25 research outputs found
Morphology and evolution of size-selected metallic clusters deposited on a metal surface: Ag
Ground-based remote sensing profiling and numerical weather prediction model to manage nuclear power plants meteorological surveillance in Switzerland
The meteorological surveillance of the four nuclear power plants in Switzerland is of first importance in a densely populated area such as the Swiss Plateau. The project "Centrales Nucléaires et Météorologie" CN-MET aimed at providing a new security tool based on one hand on the development of a high resolution numerical weather prediction (NWP) model. The latter is providing essential nowcasting information in case of a radioactive release from a nuclear power plant in Switzerland. On the other hand, the model input over the Swiss Plateau is generated by a dedicated network of surface and upper air observations including remote sensing instruments (wind profilers and temperature/humidity passive microwave radiometers). This network is built upon three main sites ideally located for measuring the inflow/outflow and central conditions of the main wind field in the planetary boundary layer over the Swiss Plateau, as well as a number of surface automatic weather stations (AWS). The network data are assimilated in real-time into the fine grid NWP model using a rapid update cycle of eight runs per day (one forecast every three hours). This high resolution NWP model has replaced the former security tool based on in situ observations (in particular one meteorological mast at each of the power plants) and a local dispersion model. It is used to forecast the dynamics of the atmosphere in the planetary boundary layer (typically the first 4 km above ground layer) and over a time scale of 24 h. This tool provides at any time (e.g. starting at the initial time of a nuclear power plant release) the best picture of the 24-h evolution of the air mass over the Swiss Plateau and furthermore generates the input data (in the form of simulated values substituting in situ observations) required for the local dispersion model used at each of the nuclear power plants locations. This paper is presenting the concept and two validation studies as well as the results of an emergency response exercise performed in winter 2009
A trajectory-based estimate of the tropospheric ozone column using the residual method
We estimate the tropospheric column ozone using a forward trajectory model to increase the horizontal resolution of the Aura Microwave Limb Sounder (MLS) derived stratospheric column ozone. Subtracting the MLS stratospheric column from Ozone Monitoring Instrument total column measurements gives the trajectory enhanced tropospheric ozone residual (TTOR). Because of different tropopause definitions, we validate the basic residual technique by computing the 200-hPa-to-surface column and comparing it to the same product from ozonesondes and Tropospheric Emission Spectrometer measurements. Comparisons show good agreement in the tropics and reasonable agreement at middle latitudes, but there is a persistent low bias in the TTOR that may be due to a slight high bias in MLS stratospheric column. With the improved stratospheric column resolution, we note a strong correlation of extratropical tropospheric ozone column anomalies with probable troposphere-stratosphere exchange events or folds. The folds can be identified by their colocation with strong horizontal tropopause gradients. TTOR anomalies due to folds may be mistaken for pollution events since folds often occur in the Atlantic and Pacific pollution corridors. We also compare the 200-hPa-to-surface column with Global Modeling Initiative chemical model estimates of the same quantity. While the tropical comparisons are good, we note that chemical model variations in 200-hPa-to-surface column at middle latitudes are much smaller than seen in the TTOR
Regional levels of ozone in the troposphere over eastern Mediterranean
[1] During the last 5 years, information on the regional tropospheric ozone levels over the eastern Mediterranean has become available but was confined to measurements at ground level. Here available information is expanded with measurements at two more rural ground level sites spanning 8 latitude, ozonesonde ascents, lidar observations, ship cruises, and aircraft flights. During wintertime the ozone monthly values are 1020 ppbv higher than values at other European sites, while during summertime the values are comparable. This results in regional ozone background levels in the area that are above the European Union (EU) 32 ppb/ 24 hours phytotoxicity limit during the entire year. Late spring lidar observations show that south and southwestern synoptic flows which are associated with Saharan dust events result in lower ozone above the planetary boundary layer (PBL) by 20-35 ppbv as compared to these during northerly flows, which transport air from continental Europe. These lidar observations along with ship measurements during July show that ozone is enhanced 1.5-2.2 times in the continental outflow, when compared to aged maritime air or air from the African continent. These results along with ozonesonde observations suggest that ozone abatement in the area is largely beyond the control of regional emissions and can be controlled only with emission reductions on a European scale. During September, measured background NO and NO2 levels between 3 and 4.5 km above sea level ranged from 1 to 221 pptv and from 102 to 580 pptv, respectively. The troposphere contains around 40-70 Dobson units of ozone during summer and around 20-30 Dobson units during winter
Southern Hemisphere Additional Ozonesondes (SHADOZ) ozone climatology (2005â2009): Tropospheric and tropical tropopause layer (TTL) profiles with comparisons to OMI-based ozone products
We present a regional and seasonal climatology of SHADOZ ozone profiles in the troposphere and tropical tropopause layer (TTL) based on measurements taken during the first five years of Aura, 2005â2009, when new stations joined the network at Hanoi, Vietnam; Hilo, Hawaii; Alajuela/Heredia, Costa Rica; Cotonou, Benin. In all, 15 stations operated during that period. A west-to-east progression of decreasing convective influence and increasing pollution leads to distinct tropospheric ozone profiles in three regions: (1) western Pacific/eastern Indian Ocean; (2) equatorial Americas (San CristĂłbal, Alajuela, Paramaribo); (3) Atlantic and Africa. Comparisons in total ozone column from soundings, the Ozone Monitoring Instrument (OMI, on Aura, 2004-) satellite and ground-based instrumentation are presented. Most stations show better agreement with OMI than they did for EP/TOMS comparisons (1998â2004; Earth-Probe/Total Ozone Mapping Spectrometer), partly due to a revised above-burst ozone climatology. Possible station biases in the stratospheric segment of the ozone measurement noted in the first 7 years of SHADOZ ozone profiles are re-examined. High stratospheric bias observed during the TOMS period appears to persist at one station. Comparisons of SHADOZ tropospheric ozone and the daily Trajectory-enhanced Tropospheric Ozone Residual (TTOR) product (based on OMI/MLS) show that the satellite-derived column amount averages 25% low. Correlations between TTOR and the SHADOZ sondes are quite good (typical r2= 0.5â0.8), however, which may account for why some published residual-based OMI products capture tropospheric interannual variability fairly realistically. On the other hand, no clear explanations emerge for why TTOR-sonde discrepancies vary over a wide range at most SHADOZ sites
A European aerosol research lidar network to establish an aerosol climatology (EARLINET)
International audienc
SHADOZ in the Aura Era
We present comparisons of observed tropical and sub-tropical ozone from the Southern Hemisphere Additional Ozonesondes (SHADOZ) project with satellite measurements using Aura's Ozone Monitoring Instrument (OMI) and Microwave Limb Sounder (MLS) instruments. Satellite products of total and derived tropospheric column ozone from OMI and profiles of ozone in the UT/LS region from MLS are used