R&D progress on second-generation crystals for Laue lens applications

The concept of a gamma-ray telescope based on a Laue lens offers the possibility to increase the sensitivity by more than an order of magnitude with respect to existing instruments. Laue lenses have been developed by our collaboration for several years : the main achievement of this R&D program was the CLAIRE lens prototype. Since then, the endeavour has been oriented towards the development of efficient diffracting elements (crystal slabs), the aim being to step from a technological Laue lens to a scientifically exploitable lens. The latest mission concept featuring a gamma-ray lens is the European Gamma-Ray Imager (GRI) which intends to make use of the Laue lens to cover energies from 200 keV to 1300 keV. Investigations of two promising materials, low mosaicity copper and gradient concentration silicon-germanium are presented in this paper. The measurements have been performed during three runs on beamline ID15A of the European Synchrotron Radiation Facility, and on the GAMS 4 instrument of the Institute Laue-Langevin (both in Grenoble, France) using highly monochromatic beam of energy close to 500 keV. Despite it was not perfectly homogeneous, the presented copper crystal exhibits peak reflectivity of 25% in accordance with theoretical predictions, and a mosaicity around 26 arcsec, the ideal range for the realization of a Laue lens such as GRI. Silicon-germanium featuring a constant gradient have been measured for the very first time at 500 keV. Two samples showed a quite homogeneous reflectivity reaching 26%, which is far from the 48% already observed in experimental crystals but a very encouraging beginning. This results have been used to estimate the performance of the GRI Laue lens design

Contrasting properties of particle-particle and hole-hole excitations in 206Tl and 210Bi nuclei

A complete-spectroscopy investigation of low-lying, low-spin states in the one-proton-hole and one-neutron-hole nucleus 206Tl has been performed by using thermal neutron capture and \u3b3-coincidence technique with the FIPPS Ge array at ILL Grenoble. The new experimental results, together with data for the one-proton-particle and one-neutron-particle nucleus 210Bi (taken from a previous study done at ILL in the EXILL campaign), allowed for an extensive comparison with predictions of shell-model calculations performed with realistic interactions. No phenomenological adjustments were introduced in the calculations. In 210Bi, state energies, transition multipolarities and decay branchings agree well with theory for the three well separated multiplets of states which dominate the low-lying excitations. On the contrary, in 206Tl significant discrepancies are observed: in the same energy region, six multiplets were identified, with a significant mixing among them being predicted, as a consequence of the smaller energy separation between the active orbitals. The discrepancies in 206Tl are attributed to the larger uncertainties in the determination of the off-diagonal matrix elements of the realistic shell-model interaction with respect to the calculated diagonal matrix elements, the only ones playing a major role in the case of 210Bi. The work points to the need of more advanced approaches in the construction of the realistic interactions

The neutron and its role in cosmology and particle physics

Experiments with cold and ultracold neutrons have reached a level of precision such that problems far beyond the scale of the present Standard Model of particle physics become accessible to experimental investigation. Due to the close links between particle physics and cosmology, these studies also permit a deep look into the very first instances of our universe. First addressed in this article, both in theory and experiment, is the problem of baryogenesis ... The question how baryogenesis could have happened is open to experimental tests, and it turns out that this problem can be curbed by the very stringent limits on an electric dipole moment of the neutron, a quantity that also has deep implications for particle physics. Then we discuss the recent spectacular observation of neutron quantization in the earth's gravitational field and of resonance transitions between such gravitational energy states. These measurements, together with new evaluations of neutron scattering data, set new constraints on deviations from Newton's gravitational law at the picometer scale. Such deviations are predicted in modern theories with extra-dimensions that propose unification of the Planck scale with the scale of the Standard Model ... Another main topic is the weak-interaction parameters in various fields of physics and astrophysics that must all be derived from measured neutron decay data. Up to now, about 10 different neutron decay observables have been measured, much more than needed in the electroweak Standard Model. This allows various precise tests for new physics beyond the Standard Model, competing with or surpassing similar tests at high-energy. The review ends with a discussion of neutron and nuclear data required in the synthesis of the elements during the "first three minutes" and later on in stellar nucleosynthesis.Comment: 91 pages, 30 figures, accepted by Reviews of Modern Physic

