Trends and variability of midlatitude stratospheric water vapour deduced from the re-evaluated Boulder balloon series and HALOE

This paper presents an updated trend analysis of water vapour in the lower midlatitude stratosphere from the Boulder balloon-borne NOAA frostpoint hygrometer measurements and from the Halogen Occulation Experiment (HALOE). Two corrections for instrumental bias are applied to homogenise the frostpoint data series, and a quality assessment of all soundings after 1991 is presented. Linear trend estimates based on the corrected data for the period 1980–2000 are up to 40% lower than previously reported. Vertically resolved trends and variability are calculated with a multi regression analysis including the quasi-biennal oscillation and equivalent latitude as explanatory variables. In the range of 380 to 640 K potential temperature (≈14 to 25 km), the frostpoint data from 1981 to 2006 show positive linear trends between 0.3±0.3 and 0.7±0.1%/yr. The same dataset shows trends between −0.2±0.3 and 1.0±0.3%/yr for the period 1992 to 2005. HALOE data over the same time period suggest negative trends ranging from −1.1±0.2 to −0.1±0.1%/yr. In the lower stratosphere, a rapid drop of water vapour is observed in 2000/2001 with little change since. At higher altitudes, the transition is more gradual, with slowly decreasing concentrations between 2001 and 2007. This pattern is consistent with a change induced by a drop of water concentrations at entry into the stratosphere. Previously noted differences in trends and variability between frostpoint and HALOE remain for the homogenised data. Due to uncertainties in reanalysis temperatures and stratospheric transport combined with uncertainties in observations, no quantitative inference about changes of water entering the stratosphere in the tropics could be made with the mid latitude measurements analysed here

The impact of cirrus clouds on tropical troposphere-to-stratosphere transport

International audienceAlthough it is well known that air enters the stratosphere preferentially through upwelling in the tropics, the exact mechanisms of troposphere-to-stratosphere transport (TST) are still unknown. Previously proposed mechanisms have been found either to be too slow (e.g., clear sky upwelling) to provide agreement with in situ tracer measurements, or to be insufficient in mass flux to act as a major supply for the Brewer-Dobson circulation (e.g., convective overshooting). In this study we evaluate whether the lofting of air via cirrus cloud-radiation interaction might offer an alternative path for TST, which is responsible for a significant fraction of the observed air mass transport. We find that a combination of deep convection and subsequent upwelling associated with cirrus clouds and clear sky can explain the supply of air for the Brewer-Dobson circulation. Thus, upwelling associated with cirrus clouds offers a mechanism for the missing second stage, which links the first stage of TST, deep convection, to the third stage, the Brewer-Dobson circulation

How stratospheric are deep stratospheric intrusions? LUAMI 2008

A large-scale comparison of water-vapour vertical-sounding instruments took place over central Europe on 17 October 2008, during a rather homogeneous deep stratospheric intrusion event (LUAMI, Lindenberg Upper-Air Methods Intercomparison). The measurements were carried out at four observational sites: Payerne (Switzerland), Bilthoven (the Netherlands), Lindenberg (north-eastern Germany), and the Zugspitze mountain (Garmisch-Partenkichen, German Alps), and by an airborne water-vapour lidar system creating a transect of humidity profiles between all four stations. A high data quality was verified that strongly underlines the scientific findings. The intrusion layer was very dry with a minimum mixing ratios of 0 to 35 ppm on its lower west side, but did not drop below 120 ppm on the higher-lying east side (Lindenberg). The dryness hardens the findings of a preceding study (“Part 1”, Trickl et al., 2014) that, e.g., 73 % of deep intrusions reaching the German Alps and travelling 6 days or less exhibit minimum mixing ratios of 50 ppm and less. These low values reflect values found in the lowermost stratosphere and indicate very slow mixing with tropospheric air during the downward transport to the lower troposphere. The peak ozone values were around 70 ppb, confirming the idea that intrusion layers depart from the lowermost edge of the stratosphere. The data suggest an increase of ozone from the lower to the higher edge of the intrusion layer. This behaviour is also confirmed by stratospheric aerosol caught in the layer. Both observations are in agreement with the idea that sections of the vertical distributions of these constituents in the source region were transferred to central Europe without major change. LAGRANTO trajectory calculations demonstrated a rather shallow outflow from the stratosphere just above the dynamical tropopause, for the first time confirming the conclusions in “Part 1” from the Zugspitze CO observations. The trajectories qualitatively explain the temporal evolution of the intrusion layers above the four stations participating in the campaign

