9,794 research outputs found
Matter-Wave Decoherence due to a Gas Environment in an Atom Interferometer
Decoherence due to scattering from background gas particles is observed for
the first time in a Mach-Zehnder atom interferometer, and compared with
decoherence due to scattering photons. A single theory is shown to describe
decoherence due to scattering either atoms or photons. Predictions from this
theory are tested by experiments with different species of background gas, and
also by experiments with different collimation restrictions on an atom beam
interferometer.Comment: 4 pages, 3 figures, accepted to PR
Experimental generation of pseudo bound entanglement
We use Nuclear Magnetic Resonance (NMR) to experimentally generate a bound
entangled (more precisely: pseudo bound entangled) state, i.e. a quantum state
which is non-distillable but nevertheless entangled. Our quantum system
consists of three qubits. We characterize the produced state via state
tomography to show that the created state has a positive partial transposition
with respect to any bipartite splitting, and we use a witness operator to prove
its entanglement.Comment: 5 page
Jahn-Teller Distortions and the Supershell Effect in Metal Nanowires
A stability analysis of metal nanowires shows that a Jahn-Teller deformation
breaking cylindrical symmetry can be energetically favorable, leading to stable
nanowires with elliptic cross sections. The sequence of stable cylindrical and
elliptical nanowires allows for a consistent interpretation of experimental
conductance histograms for alkali metals, including both the shell and
supershell structures. It is predicted that for gold, elliptical nanowires are
even more likely to form since their eccentricity is smaller than for alkali
metals. The existence of certain metastable ``superdeformed'' nanowires is also
predicted
Out of Africa: High aerosol concentrations in the upper troposphere over Africa
International audienceIn the year 2000, six flights (three southbound and three northbound) of the CARIBIC project were conducted between Germany and two destinations in the southern hemisphere (Windhoek, Namibia and Cape Town, South Africa). In the present report, results on particle number concentrations are discussed in three size ranges (>4 nm, >12 nm, and >18 nm particle diameter) during the unique transequatorial Africa flights. The flights covered a total of about 80 h in May, July, and December. Thus, no claim can be made for long-term representativeness of the aerosol data. Nevertheless, they are the first upper systematic tropospheric transequatorial aerosol profiles over Africa. The average aerosol results show a broad maximum, roughly symmetrical to the equator, which compares well in latitudinal extent to a maximum of CO concentrations measured on the same flights. This export of continental surface aerosol to the upper troposphere will be dispersed on a global scale both with the easterly flow near the equator and with the westerlies in the adjacent subtropical regions. There was strong evidence of recent new particle formation before aerosol arrival at flight level, in particular during the time periods between 9:00 and 13:00 local time over Africa. Direct and indirect climate effects of the respective particulate matter remain to be investigated by future flights with the ongoing extension of the CARIBIC payload towards size-resolved measurements above 100 nm particle diameter. At the same time global chemical transport models and aerosol dynamics models need to be extended to be able to reproduce the CARIBIC findings over Africa
Nanoscale π-π Stacked molecules are bound by collective charge fluctuations
Non-covalent π-π interactions are central to chemical and biological processes, yet the full understanding of their origin that would unite the simplicity of empirical approaches with the accuracy of quantum calculations is still missing. Here we employ a quantum-mechanical Hamiltonian model for van der Waals interactions, to demonstrate that intermolecular electron correlation in large supramolecular complexes at equilibrium distances is appropriately described by collective charge fluctuations. We visualize these fluctuations and provide connections both to orbital-based approaches to electron correlation, as well as to the simple London pairwise picture. The reported binding energies of ten supramolecular complexes obtained from the quantum-mechanical fluctuation model joined with density functional calculations are within 5% of the reference energies calculated with the diffusion quantum Monte-Carlo method. Our analysis suggests that π-π stacking in supramolecular complexes can be characterized by strong contributions to the binding energy from delocalized, collective charge fluctuations-in contrast to complexes with other types of bonding
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Out of Africa: High aerosol concentrations in the upper troposphere over Africa
In the year 2000, six flights (three southbound and three northbound) of the CARIBIC project were conducted between Germany and two destinations in the southern hemisphere (Windhoek, Namibia and Cape Town, South Africa). In the present report, results on particle number concentrations are discussed in three size ranges (>4 nm, >12 nm, and >18 nm particle diameter) during the unique transequatorial Africa flights. The flights covered a total of about 80 h in May, July, and December. Thus, no claim can be made for long-term representativeness of the aerosol data. Nevertheless, they are the first upper systematic tropospheric transequatorial aerosol profiles over Africa. The average aerosol results show a broad maximum, roughly symmetrical to the equator, which compares well in latitudinal extent to a maximum of CO concentrations measured on the same flights. This export of continental surface aerosol to the upper troposphere will be dispersed on a global scale both with the easterly flow near the equator and with the westerlies in the adjacent subtropical regions. There was strong evidence of recent new particle formation before aerosol arrival at flight level, in particular during the time periods between 9:00 and 13:00 local time over Africa. Direct and indirect climate effects of the respective particulate matter remain to be investigated by future flights with the ongoing extension of the CARIBIC payload towards size-resolved measurements above 100 nm particle diameter. At the same time global chemical transport models and aerosol dynamics models need to be extended to be able to reproduce the CARIBIC findings over Africa
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