amplification is larger at latitudes above 700 N compared to those within 64-70oN belt, and that, surprisingly; (b) the ratio of the Arctic to global rate of temperature change is not constant but varies on the decadal timescale. This time dependence will affect future projections of climate changes in the Arctic
An AeroCom initial assessment – optical properties in aerosol component modules of global models
The AeroCom exercise diagnoses multi-component aerosol modules in global modeling. In an initial assessment simulated global distributions for mass and mid-visible aerosol optical thickness (aot) were compared among 20 different modules. Model diversity was also explored in the context of previous comparisons. For the component combined aot general agreement has improved for the annual global mean. At 0.11 to 0.14, simulated aot values are at the lower end of global averages suggested by remote sensing from ground (AERONET ca. 0.135) and space (satellite composite ca. 0.15). More detailed comparisons, however, reveal that larger differences in regional distribution and significant differences in compositional mixture remain. Of particular concern are large model diversities for contributions by dust and carbonaceous aerosol, because they lead to significant uncertainty in aerosol absorption (aab). Since aot and aab, both, influence the aerosol impact on the radiative energy-balance, the aerosol (direct) forcing uncertainty in modeling is larger than differences in aot might suggest. New diagnostic approaches are proposed to trace model differences in terms of aerosol processing and transport: These include the prescription of common input (e.g. amount, size and injection of aerosol component emissions) and the use of observational capabilities from ground (e.g. measurements networks) or space (e.g. correlations between aerosol and clouds)
Investigation of CO, C2H6 and aerosols in a boreal fire plume over eastern Canada during BORTAS 2011 using ground- and satellite-based observations, and model simulations
We present the results of total column measurements of CO, C2H6 and fine mode aerosol optical depth (AOD) during the "Quantifying the impact of BOReal forest fires on Tropospheric oxidants over the Atlantic using Aircraft and Satellites" (BORTAS-B) campaign over Eastern Canada. Ground-based observations, using Fourier transform spectrometers (FTSs) and sun photometers, were carried out in July and August 2011. These measurements were taken in Halifax, Nova Scotia, which is an ideal location to monitor the outflow of boreal fires from North America, and also in Toronto, Ontario. Measurements of fine mode AOD enhancements were highly correlated with enhancements in coincident trace gas (CO and C2H6) observations between 19 and 21 July 2011, which is typical for a smoke plume event. In this paper, we focus on the identification of the origin and the transport of this smoke plume. We use back-trajectories calculated by the Canadian Meteorological Centre as well as FLEXPART forward-trajectories to demonstrate that the enhanced CO, C2H6 and fine mode AOD seen near Halifax and Toronto originated from forest fires in Northwestern Ontario that occurred between 17 and 19 July 2011. In addition, total column measurements of CO from the satellite-borne Infrared Atmospheric Sounding Interferometer (IASI) have been used to trace the smoke plume and to confirm the origin of the CO enhancement. Furthermore, the emission ratio (ERC2H6/CO) and the emission factor (EFC2H6) of C2H6 (with respect to the CO emission) were estimated from these ground-based observations. These C2H6 emission results from boreal fires in Northwestern Ontario agree well with C2H6 emission measurements from other boreal regions, and are relatively high compared to fires from other geographical regions. The ground-based CO and C2H6 observations were compared with outputs from the 3-D global chemical transport model GEOS-Chem, using the Fire Locating And Monitoring of Burning Emissions (FLAMBE) inventory. Agreement within the stated measurement uncertainty was found for the magnitude of the enhancement of the total columns of CO (~3%) and C2H6 (~8%) between the measured and modelled results. However, there is a small shift in time (of approximately 6 h) of arrival of the plume over Halifax between the results
A case study of aerosol scavenging in a biomass burning plume over eastern Canada during the 2011 BORTAS field experiment
We present measurements of a long-range smoke transport event
recorded on 20–21 July 2011 over Halifax, Nova Scotia, Canada,
during the Quantifying the impact of BOReal forest fires on
Tropospheric oxidants over the Atlantic using Aircraft and
Satellites (BORTAS-B) campaign. Ground-based Fourier transform
spectrometers and photometers detected air masses associated with
large wildland fires burning in eastern Manitoba and western
Ontario.
