6,259 research outputs found

    Density Fluctuations in an Electrolyte from Generalized Debye-Hueckel Theory

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    Near-critical thermodynamics in the hard-sphere (1,1) electrolyte is well described, at a classical level, by Debye-Hueckel (DH) theory with (+,-) ion pairing and dipolar-pair-ionic-fluid coupling. But DH-based theories do not address density fluctuations. Here density correlations are obtained by functional differentiation of DH theory generalized to {\it non}-uniform densities of various species. The correlation length Ο\xi diverges universally at low density ρ\rho as (Tρ)−1/4(T\rho)^{-1/4} (correcting GMSA theory). When ρ=ρc\rho=\rho_c one has Ο≈Ο0+/t1/2\xi\approx\xi_0^+/t^{1/2} as t≡(T−Tc)/Tc→0+t\equiv(T-T_c)/T_c\to 0+ where the amplitudes Ο0+\xi_0^+ compare informatively with experimental data.Comment: 5 pages, REVTeX, 1 ps figure included with epsf. Minor changes, references added. Accepted for publication in Phys. Rev. Let

    Competing magnetic fluctuations and orders in a multiorbital model of doped SrCo2_2As2_2

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    We revisit the intriguing magnetic behavior of the paradigmatic itinerant frustrated magnet SrCo2As2\rm{Sr}\rm{Co}_2\rm{As}_2, which shows strong and competing magnetic fluctuations yet does not develop long-range magnetic order. By calculating the static spin susceptibility χ(q)\chi(\mathbf{q}) within a realistic sixteen orbital Hubbard-Hund model, we determine the leading instability to be ferromagnetic (FM). We then explore the effect of doping and calculate the critical Hubbard interaction strength UcU_c that is required for the development of magnetic order. We find that UcU_c decreases under electron doping and with increasing Hund's coupling JJ, but increases rapidly under hole doping. This suggests that magnetic order could possibly emerge under electron doping but not under hole doping, which agrees with experimental findings. We map out the leading magnetic instability as a function of doping and Hund's coupling and find several antiferromagnetic phases in addition to FM. We also quantify the degree of itinerant frustration in the model and resolve the contributions of different orbitals to the magnetic susceptibility. Finally, we discuss the dynamic spin susceptibility, χ(q,ω)\chi(\mathbf{q}, \omega), at finite frequencies, where we recover the anisotropy of the peaks at Qπ=(π,0)\mathbf{Q}_\pi = (\pi, 0) and (0,π)(0, \pi) observed by inelastic neutron scattering that is associated with the phenomenon of itinerant magnetic frustration. By comparing results between theory and experiment, we conclude that the essential experimental features of doped SrCo2_2As2_2 are well captured by a Hubbard-Hund multiorbital model if one considers a small shift of the chemical potential towards hole doping.Comment: 19 pages, 12 figure

    Ginzburg Criterion for Coulombic Criticality

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    To understand the range of close-to-classical critical behavior seen in various electrolytes, generalized Debye-Hueckel theories (that yield density correlation functions) are applied to the restricted primitive model of equisized hard spheres. The results yield a Landau-Ginzburg free-energy functional for which the Ginzburg criterion can be explicitly evaluated. The predicted scale of crossover from classical to Ising character is found to be similar in magnitude to that derived for simple fluids in comparable fashion. The consequences in relation to experiments are discussed briefly.Comment: 4 pages, revtex, 2 tables (latex2.09 required due to revtex's incompatibility with latex2e tables

    Applications of Field-Theoretic Renormalization Group Methods to Reaction-Diffusion Problems

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    We review the application of field-theoretic renormalization group (RG) methods to the study of fluctuations in reaction-diffusion problems. We first investigate the physical origin of universality in these systems, before comparing RG methods to other available analytic techniques, including exact solutions and Smoluchowski-type approximations. Starting from the microscopic reaction-diffusion master equation, we then pedagogically detail the mapping to a field theory for the single-species reaction k A -> l A (l < k). We employ this particularly simple but non-trivial system to introduce the field-theoretic RG tools, including the diagrammatic perturbation expansion, renormalization, and Callan-Symanzik RG flow equation. We demonstrate how these techniques permit the calculation of universal quantities such as density decay exponents and amplitudes via perturbative eps = d_c - d expansions with respect to the upper critical dimension d_c. With these basics established, we then provide an overview of more sophisticated applications to multiple species reactions, disorder effects, L'evy flights, persistence problems, and the influence of spatial boundaries. We also analyze field-theoretic approaches to nonequilibrium phase transitions separating active from absorbing states. We focus particularly on the generic directed percolation universality class, as well as on the most prominent exception to this class: even-offspring branching and annihilating random walks. Finally, we summarize the state of the field and present our perspective on outstanding problems for the future.Comment: 10 figures include