The water vapour distribution in the Arctic lowermost stratosphere during the LAUTLOS campaign and related transport processes including stratosphere-troposphere exchange

International audienceBalloon-borne water vapour measurements during January and February 2004, which were obtained as part of the LAUTLOS campaign at Sodankylä, Finland, 67° N, were used to analyse the water vapour distribution in the wintertime Arctic lowermost stratosphere. A 2.5 km thick layer (or 30 K in the potential temperature scale) above the tropopause is characterized by a significant water vapour variability on a synoptic timescale with values between stratospheric and tropospheric, which is in good agreement with previously reported measurements. A cross-correlation analysis of ozone and water vapour confirms that this layer contains a mixture of stratospheric and tropospheric air masses. Some of the flights sampled laminae of enhanced water vapour above the tropopause. Meteorological analyses and backward trajectory calculations show that these features were related to filaments that had developed along the flanks of cut-off anticyclones, which had been active at this time over the Northern Atlantic. The role of the filaments was however not to transport water vapour from the troposphere to the stratosphere but rather to transport it within the stratosphere away from regions where intensive two-way stratosphere-troposphere exchange (STE) was identified. Intensive STE occurred around cut-off anticyclones in regions of strong winds, where calculations suggest the presence of clear-air turbulence (CAT). Evidences that CAT contributes to the troposphere-to-stratosphere transport (TST) are presented. However, statistically, relation between TST and CAT during the studied period is weak

The water vapour distribution in the Arctic lowermost stratosphere during LAUTLOS campaign and related transport processes including stratosphere-troposphere exchange

International audienceBalloon-borne water vapour measurements during January and February 2004, which were obtained as part of the LAUTLOS campaign at Sodankylä, Finland, 67° N, were used to analyse the water vapour distribution in the wintertime Arctic lowermost stratosphere. A 2.5 km thick layer (or 30 K in the potential temperature scale) above the local tropopause is characterized by a significant water vapour variability on a synoptic timescale with values between stratospheric and tropospheric, which is in good agreement with previously reported measurements. A cross-correlation analysis of ozone and water vapour confirms that this layer contains a mixture of stratospheric and tropospheric air masses. Some of the flights sampled laminae of enhanced water vapour above the tropopause. Meteorological analyses and backward trajectory calculations show that these features are related to filaments that had developed along the flanks of cut-off anticyclones, which had been active at this time over the Northern Atlantic. Cross-tropopause mass fluxes calculated following the Wei method are used to identify regions and processes that are important for stratosphere-troposphere exchange (STE) in high-latitudes. Intensive STE occurs around cut-off anticyclones in regions of strong winds, where calculations suggest the presence of developed clear-air turbulence. The decay of the filaments is also shown to be important for STE

In situ observations of "cold trap" dehydration in the western tropical Pacific

International audienceWater vapor sonde observations were conducted at Bandung, Indonesia (6.90 S, 107.60 E) and Tarawa, Kiribati (1.35 N, 172.91 E) in December 2003 to examine the efficiency of the "cold trap'' dehydration in the tropical tropopause layer (TTL). Trajectory analysis based on bundles of trajectories suggest that the modification of air parcels' identity due to irreversible mixing by the branching-out and merging-in of nearby trajectories is found to be an important factor, in addition to the routes air parcels are supposed to follow, for interpreting the water vapor concentrations observed by radiosondes in the TTL. Clear correspondence between the observed water vapor concentration and the estimated temperature history of air parcels is found showing that dry air parcels are exposed to low temperatures while humid air parcels do not experience cold conditions during advection, in support of the "cold trap'' hypothesis. It is suggested that the observed air parcel retained the water vapor by roughly twice as much as the minimum saturation mixing ratio after its passage through the "cold trap,'' although appreciable uncertainties remain

