104 research outputs found
Observation of a parity oscillation in the conductance of atomic wires
Using a scanning tunnel microscope or mechanically controlled break
junctions, atomic contacts of Au, Pt and Ir are pulled to form chains of atoms.
We have recorded traces of conductance during the pulling process and averaged
these for a large amount of contacts. An oscillatory evolution of conductance
is observed during the formation of the monoatomic chain suggesting a
dependence on even or odd numbers of atoms forming the chain. This behaviour is
not only present in the monovalent metal Au, as it has been previously
predicted, but is also found in the other metals which form chains suggesting
it to be a universal feature of atomic wires
Onset of dissipation in ballistic atomic wires
Electronic transport at finite voltages in free-standing gold atomic chains
of up to 7 atoms in length is studied at low temperatures using a scanning
tunneling microscope (STM). The conductance vs voltage curves show that
transport in these single-mode ballistic atomic wires is non-dissipative up to
a finite voltage threshold of the order of several mV. The onset of dissipation
and resistance within the wire corresponds to the excitation of the atomic
vibrations by the electrons traversing the wire and is very sensitive to
strain.Comment: Revtex4, 4 pages, 3 fig
Quantum interference structures in the conductance plateaus of gold nanojunctions
The conductance of breaking metallic nanojunctions shows plateaus alternated
with sudden jumps, corresponding to the stretching of stable atomic
configurations and atomic rearrangements, respectively. We investigate the
structure of the conductance plateaus both by measuring the voltage dependence
of the plateaus' slope on individual junctions and by a detailed statistical
analysis on a large amount of contacts. Though the atomic discreteness of the
junction plays a fundamental role in the evolution of the conductance, we find
that the fine structure of the conductance plateaus is determined by quantum
interference phenomenon to a great extent.Comment: 4 pages, 4 figure
Calibration of the length of a chain of single gold atoms
Using a scanning tunneling microscope or mechanically controllable break
junctions it has been shown that it is possible to control the formation of a
wire made of single gold atoms. In these experiments an interatomic distance
between atoms in the chain of ~3.6 Angstrom was reported which is not
consistent with recent theoretical calculations. Here, using precise
calibration procedures for both techniques, we measure length of the atomic
chains. Based on the distance between the peaks observed in the chain length
histogram we find the mean value of the inter-atomic distance before chain
rupture to be 2.6 +/- 0.2 A . This value agrees with the theoretical
calculations for the bond length. The discrepancy with the previous
experimental measurements was due to the presence of He gas, that was used to
promote the thermal contact, and which affects the value of the work function
that is commonly used to calibrate distances in scanning tunnelling microscopy
and mechanically controllable break junctions at low temperatures.Comment: 6 pages, 6 figure
Nanosized superconducting constrictions
Nanowires of lead between macroscopic electrodes are produced by means of an
STM. Magnetic fields may destroy the superconductivity in the electrodes, while
the wire remains in the superconducting state. The properties of the resulting
microscopic Josephson junctions are investigated.Comment: 3 pages,3 eps figures include
Local electroexfoliation of graphene with a STM tip
Graphite surfaces can be manipulated by several methods to create graphene structures of different shapes and sizes. Scanning tunneling microscopy (STM) can be used to create these structures either through mechanical contact between the tip and the surface or through electro-exfoliation. In the latter, the mechanisms involved in the process of exfoliation with an applied voltage are not fully understood. Here we show how a graphite surface can be locally exfoliated in a systematic manner by applying an electrostatic force with a STM tip at the edge of a terrace, forming triangular flakes several nanometers in length. We demonstrate, through experiments and simulations, how these flakes are created by a two-step process: first a voltage ramp must be applied at the edge of the terrace, and then the tip must be scanned perpendicularly to the edge. Ab-initio electrostatic calculations reveal that the presence of charges on the graphite surface weakens the interaction between layers allowing for exfoliation at voltages in the same range as those used experimentally. Molecular dynamics simulations show that a force applied locally on the edge of a step produces triangular flakes such as those observed under STM. Our results provide new insights towards surface modification that can be extended to other layered materials
Measurement of the conductance of a hydrogen molecule
Recent years have shown steady progress in research towards molecular
electronics [1,2], where molecules have been investigated as switches [3-5],
diodes [6], and electronic mixers [7]. In much of the previous work a Scanning
Tunnelling Microscope was employed to address an individual molecule. As this
arrangement does not provide long-term stability, more recently
metal-molecule-metal links have been made using break junction devices [8-10].
However, it has been difficult to establish unambiguously that a single
molecule forms the contact [11]. Here, we show that a single H2 molecule can
form a stable bridge between Pt electrodes. In contrast to results for other
organic molecules, the bridge has a nearly perfect conductance of one quantum
unit, carried by a single channel. The H2-bridge provides a simple test system
and a fundamental step towards understanding transport properties of
single-molecule devices.Comment: 6 pages, 4 figure
DC current through a superconducting two-barrier system
We analyze the influence of the structure within a SNS junction on the
multiple Andreev resonances in the subgap I-V characteristics. Coherent
interference processes and incoherent propagation in the normal region are
considered. The detailed geometry of the normal region where the voltage drops
in superconducting contacts can lead to observable effects in the conductance
at low voltages.Comment: 11 pages, including 7 postscript file
Proximity effect and strong coupling superconductivity in nanostructures built with an STM
We present high resolution tunneling spectroscopy data at very low
temperatures on superconducting nanostructures of lead built with an STM. By
applying magnetic fields, superconductivity is restricted to length scales of
the order of the coherence length. We measure the tunneling conductance and
analyze the phonon structure and the low energy DOS. We demonstrate the
influence of the geometry of the system on the magnetic field dependence of the
tunneling density of states, which is gapless in a large range of fields. The
behavior of the features in the tunneling conductance associated to phonon
modes are explained within current models.Comment: 4 figures, 4 page
Universality in metallic nanocohesion: a quantum chaos approach
Convergent semiclassical trace formulae for the density of states and
cohesive force of a narrow constriction in an electron gas, whose classical
motion is either chaotic or integrable, are derived. It is shown that mode
quantization in a metallic point contact or nanowire leads to universal
oscillations in its cohesive force: the amplitude of the oscillations depends
only on a dimensionless quantum parameter describing the crossover from chaotic
to integrable motion, and is of order 1 nano-Newton, in agreement with recent
experiments. Interestingly, quantum tunneling is shown to be described
quantitatively in terms of the instability of the classical periodic orbits.Comment: corrects spelling of one author name on abstract page (paper is
unchanged
- …