127 research outputs found
Raman light scattering study and microstructural analysis of epitaxial films of the electron-doped superconductor La_{2-x}Ce_{x}CuO_{4}
We present a detailed temperature-dependent Raman light scattering study of
optical phonons in molecular-beam-epitaxy-grown films of the electron-doped
superconductor La_{2-x}Ce_{x}CuO_{4} close to optimal doping (x ~ 0.08, T_c =
29 K and x ~ 0.1, T_c = 27 K). The main focus of this work is a detailed
characterization and microstructural analysis of the films. Based on
micro-Raman spectroscopy in combination with x-ray diffraction,
energy-dispersive x-ray analysis, and scanning electron microscopy, some of the
observed phonon modes can be attributed to micron-sized inclusions of Cu_{2}O.
In the slightly underdoped film (x ~ 0.08), both the Cu_{2}O modes and others
that can be assigned to the La_{2-x}Ce_{x}CuO_{4} matrix show pronounced
softening and narrowing upon cooling below T ~ T_c. Based on control
measurements on commercial Cu_{2}O powders and on a comparison to prior Raman
scattering studies of other high-temperature superconductors, we speculate that
proximity effects at La_{2-x}Ce_{x}CuO_{4}/Cu_{2}O interfaces may be
responsible for these anomalies. Experiments on the slightly overdoped
La_{2-x}Ce_{x}CuO_{4} film (x ~ 0.1) did not reveal comparable phonon
anomalies.Comment: 7 pages, 8 figure
Electron-phonon vertex in the two-dimensional one-band Hubbard model
Using quantum Monte Carlo techniques, we study the effects of electronic
correlations on the effective electron-phonon (el-ph) coupling in a
two-dimensional one-band Hubbard model. We consider a momentum-independent bare
ionic el-ph coupling. In the weak- and intermediate-correlation regimes, we
find that the on-site Coulomb interaction acts to effectively suppress the
ionic el-ph coupling at all electron- and phonon- momenta. In this regime, our
numerical simulations are in good agreement with the results of perturbation
theory to order . However, entering the strong-correlation regime, we find
that the forward scattering process stops decreasing and begins to
substantially increase as a function of , leading to an effective el-ph
coupling which is peaked in the forward direction. Whereas at weak and
intermediate Coulomb interactions, screening is the dominant correlation effect
suppressing the el-ph coupling, at larger values irreducible vertex
corrections become more important and give rise to this increase. These vertex
corrections depend crucially on the renormalized electronic structure of the
strongly correlated system.Comment: 5 pages, 4 eps-figures, minor change
Inelastic x-ray scattering investigations of lattice dynamics in SmFeAsOF superconductors
We report measurements of the phonon density of states as measured with
inelastic x-ray scattering in SmFeAsOF powders. An unexpected
strong renormalization of phonon branches around 23 meV is observed as fluorine
is substituted for oxygen. Phonon dispersion measurements on
SmFeAsOF single crystals allow us to identify the 21 meV A
in-phase (Sm,As) and the 26 meV B (Fe,O) modes to be responsible for
this renormalization, and may reveal unusual electron-phonon coupling through
the spin channel in iron-based superconductors.Comment: 4 pages, 3 figures, submitted for SNS2010 conference proceeding
Hole concentration and phonon renormalization in Ca-doped YBa_2Cu_3O_y (6.76 < y < 7.00)
In order to access the overdoped regime of the YBa_2Cu_3O_y phase diagram, 2%
Ca is substituted for Y in YBa_2Cu_3O_y (y = 7.00,6.93,6.88,6.76). Raman
scattering studies have been carried out on these four single crystals.
Measurements of the superconductivity-induced renormalization in frequency
(Delta \omega) and linewidth (\Delta 2\gamma) of the 340 cm^{-1} B_{1g} phonon
demonstrate that the magnitude of the renormalization is directly related to
the hole concentration (p), and not simply the oxygen content. The changes in
\Delta \omega with p imply that the superconducting gap (\Delta_{max})
decreases monotonically with increasing hole concentration in the overdoped
regime, and \Delta \omega falls to zero in the underdoped regime. The linewidth
renormalization \Delta 2\gamma is negative in the underdoped regime, crossing
over at optimal doping to a positive value in the overdoped state.Comment: 18 pages; 5 figures; submitted to Phys. Rev. B Oct. 24, 2002 (BX8292
On the effect of heterovalent substitutions in ruthenocuprates
We discuss the properties of superconducting derivatives of the RuSr2GdCu2O8
(1212-type) ruthenocuprate, for which heterovalent doping has been achieved
through partial substitution of Cu ions into the RuO2 planes
(Ru1-xSr2GdCu2+xO8-d, 0<x<0.75, Tcmax=72 K for x=0.3-0.4) and Ce ions into the
Gd sites (RuSr2Gd1-yCeyCu2O8, 0<y<0.1). The measurements of XANES, thermopower,
and magnetization under external pressure reveal an underdoped character of all
compounds. Muon spin rotation experiments indicate the presence of magnetic
order at low temperatures (Tm=14-2 K for x=0.1-0.4). Properties of these two
series lead us to the qualitative phase diagram for differently doped 1212-type
ruthenocuprates. The difference in temperature of magnetic ordering found for
superconducting and non-superconducting RuSr2GdCu2O8 is discussed in the
