The phase diagram of heavy fermions with Cerium and Europium ions

Doniach phase diagram of heavy fermions with Ce and Eu ions is explained by the scaling solution of the Anderson model. At high temperatures, where the rear earth ions behave as nearly independent local moments (LM) the system has a large paramagnetic entropy and its properties are defined by Kondo temperature, $T_K(p)$, where $p$ is the external parameter, like pressure or doping. For a given $T_K(p)$, the scaling law allows an estimate of the pressure or doping dependence of the coupling constant which is then used to find the dependence of the RKKY temperature $T_{RKKY}(p)$ and N\'eel temperature $T_N(p)$ on the control parameter. The competition between the on-site Kondo coupling and the off-site RKKY coupling determines the mechanism by which the system removes the paramagnetic entropy at low temperatures. The pressure-induced change of the ground state is explained by the differences in the functional form of $T_K(p)$ and $T_{RKKY}(p)$. Our theoretical results capture the main features shown by the Doniach diagram of CeRu$_2$Ge$_2$, CeCu$_2$(Ge$_{1-x}$Si$_{x})_2$ or EuCu$_2$(Ge$_{1-x}$Si$_{x})_2$.Comment: 6 pages, 2 figure

Temperature dependence of the magnetic anisotropy of metallic Y-Ba-Cu-O single crystals in the normal phase

The magnetic anisotropy measurements of metallic Y-Ba-Cu-O compounds in the normal phase reveal a temperature-dependent diamagnetic component of the susceptibility that increases with decreasing temperature. The temperature variation of the susceptibility anisotropy and its total change do not seem to be much affected by the presence of the superconductivity at some lower temperature and could not be accounted for by superconducting fluctuations. Rather, the data remind one of the behavior of some quasi-two-dimensional metals with anisotropic Fermi surfaces, reflecting the properties of the low-energy excitations in the normal phase. The anisotropy measurements above the bulk superconducting transition temperature Tc reveal the nonlinear effects, which are due to the onset of superconductivity in disconnected grains. The existence of a two-step transition, typical for granular superconductors, should be taken into consideration if the normal-phase susceptibility data are compared with the theoretical predictions in the vicinity of Tc

Kondo effect in Ce(x)La(1-x)Cu(2.05)Si(2) intermetallics

The magnetic susceptibility and susceptibility anisotropy of the quasi-binary alloy system Ce(x)La(1-x)Cu(2.05)Si(2) have been studied for low concentration of Ce ions. The single-ion desc ription is found to be valid for x < 0.1. The experimental results are discussed in terms of t he degenerate Coqblin-Schrieffer model with a crystalline electric field splitting Delta = 330 K. The properties of the model, obtained by combining the lowest-order scaling and the pertur bation theory, provide a satisfactory description of the experimental data down to 30 K. The e xperimental results between 20 K and 2 K are explained by the exact solution of the Kondo mode l for an effective doublet.Comment: 11 pages, 13 Postscript figures, 1 tabl

Complex magnetic states of heavy fermion compound CeGe

The intermetallic compound CeGe exhibits unusual magnetic behavior due to the interplay between the Kondo and the antiferromagnetic coupling. This particular system is interesting because the Kondo temperature is close to the Néel temperature, resulting in a close competition between the low-temperature interactions, which can be tuned by means of varying external parameters such as pressure and applied magnetic field. Interestingly, magnetization measurements up to 12 kbar reveal that the Néel temperature is not affected by pressure. Measurements of the electrical resistivity, however, show that the sharp upturn appearing below TN is sensitive to pressures up to 15 kbar. This suggests that pressure may change the complex antiferromagnetic spin structure. The validity of an explanation based on the magnetic superzones seen in the rare earths is discussed here

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Magnetic anisotropy and low-frequency dielectric response of weak ferromagnetic phase in k-(BEDT-TTF)

We report a detailed characterization of the magnetism and AC transport in single crystals of the organic conductor κ-(BEDT-TTF)2Cu[ N(CN)2] Cl by means of magnetic anisotropy measurements and low-frequency dielectric spectroscopy. Magnetic anisotropy obeys Curie-Weiss law with negative Curie-Weiss temperature in the temperature range 300 K-70 K. An antiferromagnetic transition with concomitant canted antiferromagnetic state is established at 22 K. A large hysteresis in the spin-flop transition and magnetic field reversal of the weak ferromagnetic magnetization are documented for the first time. A broad dielectric relaxation mode of moderate strength ($\Delta\varepsilon\approx 3\times 10^{3}$) emerges at 32 K, and weakens with temperature. The mean relaxation time, much larger than that expected for single-particle excitations, is thermally activated in a manner similar to the DC conductivity and saturates below 22 K. These features suggest the origin of the broad relaxation as an intrinsic property of the weak ferromagnetic ground state. We propose a charged domain wall in a random ferromagnetic domain structure as the relaxation entity. We argue that the observed features might be well described if Dzyaloshinsky-Moriya interaction is taken into account. A Debye relaxation with similar temperature dependence was also observed and seems to be related to an additional ferromagnetic-like, most probably, field-induced phase. We tentatively associate this phase, whose tiny contribution was sample dependent, with a Cu2+ magnetic subsystem

Complex magnetic states of the heavy fermion compound CeGe

The intermetallic compound CeGe exhibits unusual magnetic behavior owing to the interplay between Kondo and antiferromagnetic coupling. This system is interesting because the Kondo temperature is close to the Néel temperature, so there is a close competition between the low-temperature interactions, which can be tuned by varying external parameters such as pressure and applied magnetic field. Interestingly, magnetization measurements up to 12 kbar reveal that the Néel temperature is not affected by pressure. Measurements of the electrical resistivity show, however, that the sharp upturn below TN is sensitive to pressures up to 15 kbar. This suggests that pressure may change the complex antiferromagnetic spin structure. The validity of an explanation based on the magnetic superzones seen in the rare earths is discussed here