6 research outputs found

    Complex magnetic states of heavy fermion compound CeGe

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    The intermetallic compound CeGe exhibits unusual magnetic behavior due to the interplay between the Kondo and the antiferromagnetic coupling. This particular system is interesting because the Kondo temperature is close to the Néel temperature, resulting in a close competition between the low-temperature interactions, which can be tuned by means of varying external parameters such as pressure and applied magnetic field. Interestingly, magnetization measurements up to 12 kbar reveal that the Néel temperature is not affected by pressure. Measurements of the electrical resistivity, however, show that the sharp upturn appearing below TN is sensitive to pressures up to 15 kbar. This suggests that pressure may change the complex antiferromagnetic spin structure. The validity of an explanation based on the magnetic superzones seen in the rare earths is discussed here

    Magnetic fluctuations in frustrated Laves hydrides R(Mn_{1-x}Al_{x})_{2}H_{y}

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    By neutron scattering, we have studied the spin correlations and spin fluctuations in frustrated Laves hydrides, where magnetic disorder sets in the topologically frustrated Mn lattice. Below the transition towards short range magnetic order, static spin clusters coexist with fluctuating and alsmost uncorrelated spins. The magnetic response shows a complexe lineshape, connected with the presence of the magnetic inhomogeneities. Its analysis shows the existence of two different processes, relaxation and local excitations, for the spin fluctuations below the transition. The paramagnetic fluctuations are discussed in comparison with classical spin glasses, cluster glasses, and non Fermi liquid itinerant magnets

    Kondo temperature and Heavy Fermion behavior in Yb1−xYxCuAl series of alloys

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    We report, in the present article, a detailed study of the chemical substitution effects on the magnetic, electronic transport and thermal properties of the intermediate valence system YbCuAl (Yb 1-xYxCuAl series of alloys). A more complete characterization of this series of alloys is provided including the analysis of the thermal and electronic transport properties. It is worth noticing, that less attention has been paid to experimental evidences of the ?negative pressure? effects, within right side of the Doniach diagram, when the systems move away from the QCP. Thus, it is worthwhile to explore the region of higher hybridization states, when some theoretical works point even, to the existence of anomalous Kondo behaviours. The results of this study are explained by the increase of the hybridization as consequence of the negative pressure effects, obtained by the chemical substitution of Yb by Y, thus leading to the increase of TK, in agreement with the Doniach diagram. We think that the subject of this study will be of great interest for both, the readers interested in the properties of Strongly Correlated Electron materials, and those others who work on the also vast field of Rare-Earth intermetallic

    Mesoscopic magnetic states in metallic alloys with strong electronic correlations : a percolative scenario for CeNi/sub 1-x/Cu/sub x/

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    We present evidence for the existence of magnetic clusters of approximately 20 Å in the strongly correlated alloy system CeNi1-xCux (0.7 ≤ x ≤ 0.2) based on small angle neutron scattering experiments as well as the occurrence of staircaselike hysteresis cycles at very low temperature (100 mK). An unusual feature is the observation of long-range ferromagnetic order below the cluster-glass transition without any indication of a sharp transition at a Curie temperature. These observations strongly support a phenomenological model where a percolative process connects both magnetic states. The model can account for all the puzzling data previously obtained in this system, providing a new perspective with regard to the magnetic ground state of other alloyed compounds with small magnetic moments or weak ferromagnetism with intrinsic disorder effects

    Mesoscopic magnetic states in metallic alloys with strong electronic correlations : a percolative scenario for CeNi/sub 1-x/Cu/sub x/

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    We present evidence for the existence of magnetic clusters of approximately 20 Å in the strongly correlated alloy system CeNi1-xCux (0.7 ≤ x ≤ 0.2) based on small angle neutron scattering experiments as well as the occurrence of staircaselike hysteresis cycles at very low temperature (100 mK). An unusual feature is the observation of long-range ferromagnetic order below the cluster-glass transition without any indication of a sharp transition at a Curie temperature. These observations strongly support a phenomenological model where a percolative process connects both magnetic states. The model can account for all the puzzling data previously obtained in this system, providing a new perspective with regard to the magnetic ground state of other alloyed compounds with small magnetic moments or weak ferromagnetism with intrinsic disorder effects

    Magnetocaloric properties of amorphous GdNiAl obtained by mechanical grinding

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    An amorphous GdNiAl sample was prepared by mechanical grinding performed on a crystallised intermetallic..
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