421 research outputs found
Spectroscopic Evidence for the Localization of Skyrmions near Nu=1 as T->0
Optically pumped nuclear magnetic resonance measurements of Ga-71 spectra
were carried out in an n-doped GaAs/Al0.1Ga0.9As multiple quantum well sample
near the integer quantum Hall ground state Nu=1. As the temperature is lowered
(down to T~0.3 K), a ``tilted plateau'' emerges in the Knight shift data, which
is a novel experimental signature of quasiparticle localization. The dependence
of the spectra on both T and Nu suggests that the localization is a collective
process. The frozen limit spectra appear to rule out a 2D lattice of
conventional skyrmions.Comment: 4 pages (REVTEX), 5 eps figures embedded in text, published versio
Observation of a new phase transition between fully and partially polarized quantum Hall states with charge and spin gaps at
The average electron spin-polarization of two-dimensional electron
gas confined in multiple quantum-wells was measured by
nuclear magnetic resonance (NMR) near the fractional quantum Hall state with
filling factor . Above this filling factor (), a strong depolarization is observed corresponding to two spin flips per
additional flux quantum. The most remarkable behavior of the polarization is
observed at , where a quantum phase transition from a partially
polarized () to a fully polarized ()
state can be driven by increasing the ratio between the Zeeman and the Coulomb
energy above a critical value .Comment: 4 pages including 4 figure
Skyrmion Dynamics and NMR Line Shapes in QHE Ferromagnets
The low energy charged excitations in quantum Hall ferromagnets are
topological defects in the spin orientation known as skyrmions. Recent
experimental studies on nuclear magnetic resonance spectral line shapes in
quantum well heterostructures show a transition from a motionally narrowed to a
broader `frozen' line shape as the temperature is lowered at fixed filling
factor. We present a skyrmion diffusion model that describes the experimental
observations qualitatively and shows a time scale of for
the transport relaxation time of the skyrmions. The transition is characterized
by an intermediate time regime that we demonstrate is weakly sensitive to the
dynamics of the charged spin texture excitations and the sub-band electronic
wave functions within our model. We also show that the spectral line shape is
very sensitive to the nuclear polarization profile along the z-axis obtained
through the optical pumping technique.Comment: 6 pages, 4 figure
Tunneling into Ferromagnetic Quantum Hall States: Observation of a Spin Bottleneck
We explore the characteristics of equilibrium tunneling of electrons from a
3D electrode into a high mobility 2D electron system. For most 2D Landau level
filling factors, we find that tunneling can be characterized by a single,
well-defined tunneling rate. However, for spin-polarized quantum Hall states
(nu = 1, 3 and 1/3) tunneling occurs at two distinct rates that differ by up to
2 orders of magnitude. The dependence of the two rates on temperature and
tunnel barrier thickness suggests that slow in-plane spin relaxation creates a
bottleneck for tunneling of electrons.Comment: 5 pages, 4 figures, submitted to PR
Optically Pumped NMR Measurements of the Electron Spin Polarization in GaAs Quantum Wells near Landau Level Filling Factor nu=1/3
The Knight shift of Ga-71 nuclei is measured in two different electron-doped
multiple quantum well samples using optically pumped NMR. These data are the
first direct measurements of the electron spin polarization,
P(nu,T)=/max, near nu=1/3. The P(T) data at nu=1/3 probe the
neutral spin-flip excitations of a fractional quantum Hall ferromagnet. In
addition, the saturated P(nu) drops on either side of nu=1/3, even in a Btot=12
Tesla field. The observed depolarization is quite small, consistent with an
average of about 0.1 spin-flips per quasihole (or quasiparticle), a value which
does not appear to be explicable by the current theoretical understanding of
the FQHE near nu=1/3.Comment: 4 pages (REVTEX), 5 eps figures embedded in text; minor changes,
published versio
NMR Determination of 2D Electron Spin Polarization at
Using a `standard' NMR spin-echo technique we determined the spin
polarization of two-dimensional electrons, confined to GaAs quantum wells, from
the hyperfine shift of Ga nuclei in the wells. Concentrating on the temperature
and magnetic field dependencies of spin polarization at Landau level filling
factor , we find that the results are described well by a simple
model of non-interacting composite fermions, although some inconsistencies
remain when the two-dimensional electron system is tilted in the magnetic
field.Comment: 4 pages (REVTEX) AND 4 figures (PS
Dyslexia and password usage:accessibility in authentication design
