60 research outputs found
Theory of dark resonances for alkali vapors in a buffer-gas cell
We develop an analytical theory of dark resonances that accounts for the full
atomic-level structure, as well as all field-induced effects such as coherence
preparation, optical pumping, ac Stark shifts, and power broadening. The
analysis uses a model based on relaxation constants that assumes the total
collisional depolarization of the excited state. A good qualitative agreement
with experiments for Cs in Ne is obtained.Comment: 16 pages; 7 figures; revtex4. Accepted for publication in PR
EIT and diffusion of atomic coherence
We study experimentally the effect of diffusion of Rb atoms on
Electromagnetically Induced Transparency (EIT) in a buffer gas vapor cell. In
particular, we find that diffusion of atomic coherence in-and-out of the laser
beam plays a crucial role in determining the EIT resonance lineshape and the
stored light lifetime.Comment: 5 pages, 8 figure
Experimental implementation of a four-level N-type scheme for the observation of Electromagnetically Induced Transparency
A nondegenerate four-level N-type scheme was experimentally implemented to
observe electromagnetically induced transparency (EIT) at the Rb D
line. Radiations of two independent external-cavity semiconductor lasers were
used in the experiment, the current of one of them being modulated at a
frequency equal to the hyperfine-splitting frequency of the excited 5P
level. In this case, apart from the main EIT dip corresponding to the
two-photon Raman resonance in a three-level -scheme, additional dips
detuned from the main dip by a frequency equal to the frequency of the HF
generator were observed in the absorption spectrum. These dips were due to an
increase in the medium transparency at frequencies corresponding to the
three-photon Raman resonances in four-level N-type schemes. The resonance
shapes are analyzed as functions of generator frequency and magnetic field.Comment: 3 pages, 2 figure
On the unique possibility to increase significantly the contrast of dark resonances on D1 line of Rb
We propose and study, theoretically and experimentally, a new scheme of
excitation of a coherent population trapping resonance for D1 line of alakli
atoms with nuclear spin by bichromatic linearly polarized light ({\em
lin}{\em lin} field) at the conditions of spectral resolution of the
excited state. The unique properties of this scheme result in a high contrast
of dark resonance for D1 line of Rb.Comment: 9 pages, 7 figures. This material has been partially presented on
ICONO-2005, 14 May 2005, St. Petersburg, Russia. v2 references added; text is
changed a bi
Buffer-gas induced absorption resonances in Rb vapor
We observe transformation of the electromagnetically induced transparency
(EIT) resonance into the absorption resonance in a interaction
configuration in a cell filled with Rb and a buffer gas. This
transformation occurs as a one-photon detuning of the coupling fields is varied
from the atomic transition. No such absorption resonance is found in the
absence of a buffer gas. The width of the absorption resonance is several times
smaller than the width of the EIT resonance, and the changes of absorption near
these resonances are about the same. Similar absorption resonances are detected
in the Hanle configuration in a buffered cell.Comment: 11 pages, 15 figures; 13 pages, 17 figures, added numerical
simulatio
Ultra-precise measurement of optical frequency ratios
We developed a novel technique for frequency measurement and synthesis, based
on the operation of a femtosecond comb generator as transfer oscillator. The
technique can be used to measure frequency ratios of any optical signals
throughout the visible and near-infrared part of the spectrum. Relative
uncertainties of for averaging times of 100 s are possible. Using a
Nd:YAG laser in combination with a nonlinear crystal we measured the frequency
ratio of the second harmonic at 532 nm to the fundamental at
1064 nm, .Comment: 4 pages, 4 figure
Hybrid Mechanical Systems
We discuss hybrid systems in which a mechanical oscillator is coupled to
another (microscopic) quantum system, such as trapped atoms or ions,
solid-state spin qubits, or superconducting devices. We summarize and compare
different coupling schemes and describe first experimental implementations.
Hybrid mechanical systems enable new approaches to quantum control of
mechanical objects, precision sensing, and quantum information processing.Comment: To cite this review, please refer to the published book chapter (see
Journal-ref and DOI). This v2 corresponds to the published versio
Resonant nonlinear magneto-optical effects in atoms
In this article, we review the history, current status, physical mechanisms,
experimental methods, and applications of nonlinear magneto-optical effects in
atomic vapors. We begin by describing the pioneering work of Macaluso and
Corbino over a century ago on linear magneto-optical effects (in which the
properties of the medium do not depend on the light power) in the vicinity of
atomic resonances, and contrast these effects with various nonlinear
magneto-optical phenomena that have been studied both theoretically and
experimentally since the late 1960s. In recent years, the field of nonlinear
magneto-optics has experienced a revival of interest that has led to a number
of developments, including the observation of ultra-narrow (1-Hz)
magneto-optical resonances, applications in sensitive magnetometry, nonlinear
magneto-optical tomography, and the possibility of a search for parity- and
time-reversal-invariance violation in atoms.Comment: 51 pages, 23 figures, to appear in Rev. Mod. Phys. in Oct. 2002,
Figure added, typos corrected, text edited for clarit
Orbital redistribution in molecular nanostructures mediated by metal-organic bonds
Dicyanovinyl-quinquethiophene (DCV5T-Me) is a prototype conjugated oligomer for highly efficient organic solar cells. This class of oligothiophenes are built up by an electron-rich donor (D) backbone and terminal electron-deficient acceptor (A) moieties. Here, we investigated its structural and electronic properties when it is adsorbed on a Au(111) surface using low temperature scanning tunneling microscopy/spectroscopy (STM/STS) and atomic force microscopy (AFM). We find that DCV5T-Me self-assembles in extended chains, stabilized by intercalated Au atoms. The effect of metal-ligand hybridization with Au adatoms causes an energetic downshift of the DCV5T-Me lowest unoccupied molecular orbital (LUMO) with respect to the uncoordinated molecules on the surface. The asymmetric coordination of a gold atom to only one molecular end group leads to an asymmetric localization of the LUMO and LUMO+1 states at opposite sides. Using model density functional theory (DFT) calculations, we explain such orbital reshaping as a consequence of linear combinations of the original LUMO and LUMO+1 orbitals, mixed by the attachment of a bridging Au adatom. Our study shows that the alignment of molecular orbitals and their distribution within individual molecules can be modified by contacting them to metal atoms in specific sites
- …