context of the properties of substituted compounds. The high pressure oxygen
conditions required for synthesis of Ru1-xSr2RECu2+xO8-d, have been extended to
synthesis of a Ru1-xSr2Eu2-yCeyCu2+xO10-d series. The Cu->Ru doping achieved in
these phases is found to decrease the temperature for magnetic ordering as well
the volume fraction of the magnetic phase.Comment: Proceedings of the 3rd Polish-US Workshop on Magnetism and
Superconductivity of Advanced Materials, July 14-19, 2002, Ladek Zdroj
(Poland) to appear in Physica
A study of the superconducting gap in RNiBC (R = Y, Lu) single crystals by inelastic light scattering
Superconductivity-induced changes in the electronic Raman scattering response
were observed for the RNiBC (R = Y, Lu) system in different scattering
geometries. In the superconducting state, 2-like peaks were observed in
A, B, and B spectra from single crystals. The peaks in
A and B symmetries are significantly sharper and stronger than
the peak in B symmetry. The temperature dependence of the frequencies of
the 2-like peaks shows typical BCS-type behavior, but the apparent
values of the gap are strongly anisotropic for both systems. In
addition, for both YNiBC and LuNiBC systems, there exists
reproducible scattering strength below the gap which is roughly
linear to the frequency in B and B symmetries. This discovery of
scattering below the gap in non-magnetic borocarbide superconductors, which are
thought to be conventional BCS-type superconductors, is a challenge for current
understanding of superconductivity in this system.Comment: Added text, changed a figure, and added references. Will appear in
Phys. Rev.
C-axis lattice dynamics in Bi-based cuprate superconductors
We present results of a systematic study of the c axis lattice dynamics in
single layer Bi2Sr2CuO6 (Bi2201), bilayer Bi2Sr2CaCu2O8 (Bi2212) and trilayer
Bi2Sr2Ca2Cu3O10 (Bi2223) cuprate superconductors. Our study is based on both
experimental data obtained by spectral ellipsometry on single crystals and
theoretical calculations. The calculations are carried out within the framework
of a classical shell model, which includes long-range Coulomb interactions and
short-range interactions of the Buckingham form in a system of polarizable
ions. Using the same set of the shell model parameters for Bi2201, Bi2212 and
Bi2223, we calculate the frequencies of the Brillouin-zone center phonon modes
of A2u symmetry and suggest the phonon mode eigenvector patterns. We achieve
good agreement between the calculated A2u eigenfrequencies and the experimental
values of the c axis TO phonon frequencies which allows us to make a reliable
phonon mode assignment for all three Bi-based cuprate superconductors. We also
present the results of our shell model calculations for the Gamma-point A1g
symmetry modes in Bi2201, Bi2212 and Bi2223 and suggest an assignment that is
based on the published experimental Raman spectra. The
superconductivity-induced phonon anomalies recently observed in the c axis
infrared and resonant Raman scattering spectra in trilayer Bi2223 are
consistently explained with the suggested assignment.Comment: 29 pages, 13 figure
Lattice Dynamics of LaFeAsO_{1-x}F_{x} and PrFeAsO_{1-y} via Inelastic X-Ray Scattering and First-Principles Calculation
The lattice dynamics of LaFeAsO_{1-x}F_{x} (x=0, 0.1) and PrFeAsO_{1-y}
(y~0.1) are investigated using inelastic x-ray scattering and ab-initio
calculation. Measurements of powder samples provide an approximation to the
phonon DOS, while dispersion is measured from a single crystal of
PrFeAsO_{1-y}. A model that agrees reasonably well with all of the data at room
temperature is built from results of ab-initio calculations by softening the
strength of the Fe-As bond by 30%.Comment: 4 pages, 4 figures; some changes of the text and a revision of figure
Theory of Coexistence of Superconductivity and Ferroelectricity : A Dynamical Symmetry Model
We propose and investigate a model for the coexistence of Superconductivity
(SC) and Ferroelectricity (FE) based on the dynamical symmetries for
the pseudo-spin SC sector, for the displaced oscillator FE sector, and
for the composite system. We assume a minimal
symmetry-allowed coupling, and simplify the hamiltonian using a double mean
field approximation (DMFA). A variational coherent state (VCS) trial
wave-function is used for the ground state: the energy, and the relevant order
parameters for SC and FE are obtained. For positive sign of the SC-FE coupling
coefficient, a non-zero value of either order parameter can suppress the other
(FE polarization suppresses SC and vice versa). This gives some support to
"Matthias' Conjecture" [1964], that SC and FE tend to be mutually exclusive.
For such a Ferroelectric Superconductor we predict: a) the SC gap
(and ) will increase with increasing applied pressure when pressure
quenches FE as in many ferroelectrics, and b) the FE polarization will increase
with increaesing magnetic field up to . The last result is equivalent to
the prediction of a new type of Magneto-Electric Effect in a coexistent SC-FE
material. Some discussion will be given of the relation of these results to the
cuprate superconductors.Comment: 46 page
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