Penning trap mass measurements on (99-109)$Cd with ISOLTRAP and implications on the rp process

Penning trap mass measurements on neutron-deficient Cd isotopes (99-109)Cd have been performed with the ISOLTRAP mass spectrometer at ISOLDE/CERN, all with relative mass uncertainties below 3*10^8. A new mass evaluation has been performed. The mass of 99Cd has been determined for the first time which extends the region of accurately known mass values towards the doubly magic nucleus 100Sn. The implication of the results on the reaction path of the rp process in stellar X-ray bursts is discussed. In particular, the uncertainty of the abundance and the overproduction created by the rp-process for the mass A = 99 is demonstrated by reducing the uncertainty of the proton-separation energy of 100In Sp(100In) by a factor of 2.5.Comment: 14 pages, 9 figure

Beta decay of 71,73Co; probing single particle states approaching doubly magic 78Ni

Low-energy excited states in 71,73Ni populated via the {\beta} decay of 71,73Co were investigated in an experiment performed at the National Superconducting Cyclotron Laboratory (NSCL) at Michigan State University (MSU). Detailed analysis led to the construction of level schemes of 71,73Ni, which are interpreted using systematics and analyzed using shell model calculations. The 5/2- states attributed to the the f5/2 orbital and positive parity 5/2+ and 7/2+ states from the g9/2 orbital have been identified in both 71,73Ni. In 71Ni the location of a 1/2- {\beta}-decaying isomer is proposed and limits are suggested as to the location of the isomer in 73Ni. The location of positive parity cluster states are also identified in 71,73Ni. Beta-delayed neutron branching ratios obtained from this data are given for both 71,73Co.Comment: Accepted for publication in PR

The rp-process and new measurements of beta-delayed proton decay of light Ag and Cd isotopes

Recent network calculations suggest that a high temperature rp-process could explain the abundances of light Mo and Ru isotopes, which have long challenged models of p-process nuclide production. Important ingredients to network calculations involving unstable nuclei near and at the proton drip line are $\beta$-halflives and decay modes, i.e., whether or not $\beta$-delayed proton decay takes place. Of particular importance to these network calculation are the proton-rich isotopes $^{96}$Ag, $^{98}$Ag, $^{96}$Cd and $^{98}$Cd. We report on recent measurements of $\beta$-delayed proton branching ratios for $^{96}$Ag, $^{98}$Ag, and $^{98}$Cd at the on-line mass separator at GSI.Comment: 4 pages, uses espcrc1.sty. Proceedings of the 4th International Symposium Nuclei in the Cosmos, June 1996, Notre Dame/IN, USA, Ed. M. Wiescher, to be published in Nucl.Phys.A. Also available at ftp://ftp.physics.ohio-state.edu/pub/nucex/nic96-gs

Improving Fission-product Decay Data for Reactor Applications: Part I -- Decay Heat

Effort has been expended to assess the relative merits of undertaking further decay-data measurements of the main fission-product contributors to the decay heat of neutron-irradiated fissile fuel and related actinides by means of Total Absorption Gamma-ray Spectroscopy (TAGS/TAS) and Discrete Gamma-ray Spectroscopy (DGS). This review has been carried out following similar work performed under the auspices of OECD/WPEC-Subgroup 25 (2005-2007) and the International Atomic Energy Agency (2010, 2014), and various highly relevant TAGS measurements completed as a consequence of such assessments. We present our recommendations for new decay-data evaluations, along with possible requirements for total absorption and discrete high-resolution gamma-ray spectroscopy studies that cover approximately 120 fission products and various isomeric states.Comment: Submitted to European Physical Journal

Radioactive decays at limits of nuclear stability

The last decades brought an impressive progress in synthesizing and studying properties of nuclides located very far from the beta stability line. Among the most fundamental properties of such exotic nuclides, usually established first, is the half-life, possible radioactive decay modes, and their relative probabilities. When approaching limits of nuclear stability, new decay modes set in. First, beta decays become accompanied by emission of nucleons from highly excited states of daughter nuclei. Second, when the nucleon separation energy becomes negative, nucleons start to be emitted from the ground state. Here, we present a review of the decay modes occurring close to the limits of stability. The experimental methods used to produce, identify and detect new species and their radiation are discussed. The current theoretical understanding of these decay processes is overviewed. The theoretical description of the most recently discovered and most complex radioactive process - the two-proton radioactivity - is discussed in more detail.Comment: Review, 68 pages, 39 figure

βdecays of \u3csup\u3e92\u3c/sup\u3eRb, \u3csup\u3e96gs\u3c/sup\u3eY, and \u3csup\u3e142\u3c/sup\u3eCs measured with the modular total absorption spectrometer and the influence of multiplicity on total absorption spectrometry measurements

Total absorption spectroscopy is a technique that helps obtain reliable β-feeding patterns of complex decays important for nuclear structure and astrophysics modeling as well as decay heat analysis in nuclear reactors. The need for improved measurements of β-feeding patterns from fission decay products has come to the forefront of experiments that use nuclear reactors as a source of antineutrinos. Here we present more detailed results, in particular the β-decay measurements of 96gsY, and demonstrate the impact of the β-delayed γ multiplicity on the overall efficiency of Modular Total Absorption Spectrometer used at Oak Ridge National Laboratory to study the decays of fission products abundant during a nuclear fuel cycle

Experimental study of the β decay of the very neutron-rich nucleus Ge 85

The β-decay properties of the very neutron-rich nucleus Ge85, produced in the proton-induced fission of U238, were studied at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. The level scheme of As523385 populated in Ge85βγ decay was reconstructed and compared to shell-model calculations. The investigation of the systematics of low-energy levels in N=52 isotones together with shell-model analysis allowed us to provide an estimate of the low-energy structure of the more exotic N=52 isotone Cu81

Impact of Modular Total Absorption Spectrometer measurements of β decay of fission products on the decay heat and reactor ν e flux calculation

We report the results of a β-decay study of fission products Br86, Kr89, Rb89, Rb90gs, Rb90m, Kr90, Rb92, Xe139, and Cs142 performed with the Modular Total Absorption Spectrometer (MTAS) and on-line mass-separated ion beams. These radioactivities were assessed by the Nuclear Energy Agency as having high priority for decay heat analysis during a nuclear fuel cycle. We observe a substantial increase in β feeding to high excited states in all daughter isotopes in comparison to earlier data. This increases the average γ-ray energy emitted by the decay of fission fragments during the first 10 000 s after fission of U235 and Pu239 by approximately 2% and 1%, respectively, improving agreement between results of calculations and direct observations. New MTAS results reduce the reference reactor νe flux used to analyze reactor νe interaction with detector matter. The reduction determined by the ab initio method for the four nuclear fuel components, U235, U238, Pu239, and Pu241, amounts to 0.976, 0.986, 0.983, and 0.984, respectively

β and β-n decay of the neutron-rich Ge 84 nucleus

The β-decay properties of the very neutron-rich Ge84 nucleus were studied at the Holifield Radioactive Ion Beam Facility at Oak Ridge National Laboratory. Several new γ-transitions and levels were added to its decay scheme and the order of the two lowest-lying levels in the daughter As84 was corrected. For the first time γ radiation following β-delayed neutron emission was observed. The shell-model calculations and apparent β transition intensities were used to guide the spin assignment to the As84 levels, in particular for the low-energy part of the level scheme. The new spin-parity (2-) proposed for the ground state of As84 is supported also by the systematics of N=51 isotones