39 research outputs found
The poisoning effect of Mn in LaFe(1-x)Mn(x)AsO(0.89)F(0.11): unveiling a quantum critical point in the phase diagram of iron-based superconductors
A superconducting-to-magnetic transition is reported for
LaFeMnAsOF where a per thousand amount of Mn
impurities is dispersed. By employing local spectroscopic techniques like muon
spin rotation (muSR) and nuclear quadrupole resonance (NQR) on compounds with
Mn contents ranging from x=0.025% to x=0.75%, we find that the electronic
properties are extremely sensitive to the Mn impurities. In fact, a small
amount of Mn as low as 0.2% suppresses superconductivity completely. Static
magnetism, involving the FeAs planes, is observed to arise for x > 0.1% and
becomes further enhanced upon increasing Mn substitution. Also a progressive
increase of low energy spin fluctuations, leading to an enhancement of the NQR
spin-lattice relaxation rate 1/T1, is observed upon Mn substitution. The
analysis of 1/T1 for the sample closest to the the crossover between
superconductivity and magnetism (x = 0.2%) points towards the presence of an
antiferromagnetic quantum critical point around that doping level.Comment: 11 pages, 10 figure
Disorder-induced Spin Gap in the Zigzag Spin-1/2 Chain Cuprate Sr_{0.9}Ca_{0.1}CuO_2
We report a comparative study of 63Cu Nuclear Magnetic Resonance spin lattice
relaxation rates, T_1^{-1}, on undoped SrCuO_2 and Ca doped
Sr_{0.9}Ca_{0.1}CuO_2 spin chain compounds. A temperature independent T_1^{-1}
is observed for SrCuO_2 as expected for an S=1/2 Heisenberg chain.
Surprisingly, we observe an exponential decrease of T_1^{-1} for T < 90,K in
the Ca-doped sample evidencing the opening of a spin gap. The data analysis
within the J_1-J_2 Heisenberg model employing density-matrix renormalization
group calculations suggests an impurity driven small alternation of the
J_2-exchange coupling as a possible cause of the spin gap.Comment: 4 pages, 4 figure
Spin Gap in the Single Spin-1/2 Chain Cuprate SrCaCuO
We report Cu nuclear magnetic resonance and muon spin rotation
measurements on the S=1/2 antiferromagnetic Heisenberg spin chain compound
SrCaCuO. An exponentially decreasing spin-lattice
relaxation rate 1/T indicates the opening of a spin gap. This behavior is
very similar to what has been observed for the cognate zigzag spin chain
compound SrCaCuO, and confirms that the occurrence of a
spin gap upon Ca doping is independent of the interchain exchange coupling
. Our results therefore generally prove the appearance of a spin gap in an
antiferromagnetic Heisenberg spin chain induced by a local bond disorder of the
intrachain exchange coupling . A low temperature upturn of 1/T evidences
growing magnetic correlations. However, zero field muon spin rotation
measurements down to 1.5 K confirm the absence of magnetic order in this
compound which is most likely suppressed by the opening of the spin gap.Comment: 5 pages, 4 figure
Nanoscale Electronic Order in Iron Pnictides
The charge distribution in RFeAs (R=La, Sm) iron pnictides is probed using As NQR. Whereas undoped and optimally-doped/overdoped compounds feature a single charge environment, two charge environments are detected in the underdoped region. Spin- lattice relaxation measurements show their coexistence at the nanoscale. Together with the quantitative variations of the spectra with doping, they point at a local electronic order in the iron layers, where low- and high-doping-like regions would coexist. Implications for the interplay of static magnetism and superconductivity are discussed
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Electronic properties of LaO1-xFxFeAs in the normal state probed by nmr/nqr
We report 139La, 57Fe and 75As nuclear magnetic resonance (NMR) and nuclear quadrupole resonance (NQR) measurements on powders of the new LaO1−xFxFeAs superconductor for x=0 and 0.1 at temperatures up to 480 K, and compare our measured NQR spectra with local density approximation (LDA) calculations. For all three nuclei in the x=0.1 material, it is found that the local Knight shift increases monotonically with an increase in temperature, and scales with the macroscopic susceptibility, suggesting a single magnetic degree of freedom. Surprisingly, the spin lattice relaxation rates for all nuclei also scale with one another, despite the fact that the form factors for each site sample different regions of q-space. This result suggests a lack of any q-space structure in the dynamical spin susceptibility that might be expected in the presence of antiferromagnetic correlations. Rather, our results are more compatible with simple quasi-particle scattering. Furthermore, we find that the increase in the electric field gradient at the As cannot be accounted for by LDA calculations, suggesting that structural changes, in particular the position of the As in the unit cell, dominate the NQR response
Evidence for Pauli-limiting behaviour at high fields and enhanced upper critical fields near T_c in several disordered FeAs based Superconductors
We report resistivity and upper critical field B_c2(T) data for disordered
(As deficient) LaO_0.9F_0.1FeAs_1-delta in a wide temperature and high field
range up to 60 T. These samples exhibit a slightly enhanced superconducting
transition at T_c = 28.5 K and a significantly enlarged slope dB_c2/dT = -5.4
T/K near T_c which contrasts with a flattening of B_c2(T) starting near 23 K
above 30 T. The latter evidences Pauli limiting behaviour (PLB) with B_c2(0)
approximately 63 T. We compare our results with B_c2(T)-data from the
literature for clean and disordered samples. Whereas clean samples show almost
no PLB for fields below 60 to 70 T, the hitherto unexplained pronounced
flattening of B_c2(T) for applied fields H II ab observed for several
disordered closely related systems is interpreted also as a manifestation of
PLB. Consequences are discussed in terms of disorder effects within the frames
of (un)conventional superconductivity, respectively.Comment: 2 pages, 3 figures, submitted to M2S Tokyo 0