A Raman lidar at La Reunion (20.8° S, 55.5° E) for monitoring water vapour and cirrus distributions in the subtropical upper troposphere: preliminary analyses and description of a future system

A ground-based Rayleigh lidar has provided continuous observations of tropospheric water vapour profiles and cirrus cloud using a preliminary Raman channels setup on an existing Rayleigh lidar above La Reunion over the period 2002–2005. With this instrument, we performed a first measurement campaign of 350 independent water vapour profiles. A statistical study of the distribution of water vapour profiles is presented and some investigations concerning the calibration are discussed. Analysis regarding the cirrus clouds is presented and a classification has been performed showing 3 distinct classes. Based on these results, the characteristics and the design of a future lidar system, to be implemented at the new Reunion Island altitude observatory (2200 m) for long-term monitoring, is presented and numerical simulations of system performance have been realised to compare both instruments

Laboratory evaluation of the effect of nitric acid uptake on frost point hygrometer performance

Chilled mirror hygrometers (CMH) are widely used to measure water vapour in the troposphere and lower stratosphere from balloon-borne sondes. Systematic discrepancies among in situ water vapour instruments have been observed at low water vapour mixing ratios (<5 ppm) in the upper troposphere and lower stratosphere (UT/LS). Understanding the source of the measurement discrepancies is important for a more accurate and reliable determination of water vapour abundance in this region. We have conducted a laboratory study to investigate the potential interference of gas-phase nitric acid (HNO<sub>3</sub>) with the measurement of frost point temperature, and consequently the water vapour mixing ratio, determined by CMH under conditions representative of operation in the UT/LS. No detectable interference in the measured frost point temperature was found for HNO<sub>3</sub> mixing ratios of up to 4 ppb for exposure times up to 150 min. HNO<sub>3</sub> was observed to co-condense on the mirror frost, with the adsorbed mass increasing linearly with time at constant exposure levels. Over the duration of a typical balloon sonde ascent (90–120 min), the maximum accumulated HNO<sub>3</sub> amounts were comparable to monolayer coverage of the geometric mirror surface area, which corresponds to only a small fraction of the actual frost layer surface area. This small amount of co-condensed HNO<sub>3</sub> is consistent with the observed lack of HNO<sub>3</sub> interference in the frost point measurement because the CMH utilizes significant reductions (>10%) in surface reflectivity by the condensate to determine H<sub>2</sub>O

Arctic stratospheric dehydration – Part 2: Microphysical modeling

Large areas of synoptic-scale ice PSCs (polar stratospheric clouds) distinguished the Arctic winter 2009/2010 from other years and revealed unprecedented evidence of water redistribution in the stratosphere. A unique snapshot of water vapor repartitioning into ice particles was obtained under extremely cold Arctic conditions with temperatures around 183 K. Balloon-borne, aircraft and satellite-based measurements suggest that synoptic-scale ice PSCs and concurrent reductions and enhancements in water vapor are tightly linked with the observed de- and rehydration signatures, respectively. In a companion paper (Part 1), water vapor and aerosol backscatter measurements from the RECONCILE (Reconciliation of essential process parameters for an enhanced predictability of Arctic stratospheric ozone loss and its climate interactions) and LAPBIAT-II (Lapland Atmosphere–Biosphere Facility) field campaigns have been analyzed in detail. This paper uses a column version of the Zurich Optical and Microphysical box Model (ZOMM) including newly developed NAT (nitric acid trihydrate) and ice nucleation parameterizations. Particle sedimentation is calculated in order to simulate the vertical redistribution of chemical species such as water and nitric acid. Despite limitations given by wind shear and uncertainties in the initial water vapor profile, the column modeling unequivocally shows that (1) accounting for small-scale temperature fluctuations along the trajectories is essential in order to reach agreement between simulated optical cloud properties and observations, and (2) the use of recently developed heterogeneous ice nucleation parameterizations allows the reproduction of the observed signatures of de- and rehydration. Conversely, the vertical redistribution of water measured cannot be explained in terms of homogeneous nucleation of ice clouds, whose particle radii remain too small to cause significant dehydration