    Brokered Graph State Quantum Computing

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    We describe a procedure for graph state quantum computing that is tailored to fully exploit the physics of optically active multi-level systems. Leveraging ideas from the literature on distributed computation together with the recent work on probabilistic cluster state synthesis, our model assigns to each physical system two logical qubits: the broker and the client. Groups of brokers negotiate new graph state fragments via a probabilistic optical protocol. Completed fragments are mapped from broker to clients via a simple state transition and measurement. The clients, whose role is to store the nascent graph state long term, remain entirely insulated from failures during the brokerage. We describe an implementation in terms of NV-centres in diamond, where brokers and clients are very naturally embodied as electron and nuclear spins.Comment: 5 pages, 3 figure

    Second-order rotational effects on the r-modes of neutron stars

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    Techniques are developed here for evaluating the r-modes of rotating neutron stars through second order in the angular velocity of the star. Second-order corrections to the frequencies and eigenfunctions for these modes are evaluated for neutron star models. The second-order eigenfunctions for these modes are determined here by solving an unusual inhomogeneous hyperbolic boundary-value problem. The numerical techniques developed to solve this unusual problem are somewhat non-standard and may well be of interest beyond the particular application here. The bulk-viscosity coupling to the r-modes, which appears first at second order, is evaluated. The bulk-viscosity timescales are found here to be longer than previous estimates for normal neutron stars, but shorter than previous estimates for strange stars. These new timescales do not substantially affect the current picture of the gravitational radiation driven instability of the r-modes either for neutron stars or for strange stars.Comment: 13 pages, 5 figures, revte

    Cosmic-ray strangelets in the Earth's atmosphere

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    If strange quark matter is stable in small lumps, we expect to find such lumps, called ``strangelets'', on Earth due to a steady flux in cosmic rays. Following recent astrophysical models, we predict the strangelet flux at the top of the atmosphere, and trace the strangelets' behavior in atmospheric chemistry and circulation. We show that several strangelet species may have large abundances in the atmosphere; that they should respond favorably to laboratory-scale preconcentration techniques; and that they present promising targets for mass spectroscopy experiments.Comment: 28 pages, 4 figures, revtex

    Anisotropic Coarsening: Grain Shapes and Nonuniversal Persistence

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    We solve a coarsening system with small but arbitrary anisotropic surface tension and interface mobility. The resulting size-dependent growth shapes are significantly different from equilibrium microcrystallites, and have a distribution of grain sizes different from isotropic theories. As an application of our results, we show that the persistence decay exponent depends on anisotropy and hence is nonuniversal.Comment: 4 pages (revtex), 2 eps figure

    Model of the Quark Mixing Matrix

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    The structure of the Cabibbo-Kobayashi-Maskawa (CKM) matrix is analyzed from the standpoint of a composite model. A model is constructed with three families of quarks, by taking tensor products of sufficient numbers of spin-1/2 representations and imagining the dominant terms in the mass matrix to arise from spin-spin interactions. Generic results then obtained include the familiar relation ∣Vus∣=(md/ms)1/2−(mu/mc)1/2|V_{us}| = (m_d/m_s)^{1/2} - (m_u/m_c)^{1/2}, and a less frequently seen relation ∣Vcb∣=2[(ms/mb)−(mc/mt)]|V_{cb}| = \sqrt{2} [(m_s/m_b) - (m_c/m_t)]. The magnitudes of VubV_{ub} and VtdV_{td} come out naturally to be of the right order. The phase in the CKM matrix can be put in by hand, but its origin remains obscure.Comment: Presented by Mihir P. Worah at DPF 92 Meeting, Fermilab, November, 1992. 3 pages, LaTeX fil

    Transgenic expression of the dicotyledonous pattern recognition receptor EFR in rice leads to ligand-dependent activation of defense responses

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    Plant plasma membrane localized pattern recognition receptors (PRRs) detect extracellular pathogen-associated molecules. PRRs such as Arabidopsis EFR and rice XA21 are taxonomically restricted and are absent from most plant genomes. Here we show that rice plants expressing EFR or the chimeric receptor EFR::XA21, containing the EFR ectodomain and the XA21 intracellular domain, sense both Escherichia coli- and Xanthomonas oryzae pv. oryzae (Xoo)-derived elf18 peptides at sub-nanomolar concentrations. Treatment of EFR and EFR::XA21 rice leaf tissue with elf18 leads to MAP kinase activation, reactive oxygen production and defense gene expression. Although expression of EFR does not lead to robust enhanced resistance to fully virulent Xoo isolates, it does lead to quantitatively enhanced resistance to weakly virulent Xoo isolates. EFR interacts with OsSERK2 and the XA21 binding protein 24 (XB24), two key components of the rice XA21-mediated immune response. Rice-EFR plants silenced for OsSERK2, or overexpressing rice XB24 are compromised in elf18-induced reactive oxygen production and defense gene expression indicating that these proteins are also important for EFR-mediated signaling in transgenic rice. Taken together, our results demonstrate the potential feasibility of enhancing disease resistance in rice and possibly other monocotyledonous crop species by expression of dicotyledonous PRRs. Our results also suggest that Arabidopsis EFR utilizes at least a subset of the known endogenous rice XA21 signaling components
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