King-plot analysis of isotope shifts in simple diatomic molecules

We demonstrate that the isotope shift in isotopomers of diatomic molecules, where the nucleus of one of its constituent atoms is replaced by another isotope, can be expressed as the sum of a field shift and a mass shift, similar to the atomic case. We show that a linear relation holds between atomic and molecular isotopes shifts, thus extending the King-plot analysis to molecular isotope shifts. Optical isotope shifts in YbF and ZrO and infrared isotope shifts in SnH are analyzed with a molecular King-plot approach, utilizing Yb$^{+}$ and Zr$^{+}$ ionic isotope shifts and charge radii of Sn obtained with non-optical methods. The changes in the mean-squared nuclear charge radii $\delta \langle r^2 \rangle$ of $^{170-174,176}$Yb and $^{90-92,94,96}$Zr extracted from the molecular transitions are found to be in excellent agreement with the values from the spectroscopy of Yb$^{+}$ and Zr$^{+}$, respectively. On the contrary, in the case of the vibrational-rotational transition in SnH, no sensitivity to the nuclear volume could be deduced within the experimental resolution, which makes it unsuitable for the extraction of nuclear charge radii but provides insights into the molecular electronic wave function not accessible via other methods. The new opportunities offered by the molecular King-plot analysis for research in nuclear structure and molecular physics are discussed.Comment: Accepted at Physical Review X. Link to abstract: https://journals.aps.org/prx/accepted/be075Kf7E0c16505459d9fa833408356a593fd90

Precision Measurement of 11Li moments: Influence of Halo Neutrons on the 9Li Core

The electric quadrupole moment and the magnetic moment of the 11Li halo nucleus have been measured with more than an order of magnitude higher precision than before, |Q| = 33.3(5)mb and mu=3.6712(3)mu_N, revealing a 8.8(1.5)% increase of the quadrupole moment relative to that of 9Li. This result is compared to various models that aim at describing the halo properties. In the shell model an increased quadrupole moment points to a significant occupation of the 1d orbits, whereas in a simple halo picture this can be explained by relating the quadrupole moments of the proton distribution to the charge radii. Advanced models so far fail to reproduce simultaneously the trends observed in the radii and quadrupole moments of the lithium isotopes.Comment: 4 pages, 4 figures, 1 tabl

Magnetic Moment of the Fragmentation Aligned 61Fe(9/2)+ Isomer

We report on the g factor measurement of the isomer in $^{61}Fe$ ($E^{*}=861 keV$). The isomer was produced and spin-aligned via a projectile-fragmentation reaction at intermediate energy, the Time Dependent Perturbed Angular Distribution (TDPAD) method being used for the measurement of the g factor. For the first time, due to significant improvements of the experimental technique, an appreciable residual alignment of the isomer has been observed, allowing a precise determination of its g factor: $g=-0.229(2)$. Comparison of the experimental g factor with shell-model and mean field calculations confirms the $9/2^+$ spin and parity assignments and suggests the onset of deformation due to the intrusion of Nilsson orbitals emerging from the $\nu g_{9/2}$.Comment: 4 figures. Submitted to Phys. Rev. Let

A new beamline for laser spin-polarization at ISOLDE

A beamline dedicated to the production of laser-polarized radioactive beams has been constructed at ISOLDE, CERN. We present here different simulations leading to the design and construction of the setup, as well as technical details of the full setup and examples of the achieved polarizations for several radioisotopes. Beamline simulations show a good transmission through the entire line, in agreement with observations. Simulations of the induced nuclear spin-polarization as a function of atom-laser interaction length are presented for $^{26,28}$Na, [1] and for $^{35}$Ar, which is studied in this work. Adiabatic spin rotation of the spin-polarized ensemble of atoms, and how this influences the observed nuclear ensemble polarization, are also performed for the same nuclei. For $^{35}$Ar, we show that multiple-frequency pumping enhances the ensemble polarization by a factor 1.85, in agreement with predictions from a rate equations model. [1] J. Phys. G: Nucl. Part. Phys./174408400

Perspectives for the VITO beam line at ISOLDE, CERN

By using polarized ion beams in combination with the β-NMR technique, the Versatile Ion-polarized Techniques On-line (VITO) experiment at ISOLDE, CERN links together expertise from different fields in an unique experimental setup. An overview of the experimental techniques and a general description of the newly designed beam line are presented. Potential uses in multidisciplinary research and perspectives for future experiments are discussed