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We investigate a plume with high trace gas amounts but low amounts
of particles that preceded and overlapped at the Halifax site with
a second plume with high trace gas loadings and significant amounts
of particulate material. We show that the first plume experienced
a meteorological scavenging event, but the second plume had not been
similarly scavenged. This points to the necessity to account
carefully for the plume history when considering long-range
transport since simultaneous or near-simultaneous times of arrival
are not necessarily indicative of either similar trajectories or
meteorological history. We investigate the origin of the scavenged
plume, and the possibility of an aerosol wet deposition event
occurring in the plume ~ 24 h prior to the measurements over
Halifax. The region of lofting and scavenging is only monitored on
an intermittent basis by the present observing network, and thus we
must consider many different pieces of evidence in an effort to
understand the early dynamics of the plume. Through this discussion
we also demonstrate the value of having many simultaneous
remote-sensing measurements in order to understand the physical and
chemical behaviour of biomass burning plumes
AÂ microwave satellite water vapour column retrieval for polar winter conditions
AÂ new microwave satellite water vapour retrieval for the polar winter
atmosphere is presented. The retrieval builds on the work of Miao et al. (2001) and Melsheimer and Heygster (2008), employing auxiliary
information for atmospheric conditions and numerical optimization. It was
tested using simulated and actual measurements from the Microwave Humidity
Sounder (MHS) satellite instruments. Ground truth was provided by the G-band
vapour radiometer (GVR) at Barrow, Alaska. For water vapour columns less than
6 kg m<sup>−2</sup>, comparisons between the retrieval and GVR result in a root mean square (RMS) deviation of 0.39 kg m<sup>−2</sup> and a systematic bias of 0.08 kg m<sup>−2</sup>. These results are compared with RMS
deviations and biases at Barrow for the retrieval of Melsheimer and Heygster (2008), the AIRS and MIRS satellite data products, and the ERA-Interim, NCEP, JRA-55, and ASR reanalyses. When applied to MHS measurements, the new retrieval
produces a smaller RMS deviation and bias than for the earlier retrieval and
satellite data products. The RMS deviations for the new retrieval were
comparable to those for the ERA-Interim, JRA-55, and ASR reanalyses; however,
the MHS retrievals have much finer horizontal resolution (15 km at
nadir) and reveal more structure. The new retrieval can be used to obtain
pan-Arctic maps of water vapour columns of unprecedented quality. It may also
be applied to measurements from the Special Sensor Microwave/Temperature 2
(SSM/T2), Advanced Microwave Sounding Unit B (AMSU-B), Special Sensor
Microwave Imager/Sounder (SSMIS), Advanced Technology Microwave Sounder
(ATMS), and Chinese MicroWave Humidity Sounder (MWHS) instruments
Cytogenetic Research on Hexaploid Alfalfa, Medicago Sativa
SUMMARYA spontaneously occurring hexaploid plant (2 n = 6x=48) was found among white-flowered tetraploid plants of Medicago sativa.This plant was studied from a morphological and cytological point of view. All the metaphases observed showed 48 chromosomes, six of which with large satellites. Total chromosome length ranged from μ 1.34 to μ 2.25 whereas that of tetraploid ranged from μ 2.08 to μ 2.83. Most diakinesis showed bivalents and 1 or, more frequently, 2 quadrivalents. Two or more univalents were observed in 56.4% of metaphases I and lagging chromosomes, varying in number from 1 to 4, were observed in 60% of anaphases II. Hexaploid pollen stainability (81%) was the same as in the tetraploid plants used as control (80%). The pollen grains were very variable in diameter (μ) and therefore two classes were distinguished: a smaller (diameter μ. 25.5) and a larger one (diameter μ 40.0). Such variability probably means that the hexaploid plant produces many unbalanced gametes which, in association with mei..
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