Magnetohydrodynamic rotation in an annulus

Liquid metal conductor confined between two concentric cylindrical electrode

Hyperfine-mediated gate-driven electron spin resonance

An all-electrical spin resonance effect in a GaAs few-electron double quantum dot is investigated experimentally and theoretically. The magnetic field dependence and absence of associated Rabi oscillations are consistent with a novel hyperfine mechanism. The resonant frequency is sensitive to the instantaneous hyperfine effective field, and the effect can be used to detect and create sizable nuclear polarizations. A device incorporating a micromagnet exhibits a magnetic field difference between dots, allowing electrons in either dot to be addressed selectively.Comment: related papers available at http://marcuslab.harvard.ed

Spin filling of a quantum dot derived from excited-state spectroscopy

We study the spin filling of a semiconductor quantum dot using excited-state spectroscopy in a strong magnetic field. The field is oriented in the plane of the two-dimensional electron gas in which the dot is electrostatically defined. By combining the observation of Zeeman splitting with our knowledge of the absolute number of electrons, we are able to determine the ground state spin configuration for one to five electrons occupying the dot. For four electrons, we find a ground state spin configuration with total spin S=1, in agreement with Hund's first rule. The electron g-factor is observed to be independent of magnetic field and electron number.Comment: 11 pages, 7 figures, submitted to New Journal of Physics, focus issue on Solid State Quantum Informatio

Asymmetry of Nonlinear Transport and Electron Interactions in Quantum Dots

The symmetry properties of transport beyond the linear regime in chaotic quantum dots are investigated experimentally. A component of differential conductance that is antisymmetric in both applied source-drain bias V and magnetic field B, absent in linear transport, is found to exhibit mesoscopic fluctuations around a zero average. Typical values of this component allow a measurement of the electron interaction strength.Comment: related papers at http://marcuslab.harvard.ed

Conditional operation of a spin qubit

We report coherent operation of a singlet-triplet qubit controlled by the arrangement of two electrons in an adjacent double quantum dot. The system we investigate consists of two pairs of capacitively coupled double quantum dots fabricated by electrostatic gates on the surface of a GaAs heterostructure. We extract the strength of the capacitive coupling between qubit and double quantum dot and show that the present geometry allows fast conditional gate operation, opening pathways to multi-qubit control and implementation of quantum algorithms with spin qubits.Comment: related papers here: http://marcuslab.harvard.ed

Facile O-atom insertion into C-C and C-H bonds by a trinuclear copper complex designed to harness a singlet oxene

Two trinuclear copper [CuICuICuI(L)]1+ complexes have been prepared with the multidentate ligands (L) 3,3'-(1,4-diazepane-1,4-diyl)bis(1-((2-(dimethylamino)ethyl)(methyl)amino)propan-2-ol) (7-Me) and (3,3'-(1,4-diazepane-1,4-diyl)bis(1-((2-(diethylamino) ethyl)(ethyl) amino)propan-2-ol) (7-Et) as models for the active site of the particulate methane monooxygenase (pMMO). The ligands were designed to form the proper spatial and electronic geometry to harness a "singlet oxene," according to the mechanism previously suggested by our laboratory. Consistent with the design strategy, both [CuICuICuI(L)]1+ reacted with dioxygen to form a putative bis(µ3-oxo)CuIICuIICuIII species, capable of facile O-atom insertion across the central C-C bond of benzil and 2,3-butanedione at ambient temperature and pressure. These complexes also catalyze facile O-atom transfer to the C-H bond of CH3CN to form glycolonitrile. These results, together with our recent biochemical studies on pMMO, provide support for our hypothesis that the hydroxylation site of pMMO contains a trinuclear copper cluster that mediates C-H bond activation by a singlet oxene mechanism

Geometry of Discrete Quantum Computing

Conventional quantum computing entails a geometry based on the description of an n-qubit state using 2^{n} infinite precision complex numbers denoting a vector in a Hilbert space. Such numbers are in general uncomputable using any real-world resources, and, if we have the idea of physical law as some kind of computational algorithm of the universe, we would be compelled to alter our descriptions of physics to be consistent with computable numbers. Our purpose here is to examine the geometric implications of using finite fields Fp and finite complexified fields Fp^2 (based on primes p congruent to 3 mod{4}) as the basis for computations in a theory of discrete quantum computing, which would therefore become a computable theory. Because the states of a discrete n-qubit system are in principle enumerable, we are able to determine the proportions of entangled and unentangled states. In particular, we extend the Hopf fibration that defines the irreducible state space of conventional continuous n-qubit theories (which is the complex projective space CP{2^{n}-1}) to an analogous discrete geometry in which the Hopf circle for any n is found to be a discrete set of p+1 points. The tally of unit-length n-qubit states is given, and reduced via the generalized Hopf fibration to DCP{2^{n}-1}, the discrete analog of the complex projective space, which has p^{2^{n}-1} (p-1)\prod_{k=1}^{n-1} (p^{2^{k}}+1) irreducible states. Using a measure of entanglement, the purity, we explore the entanglement features of discrete quantum states and find that the n-qubit states based on the complexified field Fp^2 have p^{n} (p-1)^{n} unentangled states (the product of the tally for a single qubit) with purity 1, and they have p^{n+1}(p-1)(p+1)^{n-1} maximally entangled states with purity zero.Comment: 24 page

New Gauge Invariant Formulation of the Chern-Simons Gauge Theory: Classical and Quantal Analysis

Recently proposed new gauge invariant formulation of the Chern-Simons gauge theory is considered in detail. This formulation is consistent with the gauge fixed formulation. Furthermore it is found that the canonical (Noether) Poincar\'e generators are not gauge invariant even on the constraints surface and do not satisfy the Poincar\'e algebra contrast to usual case. It is the improved generators, constructed from the symmetric energy-momentum tensor, which are (manifestly) gauge invariant and obey the quantum as well as classical Poincar\'e algebra. The physical states are constructed and it is found in the Schr\"odinger picture that unusual gauge invariant longitudinal mode of the gauge field is crucial for constructing the physical wavefunctional which is genuine to (pure) Chern-Simons theory. In matching to the gauge fixed formulation, we consider three typical gauges, Coulomb, axial and Weyl gauges as explicit examples. Furthermore, recent several confusions about the effect of Dirac's dressing function and the gauge fixings are clarified. The analysis according to old gauge independent formulation a' la Dirac is summarized in an appendix.Comment: No figures, 44 page

Application of the canonical quantization of systems with curved phase space to the EMDA theory

The canonical quantization of dynamical systems with curved phase space introduced by I.A. Batalin, E.S. Fradkin and T.E. Fradkina is applied to the four-dimensional Einstein-Maxwell Dilaton-Axion theory. The spherically symmetric case with radial fields is considered. The Lagrangian density of the theory in the Einstein frame is written as an expression with first order in time derivatives of the fields. The phase space is curved due to the nontrivial interaction of the dilaton with the axion and the electromagnetic fields.Comment: 23 pages in late