85 research outputs found
Attosecond electron spectroscopy using a novel interferometric pump-probe technique
We present an interferometric pump-probe technique for the characterization
of attosecond electron wave packets (WPs) that uses a free WP as a reference to
measure a bound WP. We demonstrate our method by exciting helium atoms using an
attosecond pulse with a bandwidth centered near the ionization threshold, thus
creating both a bound and a free WP simultaneously. After a variable delay, the
bound WP is ionized by a few-cycle infrared laser precisely synchronized to the
original attosecond pulse. By measuring the delay-dependent photoelectron
spectrum we obtain an interferogram that contains both quantum beats as well as
multi-path interference. Analysis of the interferogram allows us to determine
the bound WP components with a spectral resolution much better than the inverse
of the attosecond pulse duration.Comment: 5 pages, 4 figure
Copper Sorption by Coal Substances from Aqueous Solutions
The copper cations sorption by brown coal, humic acids and residual coal samples after the extraction of humic acid was studied by using the methods of spectroscopy FT-IR, EPR, Solid State CP/MAS 13C-NMR. Samples of lignite (brown coal) of the Tisulsky deposit (TL) of Kansk-Achinsk brown coal basin (Russia), its naturaloxidized form (NOLF), as well as samples of the humic acids (HA) extracted from them, and the residual coal after the extraction of humic acids (RC) were used as sorbents. The copper cations sorption process by the investigated samples depends on contribution of several mechanisms in varying degrees. It may be an ion exchange; complexation with the functional groups of the electron donor; complexation to form the bond Mez+ – HA due to the presence of the free π-electrons on the surface. The quantity of adsorbed copper cations depends on the functional and structural composition of the investigated samples. The copper cations sorption by the coals, humic acids and residual coals reduces the number of paramagnetic centers in the samples and the intensity of the NMR spectra. The copper cations sorption by HA from TL is determined by the significant contribution of the ion exchange process. HA from NOLF; initial TL and NOLF; RC TL and RC NOLF sorb copper cations mainly due to the formation of complexes with individual functional groups and the negatively charged surface portions. The data of 13C-NMR and EPR studies have shown that the aromatic structures make the main contribution to the complexation
Transition energy and lifetime for the ground state hyperfine splitting of high Z lithiumlike ions
The ground state hyperfine splitting values and the transition probabilities
between the hyperfine structure components of high Z lithiumlike ions are
calculated in the range . The relativistic, nuclear, QED and
interelectronic interaction corrections are taken into account. It is found
that the Bohr-Weisskopf effect can be eliminated in a combination of the
hyperfine splitting values of the hydrogenlike and lithiumlike ions of an
isotope. This gives a possibility for testing the QED effects in a combination
of the strong electric and magnetic fields of the heavy nucleus. Using the
experimental result for the hyperfine splitting in ^{209}Bi^{82+}, the 2s
hyperfine splitting in ^{209}Bi^{80+} is calculated to be \Delta E=0.7969(2)
eV.Comment: The nuclear charge distribution correction \delta is corrected, 14
pages, Late
Trap with ultracold neutrons as a detector of dark matter particles with long-range forces
The possibility of using a trap with ultracold neutrons as a detector of dark
matter particles with long-range forces is considered. The basic advantage of
the proposed method lies in possibility of detecting the recoil energy 10-7 eV.
The restrictions on parameters of Yukawa type interaction potential between
dark matter particles and a neutron are presented for different dark matter
densities on the Earth. The assumption concerned with long-range interaction of
dark matter particles and ordinary matter leads to a substantial enhancement of
cross section at low energy. Consequently, there arises a possibility of
capture and accumulation of dark matter in a gravitational field of the Earth.
Rough estimation of accumulation of low-energy dark matter on the Earth is
discussed. The first experimental restrictions for existence of dark matter
with long-range forces on the Earth are presented.Comment: 17 pages, 6 figure
Efficient and accurate modeling of electron photoemission in nanostructures with TDDFT
We derive and extend the time-dependent surface-flux method introduced in [L. Tao, A. Scrinzi, New J. Phys. 14, 013021 (2012)] within a time-dependent density-functional theory (TDDFT) formalism and use it to calculate photoelectron spectra and angular distributions of atoms and molecules when excited by laser pulses. We present other, existing computational TDDFT methods that are suitable for the calculation of electron emission in compact spatial regions, and compare their results. We illustrate the performance of the new method by simulating strong-field ionization of C60 fullerene and discuss final state effects in the orbital reconstruction of planar organic molecules
Attosecond imaging of XUV-induced atomic photoemission and Auger decay in strong laser fields
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