113 research outputs found
A valley-spin qubit in a carbon nanotube
Although electron spins in III-V semiconductor quantum dots have shown great
promise as qubits, a major challenge is the unavoidable hyperfine decoherence
in these materials. In group IV semiconductors, the dominant nuclear species
are spinless, allowing for qubit coherence times that have been extended up to
seconds in diamond and silicon. Carbon nanotubes are a particularly attractive
host material, because the spin-orbit interaction with the valley degree of
freedom allows for electrical manipulation of the qubit. In this work, we
realise such a qubit in a nanotube double quantum dot. The qubit is encoded in
two valley-spin states, with coherent manipulation via electrically driven spin
resonance (EDSR) mediated by a bend in the nanotube. Readout is performed by
measuring the current in Pauli blockade. Arbitrary qubit rotations are
demonstrated, and the coherence time is measured via Hahn echo. Although the
measured decoherence time is only 65 ns in our current device, this work offers
the possibility of creating a qubit for which hyperfine interaction can be
virtually eliminated
Coupling molecular spin states by photon-assisted tunneling
Artificial molecules containing just one or two electrons provide a powerful
platform for studies of orbital and spin quantum dynamics in nanoscale devices.
A well-known example of these dynamics is tunneling of electrons between two
coupled quantum dots triggered by microwave irradiation. So far, these
tunneling processes have been treated as electric dipole-allowed
spin-conserving events. Here we report that microwaves can also excite
tunneling transitions between states with different spin. In this work, the
dominant mechanism responsible for violation of spin conservation is the
spin-orbit interaction. These transitions make it possible to perform detailed
microwave spectroscopy of the molecular spin states of an artificial hydrogen
molecule and open up the possibility of realizing full quantum control of a two
spin system via microwave excitation.Comment: 13 pages, 9 figure
Tunable few-electron double quantum dots and Klein tunnelling in ultra-clean carbon nanotubes
Quantum dots defined in carbon nanotubes are a platform for both basic
scientific studies and research into new device applications. In particular,
they have unique properties that make them attractive for studying the coherent
properties of single electron spins. To perform such experiments it is
necessary to confine a single electron in a quantum dot with highly tunable
barriers, but disorder has until now prevented tunable nanotube-based
quantum-dot devices from reaching the single-electron regime. Here, we use
local gate voltages applied to an ultra-clean suspended nanotube to confine a
single electron in both a single quantum dot and, for the first time, in a
tunable double quantum dot. This tunability is limited by a novel type of
tunnelling that is analogous to that in the Klein paradox of relativistic
quantum mechanics.Comment: 21 pages including supplementary informatio
Electron cotunneling through doubly occupied quantum dots: effect of spin configuration
A microscopic theory is presented for electron cotunneling through doubly occupied quantum dots in the Coulomb blockade regime. Beyond the semiclassic framework of phenomenological models, a fully quantum mechanical solution for cotunneling of electrons through a one-dimensional quantum dot is obtained using a quantum transmitting boundary method without any fitting parameters. It is revealed that the cotunneling conductance exhibits strong dependence on the spin configuration of the electrons confined inside the dot. Especially for the triplet configuration, the conductance shows an obvious deviation from the well-known quadratic dependence on the applied bias voltage. Furthermore, it is found that the cotunneling conductance reveals more sensitive dependence on the barrier width than the height
Valley-spin blockade and spin resonance in carbon nanotubes
Manipulation and readout of spin qubits in quantum dots made in III-V
materials successfully rely on Pauli blockade that forbids transitions between
spin-triplet and spin-singlet states. Quantum dots in group IV materials have
the advantage of avoiding decoherence from the hyperfine interaction by
purifying them with only zero-spin nuclei. Complications of group IV materials
arise from the valley degeneracies in the electronic bandstructure. These lead
to complicated multiplet states even for two-electron quantum dots thereby
significantly weakening the selection rules for Pauli blockade. Only recently
have spin qubits been realized in silicon devices where the valley degeneracy
is lifted by strain and spatial confinement. In carbon nanotubes Pauli blockade
can be observed by lifting valley degeneracy through disorder. In clean
nanotubes, quantum dots have to be made ultra-small to obtain a large energy
difference between the relevant multiplet states. Here we report on
low-disorder nanotubes and demonstrate Pauli blockade based on both valley and
spin selection rules. We exploit the bandgap of the nanotube to obtain a large
level spacing and thereby a robust blockade. Single-electron spin resonance is
detected using the blockade.Comment: 31 pages including supplementary informatio
Electrically driven single electron spin resonance in a slanting Zeeman field
The rapidly rising fields of spintronics and quantum information science have
led to a strong interest in developing the ability to coherently manipulate
electron spins. Electron spin resonance (ESR) is a powerful technique to
manipulate spins that is commonly achieved by applying an oscillating magnetic
field. However, the technique has proven very challenging when addressing
individual spins. In contrast, by mixing the spin and charge degrees of freedom
in a controlled way through engineered non-uniform magnetic fields, electron
spin can be manipulated electrically without the need of high-frequency
magnetic fields. Here we realize electrically-driven addressable spin rotations
on two individual electrons by integrating a micron-size ferromagnet to a
double quantum dot device. We find that the electrical control and spin
selectivity is enabled by the micro-magnet's stray magnetic field which can be
tailored to multi-dots architecture. Our results demonstrate the feasibility of
manipulating electron spins electrically in a scalable way.Comment: 25 pages, 6 figure
Nanoscale spin rectifiers controlled by the Stark effect
The control of orbital and spin state of single electrons is a key ingredient
for quantum information processing, novel detection schemes, and, more
generally, is of much relevance for spintronics. Coulomb and spin blockade (SB)
in double quantum dots (DQDs) enable advanced single-spin operations that would
be available even for room-temperature applications for sufficiently small
devices. To date, however, spin operations in DQDs were observed at sub-Kelvin
temperatures, a key reason being that scaling a DQD system while retaining an
independent field-effect control on the individual dots is very challenging.
