1,992 research outputs found
Electron-ion recombination of Si IV forming Si III: Storage-ring measurement and multiconfiguration Dirac-Fock calculations
The electron-ion recombination rate coefficient for Si IV forming Si III was
measured at the heavy-ion storage-ring TSR. The experimental electron-ion
collision energy range of 0-186 eV encompassed the 2p(6) nl n'l' dielectronic
recombination (DR) resonances associated with 3s to nl core excitations, 2s
2p(6) 3s nl n'l' resonances associated with 2s to nl (n=3,4) core excitations,
and 2p(5) 3s nl n'l' resonances associated with 2p to nl (n=3,...,infinity)
core excitations. The experimental DR results are compared with theoretical
calculations using the multiconfiguration Dirac-Fock (MCDF) method for DR via
the 3s to 3p n'l' and 3s to 3d n'l' (both n'=3,...,6) and 2p(5) 3s 3l n'l'
(n'=3,4) capture channels. Finally, the experimental and theoretical plasma DR
rate coefficients for Si IV forming Si III are derived and compared with
previously available results.Comment: 13 pages, 9 figures, 3 tables. Accepted for publication in Physical
Review
Changes in antimicrobial resistance of Escherichia coli causing urinary tract infections in hospitalized children
Fragmentation and systematics of the Pygmy Dipole Resonance in the stable N=82 isotones
The low-lying electric dipole (E1) strength in the semi-magic nucleus 136Xe
has been measured which finalizes the systematic survey to investigate the
so-called pygmy dipole resonance (PDR) in all stable even N=82 isotones with
the method of nuclear resonance fluorescence using real photons in the entrance
channel. In all cases, a fragmented resonance-like structure of E1 strength is
observed in the energy region 5 MeV to 8 MeV. An analysis of the fragmentation
of the strength reveals that the degree of fragmentation decreases towards the
proton-deficient isotones while the total integrated strength increases
indicating a dependence of the total strength on the neutron-to-proton ratio.
The experimental results are compared to microscopic calculations within the
quasi-particle phonon model (QPM). The calculation includes complex
configurations of up to three phonons and is able to reproduce also the
fragmentation of the E1 strength which allows to draw conclusions on the
damping of the PDR. Calculations and experimental data are in good agreement in
the degree of fragmentation and also in the integrated strength if the
sensitivity limit of the experiments is taken into account
Magnetic Sublevel Population and Alignment for the Excitation of H- and He-like Uranium in Relativistic Collisions
We have measured the alignment of the L-shell magnetic-substates following
the K-shell excitation of hydrogen- and helium-like uranium in relativistic
collisions with a low-Z gaseous target. Within this experiment the population
distribution for the L-shell magnetic sublevels has been obtained via an
angular differential study of the decay photons associated with the subsequent
de-excitation process. The results show a very distinctive behavior for the H-
and He-like heavy systems. In particular for excitation of
He-like uranium, a considerable alignment of the L-shell levels was observed. A
comparison of our experimental findings with recent rigorous relativistic
predictions provides a good qualitative and a reasonable quantitative
agreement, emphasizing the importance of the magnetic-interaction and many-body
effects in the strong-field domain of high-Z ions
Relativistic and retardation effects in the two--photon ionization of hydrogen--like ions
The non-resonant two-photon ionization of hydrogen-like ions is studied in
second-order perturbation theory, based on the Dirac equation. To carry out the
summation over the complete Coulomb spectrum, a Green function approach has
been applied to the computation of the ionization cross sections. Exact
second-order relativistic cross sections are compared with data as obtained
from a relativistic long-wavelength approximation as well as from the scaling
of non-relativistic results. For high-Z ions, the relativistic wavefunction
contraction may lower the two-photon ionization cross sections by a factor of
two or more, while retardation effects appear less pronounced but still give
rise to non-negligible contributions.Comment: 6 pages, 2 figure
The local adsorption structure of benzene on Si(001)-(2 × 1): a photoelectron diffraction investigation
Scanned-energy mode C 1s photoelectron diffraction has been used to investigate the local adsorption geometry of benzene on Si(001) at saturation coverage and room temperature. The results show that two different local bonding geometries coexist, namely the 'standard butterfly' (SB) and 'tilted bridge' (TB) forms, with a composition of 58 ± 29% of the SB species. Detailed structural parameter values are presented for both species including Si–C bond lengths. On the basis of published measurements of the rate of conversion of the SB to the TB form on this surface, we estimate that the timescale of our experiment is sufficient for achieving equilibrium, and in this case our results indicate that the difference in the Gibbs free energy of adsorption, ΔG(TB)−ΔG(SB), is in the range −0.023 to +0.049 eV. We suggest, however, that the relative concentration of the two species may also be influenced by a combination of steric effects influencing the kinetics, and a sensitivity of the adsorption energies of the adsorbed SB and TB forms to the nature of the surrounding benzene molecules
- …