Spin-parities of sub-threshold resonances in the 18^{18}F(p, α\alpha)15^{15}O reaction

The $^{18}$F(p, $\alpha$)$^{15}$O reaction is key to determining the $^{18}$F abundance in classical novae. However, the cross section for this reaction has large uncertainties at low energies largely caused by interference effects. Here, we resolve a longstanding issue with unknown spin-parities of sub-threshold states in $^{19}$Ne that reduces these uncertainties. The $^{20}$Ne($^3$He, $^4$He)$^{19}$Ne neutron pick-up reaction was used to populate $^{19}$Ne excited states, focusing on the energy region of astrophysical interest ($\approx$ 6 - 7 MeV). The experiment was performed at the Triangle Universities Nuclear Laboratory using the high resolution Enge split-pole magnetic spectrograph. Spins and parities were found for states in the astrophysical energy range. In particular, the state at 6.133 MeV (E$_{r}^{\text{c.m.}} = -278$ keV) was found to have spin and parity of $3/2^+$ and we confirm the existence of an unresolved doublet close to 6.288 MeV (E$_{r}^{\text{c.m.}} = -120$ keV) with J$^{\pi}$ = $1/2^+$ and a high-spin state. Using these results, we demonstrate a significant factor of two decrease in the reaction rate uncertainties at nova temperatures.Comment: 15 pages, 6 figures, accepted in Phys. Rev. C. Corrected typos and reference

Study of the 25Mg(d,p)26Mg reaction to constrain the 25Al(p,γ )26Si resonant reaction rates in nova burning conditions

The rate of the $$^{25}$$Al(p, $$\gamma$$)$$^{26}$$Si reaction is one of the few key remaining nuclear uncertainties required for predicting the production of the cosmic $$\gamma$$-ray emitter $$^{26}$$Al in explosive burning in novae. This reaction rate is dominated by three key resonances ($$J^{\pi }=0^{+}$$, $$1^{+}$$ and $$3^{+}$$) in $$^{26}$$Si. Only the $$3^{+}$$ resonance strength has been directly constrained by experiment. A high resolution measurement of the $$^{25}$$Mg(d, p) reaction was used to determine spectroscopic factors for analog states in the mirror nucleus, $$^{26}$$Mg. A first spectroscopic factor value is reported for the $$0^{+}$$ state at 6.256 MeV, and a strict upper limit is set on the value for the $$1^{+}$$ state at 5.691 MeV, that is incompatible with an earlier ($$^{4}$$He, $$^{3}$$He) study. These results are used to estimate proton partial widths, and resonance strengths of analog states in $$^{26}$$Si contributing to the $$^{25}$$Al(p, $$\gamma$$)$$^{26}$$Si reaction rate in nova burning conditions

Production of 26Al in stellar hydrogen-burning environments: spectroscopic properties of states in 27Si

Model predictions of the amount of the radioisotope 26Al produced in hydrogen-burning environments require reliable estimates of the thermonuclear rates for the 26gAl(p,{\gamma})27Si and 26mAl(p,{\gamma})27Si reactions. These rates depend upon the spectroscopic properties of states in 27Si within about 1 MeV of the 26gAl+p threshold (Sp = 7463 keV). We have studied the 28Si(3He,{\alpha})27Si reaction at 25 MeV using a high-resolution quadrupole-dipole-dipole-dipole magnetic spectrograph. For the first time with a transfer reaction, we have constrained J{\pi} values for states in 27Si over Ex = 7.0 - 8.1 MeV through angular distribution measurements. Aside from a few important cases, we generally confirm the energies and spin-parity assignments reported in a recent {\gamma}-ray spectroscopy study. The magnitudes of neutron spectroscopic factors determined from shell-model calculations are in reasonable agreement with our experimental values extracted using this reaction.Comment: accepted for publication in Phys. Rev.

Spin-parities of sub-threshold resonances in the 18^{18}F(p, αα)15^{15}O reaction

The $^{18}$F(p, $\alpha$)$^{15}$O reaction is key to determining the $^{18}$F abundance in classical novae. However, the cross section for this reaction has large uncertainties at low energies largely caused by interference effects. Here, we resolve a longstanding issue with unknown spin-parities of sub-threshold states in $^{19}$Ne that reduces these uncertainties. The $^{20}$Ne($^3$He, $^4$He)$^{19}$Ne neutron pick-up reaction was used to populate $^{19}$Ne excited states, focusing on the energy region of astrophysical interest ($\approx$ 6 - 7 MeV). The experiment was performed at the Triangle Universities Nuclear Laboratory using the high resolution Enge split-pole magnetic spectrograph. Spins and parities were found for states in the astrophysical energy range. In particular, the state at 6.133 MeV (E$_{r}^{\text{c.m.}} = -278$ keV) was found to have spin and parity of $3/2^+$ and we confirm the existence of an unresolved doublet close to 6.288 MeV (E$_{r}^{\text{c.m.}} = -120$ keV) with J$^{\pi}$ = $1/2^+$ and a high-spin state. Using these results, we demonstrate a significant factor of two decrease in the reaction rate uncertainties at nova temperatures

Structure of S30 with S32(p,t)S30 and the thermonuclear P29(p,γ)S30 reaction rate

The structure of proton unbound S30 states is important for determining the P29(p,γ)S30 reaction rate, which influences explosive hydrogen burning in classical novae and type I x-ray bursts. The reaction rate in this temperature regime had been previously predicted to be dominated by two low-lying, unobserved, Jπ= 3+ and 2+ resonances above the proton threshold in S30. To search for these levels, the structure of S30 was studied using the S32(p,t)S30 transfer reaction with a magnetic spectrograph. We have confirmed a previous detection of a state near 4700 keV, which had tentatively been assigned Jπ=3+. We have also discovered a new state at 4814(3) keV, which is a strong candidate for the other important resonance (Jπ=2+). The new P29(p,γ)S30 reaction rate is up to 4-20 times larger than previously determined rates over the relevant temperature range. The uncertainty in the reaction rate due to uncertainties in the resonance energies has been significantly reduced. © 2010 The American Physical Society

