26,654 research outputs found

    Infrared absorption and Raman scattering on coupled plasmon--phonon modes in superlattices

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    We consider theoretically a superlattice formed by thin conducting layers separated spatially between insulating layers. The dispersion of two coupled phonon-plasmon modes of the system is analyzed by using Maxwell's equations, with the influence of retardation included. Both transmission for the finite plate as well as absorption for the semi-infinite superlattice in the infrared are calculated. Reflectance minima are determined by the longitudinal and transverse phonon frequencies in the insulating layers and by the density-state singularities of the coupled modes. We evaluate also the Raman cross section from the semi-infinite superlattice.Comment: 20 pages,14 figure

    Complete homochirality induced by the nonlinear autocatalysis and recycling

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    A nonlinear autocatalysis of a chiral substance is shown to achieve homochirality in a closed system, if the back-reaction is included. Asymmetry in the concentration of two enantiomers or the enantiometric excess increases due to the nonlinear autocatalysis. Furthermore, when the back-reaction is taken into account, the reactant supplied by the decomposition of the enantiomers is recycled to produce more and more the dominant one, and eventually the homochirality is established.Comment: 4 pages, 2 figure

    Attosecond screening dynamics mediated by electron-localization

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    Transition metals with their densely confined and strongly coupled valence electrons are key constituents of many materials with unconventional properties, such as high-Tc superconductors, Mott insulators and transition-metal dichalcogenides. Strong electron interaction offers a fast and efficient lever to manipulate their properties with light, creating promising potential for next-generation electronics. However, the underlying dynamics is a fast and intricate interplay of polarization and screening effects, which is poorly understood. It is hidden below the femtosecond timescale of electronic thermalization, which follows the light-induced excitation. Here, we investigate the many-body electron dynamics in transition metals before thermalization sets in. We combine the sensitivity of intra-shell transitions to screening effects with attosecond time resolution to uncover the interplay of photo-absorption and screening. First-principles time-dependent calculations allow us to assign our experimental observations to ultrafast electronic localization on d-orbitals. The latter modifies the whole electronic structure as well as the collective dynamic response of the system on a timescale much faster than the light-field cycle. Our results demonstrate a possibility for steering the electronic properties of solids prior to electron thermalization, suggesting that the ultimate speed of electronic phase transitions is limited only by the duration of the controlling laser pulse. Furthermore, external control of the local electronic density serves as a fine tool for testing state-of-the art models of electron-electron interactions. We anticipate our study to facilitate further investigations of electronic phase transitions, laser-metal interactions and photo-absorption in correlated electron systems on its natural timescale

    Phase statistics of seismic coda waves

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    We report the analysis of the statistics of the phase fluctuations in the coda of earthquakes recorded during a temporary experiment deployed at Pinyon Flats Observatory, California. The practical measurement of the phase is discussed and the main pitfalls are underlined. For large values, the experimental distributions of the phase first, second and third derivatives obey universal power-law decays whose exponents are remarkably well predicted by circular Gaussian statistics. For small values, these distributions are flat. The details of the transition between the plateau and the power-law behavior are governed by the wavelength. The correlation function of the first phase derivative along the array shows a simple algebro-exponential decay with the mean free path as the only length scale. Although only loose bounds are provided in this study, our work suggests a new method to estimate the degree of heterogeneity of the crComment: 4 figures, submitted to Physical Review Letter

    Four-spin-exchange- and magnetic-field-induced chiral order in two-leg spin ladders

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    We propose a mechanism of a vector chiral long-range order in two-leg spin-1/2 and spin-1 antiferromagnetic ladders with four-spin exchanges and a Zeeman term. It is known that for one-dimensional quantum systems, spontaneous breakdown of continuous symmetries is generally forbidden. Any vector chiral order hence does not appear in spin-rotationally [SU(2)]-symmetric spin ladders. However, if a magnetic field is added along the S^z axis of ladders and the SU(2) symmetry is reduced to the U(1) one, the z component of a vector chiral order can emerge with the remaining U(1) symmetry unbroken. Making use of Abelian bosonization techniques, we actually show that a certain type of four-spin exchange can yield a vector chiral long-range order in spin-1/2 and spin-1 ladders under a magnetic field. In the chiral-ordered phase, the Z_2 interchain-parity (i.e., chain-exchange) symmetry is spontaneously broken. We also consider effects of perturbations breaking the parity symmetry.Comment: 8 pages, 1 figure, RevTex, published versio

    Implication of Omega_m through the Morphological Analysis of Weak Lensing Fields

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    We apply the morphological descriptions of two-dimensional contour map, the so-called Minkowski functionals (the area fraction, circumference, and Euler characteristics), to the convergence field Îș(Ξ)\kappa(\bm{\theta}) of the large-scale structure reconstructed from the shear map produced by the ray-tracing simulations. The perturbation theory of structure formation has suggested that the non-Gaussian features on the Minkowski functionals with respect to the threshold in the weakly nonlinear regime are induced by the three skewness parameters of Îș\kappa that are sensitive to the density parameter of matter, Ωm\Omega_{\rm m}. We show that, in the absence of noise due to the intrinsic ellipticities of source galaxies with which the perturbation theory results can be recovered, the accuracy of Ωm\Omega_{\rm m} determination is improved by ∌20\sim 20% using the Minkowski functionals compared to the conventional method of using the direct measure of skewness.Comment: 4 pages, 3 figures, to appear in ApJ Lette
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