18 research outputs found

    The elevated Curie temperature and half-metallicity in the ferromagnetic semiconductor Lax_{x}Eu1−x_{1-x}O

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    Here we study the effect of La doping in EuO thin films using SQUID magnetometry, muon spin rotation (μ\muSR), polarized neutron reflectivity (PNR), and density functional theory (DFT). The μ\muSR data shows that the La0.15_{0.15}Eu0.85_{0.85}O is homogeneously magnetically ordered up to its elevated TCT_{\rm C}. It is concluded that bound magnetic polaron behavior does not explain the increase in TCT_{\rm C} and an RKKY-like interaction is consistent with the μ\muSR data. The estimation of the magnetic moment by DFT simulations concurs with the results obtained by PNR, showing a reduction of the magnetic moment per Lax_{x}Eu1−x_{1-x}O for increasing lanthanum doping. This reduction of the magnetic moment is explained by the reduction of the number of Eu-4ff electrons present in all the magnetic interactions in EuO films. Finally, we show that an upwards shift of the Fermi energy with La or Gd doping gives rise to half-metallicity for doping levels as high as 3.2 %.Comment: 7 pages, 11 figure

    Helical magnetic structure and the anomalous and topological Hall effects in epitaxial B20 Fe1−y_{1-y}Coy_yGe films

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    Epitaxial films of the B20-structure alloy Fe1−y_{1-y}Coy_yGe were grown by molecular beam epitaxy on Si (111) substrates. The magnetization varied smoothly from the bulk-like values of one Bohr magneton per Fe atom for FeGe to zero for non-magnetic CoGe. The chiral lattice structure leads to a Dzyaloshinskii-Moriya interaction (DMI), and the films' helical magnetic ground state was confirmed using polarized neutron reflectometry measurements. The pitch of the spin helix, measured by this method, varies with Co content yy and diverges at y∼0.45y \sim 0.45. This indicates a zero-crossing of the DMI, which we reproduced in calculations using first principle methods. We also measured the longitudinal and Hall resistivity of our films as a function of magnetic field, temperature, and Co content yy. The Hall resistivity is expected to contain contributions from the ordinary, anomalous, and topological Hall effects. Both the anomalous and topological Hall resistivities show peaks around y∼0.5y \sim 0.5. Our first principles calculations show a peak in the topological Hall constant at this value of yy, related to the strong spin-polarisation predicted for intermediate values of yy. Half-metallicity is predicted for y=0.6y = 0.6, consistent with the experimentally observed linear magnetoresistance at this composition. Whilst it is possible to reconcile theory with experiment for the various Hall effects for FeGe, the large topological Hall resistivities for y∼0.5y \sim 0.5 are much larger then expected when the very small emergent fields associated with the divergence in the DMI are taken into account

    An accurate in vitro model of the E. coli envelope

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    Gram-negative bacteria are an increasingly serious source of antibiotic-resistant infections, partly owing to their characteristic protective envelope. This complex, 20 nm thick barrier includes a highly impermeable, asymmetric bilayer outer membrane (OM), which plays a pivotal role in resisting antibacterial chemotherapy. Nevertheless, the OM molecular structure and its dynamics are poorly understood because the structure is difficult to recreate or study in vitro. The successful formation and characterization of a fully asymmetric model envelope using Langmuir-Blodgett and Langmuir-Schaefer methods is now reported. Neutron reflectivity and isotopic labeling confirmed the expected structure and asymmetry and showed that experiments with antibacterial proteins reproduced published in vivo behavior. By closely recreating natural OM behavior, this model provides a much needed robust system for antibiotic development

    Strain dependent selection of spin-slip phases in sputter deposited thin-film epitaxial holmium

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    We report the structural and magnetic characterization of sputter deposited epitaxial Ho. We present room temperature characterization by atomic force microscopy and x-ray diffraction and temperature dependent characterization by x-ray diffraction and neutron diffraction. The data show the onset and change of the magnetic state as a function of temperature. Films of different thickness, exhibiting signs of differing epitaxially induced strain, tend towards specific spin-slip phases in the low temperature regime. The more highly strained thinnest films tend towards values with a longer magnetic wavelength

    Recruitment and Selection of Graduates - A Survey on FHS UK Graduates

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    We present a detailed structural and magnetic characterization of sputter deposited thin film erbium, determined by x-ray diffraction, transport measurements, magnetometry and neutron diffraction. This provides information on the onset and change of the magnetic state as a function of temperature and applied magnetic field. Many of the features of bulk material are reproduced. Also of interest is the identification of a conical magnetic state which repeats with a wavevector parallel to the c axis τc = 4/17 in units of the reciprocal lattice parameter c*, which is a state not observed in any other thin film or bulk measurements. The data from the various techniques are combined to construct magnetic field, temperature (H, T)–phase diagrams for the 200 nm-thick Er sample that serves as a foundation for future exploitation of this complex magnetic thin film system.ISSN:2045-232
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