Nuclear structure of 30S and its implications for nucleosynthesis in classical novae

The uncertainty in the 29P(p,gamma)30S reaction rate over the temperature range of 0.1 - 1.3 GK was previously determined to span ~4 orders of magnitude due to the uncertain location of two previously unobserved 3+ and 2+ resonances in the 4.7 - 4.8 MeV excitation region in 30S. Therefore, the abundances of silicon isotopes synthesized in novae, which are relevant for the identification of presolar grains of putative nova origin, were uncertain by a factor of 3. To investigate the level structure of 30S above the proton threshold (4394.9(7) keV), a charged-particle spectroscopy and an in-beam gamma-ray spectroscopy experiments were performed. Differential cross sections of the 32S(p,t)30S reaction were measured at 34.5 MeV. Distorted wave Born approximation calculations were performed to constrain the spin-parity assignments of the observed levels. An energy level scheme was deduced from gamma-gamma coincidence measurements using the 28Si(3He,n-gamma)30S reaction. Spin-parity assignments based on measurements of gamma-ray angular distributions and gamma-gamma directional correlation from oriented nuclei were made for most of the observed levels of 30S. As a result, the resonance energies corresponding to the excited states in 4.5 MeV - 6 MeV region, including the two astrophysically important states predicted previously, are measured with significantly better precision than before. The uncertainty in the rate of the 29P(p,gamma)30S reaction is substantially reduced over the temperature range of interest. Finally, the influence of this rate on the abundance ratios of silicon isotopes synthesized in novae are obtained via 1D hydrodynamic nova simulations.Comment: 22 pages, 12 figure

Experimental investigation of the 30S(α, p) thermonuclear reaction in x-ray bursts

We performed the first measurement of 30 S+α resonant elastic scattering to experimentally examine the 30 S(α, p) stellar reaction rate in type I x-ray bursts. These bursts are the most frequent thermonuclear explosions in the galaxy, resulting from thermonuclear runaway on the surface of accreting neutron star binaries. The 30 S(α, p) reaction plays a critical role in burst models, yet very little is known about the compound nucleus 34 Ar at these energies nor the reaction rate itself. We performed a measurement of alpha elastic scattering with a radioactive beam of 30 S to experimentally probe the entrance channel. Utilizing a gaseous active target system and silicon detector array, we extracted the excitation function from 1.8 to 5.5 MeV near 160° in the center-of-mass frame. The experimental data were analyzed with an R -Matrix calculation, and we discovered several new resonances and extracted their quantum properties (resonance energy, width, spin, and parity). Finally, we calculated the narrow resonant thermonuclear reaction rate of 30 S(α, p) for these new resonances

Constraining nova observables: direct measurements of resonance strengths in 33S(p,\gamma)34Cl

The 33S(p,\gamma)34Cl reaction is important for constraining predictions of certain isotopic abundances in oxygen-neon novae. Models currently predict as much as 150 times the solar abundance of 33S in oxygen-neon nova ejecta. This overproduction factor may, however, vary by orders of magnitude due to uncertainties in the 33S(p,\gamma)34Cl reaction rate at nova peak temperatures. Depending on this rate, 33S could potentially be used as a diagnostic tool for classifying certain types of presolar grains. Better knowledge of the 33S(p,\gamma)34Cl rate would also aid in interpreting nova observations over the S-Ca mass region and contribute to the firm establishment of the maximum endpoint of nova nucleosynthesis. Additionally, the total S elemental abundance which is affected by this reaction has been proposed as a thermometer to study the peak temperatures of novae. Previously, the 33S(p,\gamma)34Cl reaction rate had only been studied directly down to resonance energies of 432 keV. However, for nova peak temperatures of 0.2-0.4 GK there are 7 known states in 34Cl both below the 432 keV resonance and within the Gamow window that could play a dominant role. Direct measurements of the resonance strengths of these states were performed using the DRAGON recoil separator at TRIUMF. Additionally two new states within this energy region are reported. Several hydrodynamic simulations have been performed, using all available experimental information for the 33S(p,\gamma)34Cl rate, to explore the impact of the remaining uncertainty in this rate on nucleosynthesis in nova explosions. These calculations give a range of ~ 20-150 for the expected 33S overproduction factor, and a range of ~ 100-450 for the 32S/33S ratio expected in ONe novae.Comment: 12 pages, 8 figures, Accepted for publication in Physical Review

Photon shot-noise limited transient absorption soft X-ray spectroscopy at the European XFEL

Femtosecond transient soft X-ray Absorption Spectroscopy (XAS) is a very promising technique that can be employed at X-ray Free Electron Lasers (FELs) to investigate out-of-equilibrium dynamics for material and energy research. Here we present a dedicated setup for soft X-rays available at the Spectroscopy & Coherent Scattering (SCS) instrument at the European X-ray Free Electron Laser (EuXFEL). It consists of a beam-splitting off-axis zone plate (BOZ) used in transmission to create three copies of the incoming beam, which are used to measure the transmitted intensity through the excited and unexcited sample, as well as to monitor the incoming intensity. Since these three intensity signals are detected shot-by-shot and simultaneously, this setup allows normalized shot-by-shot analysis of the transmission. For photon detection, the DSSC imaging detector, which is capable of recording up to 800 images at 4.5 MHz frame rate during the FEL burst, is employed and allows approaching the photon shot-noise limit. We review the setup and its capabilities, as well as the online and offline analysis tools provided to users