Excited States and Collectivity in

The γ decays of excited states in the very neutron-rich nucleus 88Se have been observed following the cold neutron-induced fission of 235U at the PF1B facility of the Institut Laue-Langevin (ILL), Grenoble. The EXILL array was used to measure γ - γ - γ coincidences, which were then analysed to build a level scheme of 88Se. A low (2+1) energy hints at the onset of quadrupole deformation and the identification of possible members of a (2+2) band provide evidence for γ vibrations. Shell-model calculations using a 78Ni core reproduce the experimental decay scheme well, implying that interactions between particles in the π f5/2 p and vsd orbits are responsible for much of the collectivity present. The algebraic collective model has also been used to interpret the experimental data, showing that that the experimental spectrum is consistent with 88Se being a transitional nucleus, possessing weak static β deformation and γ instability

Identification of excited states and collectivity in 88^{88}Se

International audienceThe γ decays of excited states in the very neutron-rich nucleus Se88 have been observed following the neutron-induced fission of U235. The measurement was performed using the EXILL array of Ge detectors at the PF1B cold-neutron beam facility of the Institut Laue-Langevin, Grenoble. The level scheme of Se88 was established using γ-γ-γ coincidences. A low (21+) energy hints at the onset of quadrupole deformation, and the identification of possible members of a (22+) band provide evidence for γ vibrations. Shell-model calculations using a Ni78 core reproduce the decay scheme well. Equivalent deformation and B(E2) values have previously been predicted for Se88 using pseudo-SU(3), shell-model, and beyond mean-field frameworks implying that interactions between particles in the πf5/2p and νsd orbits are mostly responsible for the collectivity present

Structure of <math><mrow><mi>N</mi><mo>=</mo><mn>56</mn></mrow></math> isotones with <math><mrow><mn>36</mn><mo>≤</mo><mi>Z</mi><mo>≤</mo><mn>42</mn></mrow></math> protons

International audienceExcited levels in Kr92, Zr96, and Mo98 nuclei were reinvestigated using high-statistics multiple-γ coincidence data measured with the EXILL and FIPPS Ge arrays, following neutron-induced fission of U235 and neutron capture on a Mo97 target, respectively. The experimental goal was to search for new levels, especially with low spins, as well as to firm up spin-parity assignments to known levels. In total of 16 new levels with 64 new or corrected decays and 35 new or improved spin-parity assignments were observed in the three nuclei. We also performed large-scale shell-model calculations to learn more about the microscopic structure of levels in these nuclei. The evolution of collectivity in N=56 isotones is discussed, stressing the important role of various single-particle excitations, in particular of the πg9/2 orbital, in the shape evolution in the region

Excited States and Collectivity in 88Se

The γ decays of excited states in the very neutron-rich nucleus 88Se have been observed following the cold neutron-induced fission of 235U at the PF1B facility of the Institut Laue-Langevin (ILL), Grenoble. The EXILL array was used to measure γ - γ - γ coincidences, which were then analysed to build a level scheme of 88Se. A low (2+1) energy hints at the onset of quadrupole deformation and the identification of possible members of a (2+2) band provide evidence for γ vibrations. Shell-model calculations using a 78Ni core reproduce the experimental decay scheme well, implying that interactions between particles in the π f5/2 p and vsd orbits are responsible for much of the collectivity present. The algebraic collective model has also been used to interpret the experimental data, showing that that the experimental spectrum is consistent with 88Se being a transitional nucleus, possessing weak static β deformation and γ instability

Structure of 90,91^{90,91}Kr nuclei: Solving the puzzle of their population in fission

International audienceExcited states of $^{90,91}$Kr nuclei have been populated following the cold-neutron-induced fission of a $^{235}$U target. The γ rays emitted following fission reactions were measured using the highly efficient array of high-purity Ge detectors, EXILL, at the Institute-Laue-Langevin, Grenoble. The surprisingly low population of $^{91}$Kr reported in the spontaneous fission of $^{252}$Cf measurement has been explained and new level schemes of $^{90,91}$Kr nuclei were established. Moderate γ collectivity is observed in both nuclei. Large-scale shell-model calculations support the experimental picture of the Z=36, Kr isotopes forming a border line between lower-Z nuclei showing moderate γ collectivity and the heavier-Z nuclei, where distinct shape changes are observed