Governments and businesses are moving online with alacrity, driven by potential cost savings, changing consumer and citizen expectations, and the momentum towards general digital provision. Services are legally required to be inclusive and accessible. Now consider that almost every online service, where people have to identify themselves, requires a password. Passwords seem to be accessible, until one considers specific disabilities, one of which can lead to many challenges: dyslexia being a case in point. Dyslexia is associated with word processing and retention difficulties, and passwords are essentially words, phrases or alphanumeric combinations. We report on a literature review conducted to identify extant research into the impact of dyslexia on password usage, as well as any ameliorations that have been proposed. We discovered a relatively neglected field. We conclude with recommendations for future research into the needs of a large population of dyslexics who seem to struggle with passwords, in a world where avoiding passwords has become almost impossible. The main contribution of this paper is to highlight the difficulties dyslexics face with passwords, and to suggest some avenues for future research in this area
Spintronics: Fundamentals and applications
Spintronics, or spin electronics, involves the study of active control and
manipulation of spin degrees of freedom in solid-state systems. This article
reviews the current status of this subject, including both recent advances and
well-established results. The primary focus is on the basic physical principles
underlying the generation of carrier spin polarization, spin dynamics, and
spin-polarized transport in semiconductors and metals. Spin transport differs
from charge transport in that spin is a nonconserved quantity in solids due to
spin-orbit and hyperfine coupling. The authors discuss in detail spin
decoherence mechanisms in metals and semiconductors. Various theories of spin
injection and spin-polarized transport are applied to hybrid structures
relevant to spin-based devices and fundamental studies of materials properties.
Experimental work is reviewed with the emphasis on projected applications, in
which external electric and magnetic fields and illumination by light will be
used to control spin and charge dynamics to create new functionalities not
feasible or ineffective with conventional electronics.Comment: invited review, 36 figures, 900+ references; minor stylistic changes
from the published versio
Cryogenics free production of hyperpolarized 129Xe and 83Kr for biomedical MRI applications
As an alternative to cryogenic gas handling, hyperpolarized (hp) gas mixtures were extracted directly from the spin exchange optical pumping (SEOP) process through expansion followed by compression to ambient pressure for biomedical MRI applications. The omission of cryogenic gas separation generally requires the usage of high xenon or krypton concentrations at low SEOP gas pressures to generate hp 129Xe or hp 83Kr with sufficient MR signal intensity for imaging applications. Two different extraction schemes for the hp gasses were explored with focus on the preservation of the nuclear spin polarization. It was found that an extraction scheme based on an inflatable, pressure controlled balloon is sufficient for hp 129Xe handling, while 83Kr can efficiently be extracted through a single cycle piston pump. The extraction methods were tested for ex vivo MRI applications with excised rat lungs. Precise mixing of the hp gases with oxygen, which may be of interest for potential in vivo applications, was accomplished during the extraction process using a piston pump. The 83Kr bulk gas phase T1 relaxation in the mixtures containing more than approximately 1% O2 was found to be slower than that of 129Xe in corresponding mixtures. The experimental setup also facilitated 129Xe T1 relaxation measurements as a function of O2 concentration within excised lungs
Activation and Deactivation of a Robust Immobilized Cp*Ir-Transfer Hydrogenation Catalyst: A Multielement in Situ X-ray Absorption Spectroscopy Study
A highly robust immobilized [Cp*IrCl2]2 precatalyst on Wang resin for transfer hydrogenation, which can be recycled up to 30 times, was studied using a novel combination of X-ray absorption spectroscopy (XAS) at Ir L3-edge, Cl K-edge, and K K-edge. These culminate in in situ XAS experiments that link structural changes of the Ir complex with its catalytic activity and its deactivation. Mercury poisoning and “hot filtration” experiments ruled out leached Ir as the active catalyst. Spectroscopic evidence indicates the exchange of one chloride ligand with an alkoxide to generate the active precatalyst. The exchange of the second chloride ligand, however, leads to a potassium alkoxide–iridate species as the deactivated form of this immobilized catalyst. These findings could be widely applicable to the many homogeneous transfer hydrogenation catalysts with Cp*IrCl substructure
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