Here we show that quantum-confined Stark effect allows an independent
addressing of two dots only 5 nm apart with no need for aligned nanometer-size
local gating. We thus demonstrate a scalable method to fully control a DQD
device, regardless of its physical size. In the present implementation we show
InAs/InP nanowire (NW) DQDs that display an experimentally detectable SB up to
10 K. We also report and discuss an unexpected re-entrant SB lifting as a
function magnetic-field intensity
An addressable quantum dot qubit with fault-tolerant control fidelity
Exciting progress towards spin-based quantum computing has recently been made
with qubits realized using nitrogen-vacancy (N-V) centers in diamond and
phosphorus atoms in silicon, including the demonstration of long coherence
times made possible by the presence of spin-free isotopes of carbon and
silicon. However, despite promising single-atom nanotechnologies, there remain
substantial challenges in coupling such qubits and addressing them
individually. Conversely, lithographically defined quantum dots have an
exchange coupling that can be precisely engineered, but strong coupling to
noise has severely limited their dephasing times and control fidelities. Here
we combine the best aspects of both spin qubit schemes and demonstrate a
gate-addressable quantum dot qubit in isotopically engineered silicon with a
control fidelity of 99.6%, obtained via Clifford based randomized benchmarking
and consistent with that required for fault-tolerant quantum computing. This
qubit has orders of magnitude improved coherence times compared with other
quantum dot qubits, with T_2* = 120 mus and T_2 = 28 ms. By gate-voltage tuning
of the electron g*-factor, we can Stark shift the electron spin resonance (ESR)
frequency by more than 3000 times the 2.4 kHz ESR linewidth, providing a direct
path to large-scale arrays of addressable high-fidelity qubits that are
compatible with existing manufacturing technologies
One-dimensional Topological Edge States of Bismuth Bilayers
The hallmark of a time-reversal symmetry protected topologically insulating
state of matter in two-dimensions (2D) is the existence of chiral edge modes
propagating along the perimeter of the system. To date, evidence for such
electronic modes has come from experiments on semiconducting heterostructures
in the topological phase which showed approximately quantized values of the
overall conductance as well as edge-dominated current flow. However, there have
not been any spectroscopic measurements to demonstrate the one-dimensional (1D)
nature of the edge modes. Among the first systems predicted to be a 2D
topological insulator are bilayers of bismuth (Bi) and there have been recent
experimental indications of possible topological boundary states at their
edges. However, the experiments on such bilayers suffered from irregular
structure of their edges or the coupling of the edge states to substrate's bulk
states. Here we report scanning tunneling microscopy (STM) experiments which
show that a subset of the predicted Bi-bilayers' edge states are decoupled from
states of Bi substrate and provide direct spectroscopic evidence of their 1D
nature. Moreover, by visualizing the quantum interference of edge mode
quasi-particles in confined geometries, we demonstrate their remarkable
coherent propagation along the edge with scattering properties that are
consistent with strong suppression of backscattering as predicted for the
propagating topological edge states.Comment: 15 pages, 5 figures, and supplementary materia
Pumped double quantum dot with spin-orbit coupling
We study driven by an external electric field quantum orbital and spin dynamics of electron in a one-dimensional double quantum dot with spin-orbit coupling. Two types of external perturbation are considered: a periodic field at the Zeeman frequency and a single half-period pulse. Spin-orbit coupling leads to a nontrivial evolution in the spin and orbital channels and to a strongly spin- dependent probability density distribution. Both the interdot tunneling and the driven motion contribute into the spin evolution. These results can be important for the design of the spin manipulation schemes in semiconductor nanostructures
- âŚ