Contrasting properties of particle-particle and hole-hole excitations in ²⁰⁶Tl and ²¹⁰Bi nuclei

A complete-spectroscopy investigation of low-lying, low-spin states in the one-proton-hole and one-neutron-hole nucleus 206Tl has been performed by using thermal neutron capture and γ-coincidence technique with the FIPPS Ge array at ILL Grenoble. The new experimental results, together with data for the one-proton-particle and one-neutron-particle nucleus 210Bi (taken from a previous study done at ILL in the EXILL campaign), allowed for an extensive comparison with predictions of shell-model calculations performed with realistic interactions. No phenomenological adjustments were introduced in the calculations. In 210Bi, state energies, transition multipolarities and decay branchings agree well with theory for the three well separated multiplets of states which dominate the low-lying excitations. On the contrary, in 206Tl significant discrepancies are observed: in the same energy region, six multiplets were identified, with a significant mixing among them being predicted, as a consequence of the smaller energy separation between the active orbitals. The discrepancies in 206Tl are attributed to the larger uncertainties in the determination of the off-diagonal matrix elements of the realistic shell-model interaction with respect to the calculated diagonal matrix elements, the only ones playing a major role in the case of 210Bi. The work points to the need of more advanced approaches in the construction of the realistic interactions

The mutable nature of particle-core excitations with spin in the one-valence-proton nucleus ¹³³Sb

The γ-ray decay of excited states of the one-valence-proton nucleus ¹³³Sb has been studied using cold-neutron induced fission of ²³⁵U and ²⁴¹Pu targets, during the EXILL campaign at the ILL reactor in Grenoble. By using a highly efficient HPGe array, coincidences between γ-rays prompt with the fission event and those delayed up to several tens of microseconds were investigated, allowing to observe, for the first time, high-spin excited states above the 16.6 μs isomer. Lifetimes analysis, performed by fast-timing techniques with LaBr₃(Ce) scintillators, revealed a difference of almost two orders of magnitude in B(M1) strength for transitions between positive-parity medium-spin yrast states. The data are interpreted by a newly developed microscopic model which takes into account couplings between core excitations (both collective and non-collective) of the doubly magic nucleus ¹³²Sn and the valence proton, using the Skyrme effective interaction in a consistent way. The results point to a fast change in the nature of particle-core excitations with increasing spin

Detailed low-spin spectroscopy of Ni 65 via neutron capture reaction

An extended investigation of the low-spin structure of the Ni65 nucleus was performed at the Institut Laue-Langevin, Grenoble, France, via the neutron capture reaction Ni64(n,γ)Ni65, using the Fission Product Prompt Gamma-Ray Spectrometer High-Purity Ge array. The level scheme of Ni65 was significantly expanded, with two new levels and 87 newly found transitions. Angular correlation analyses were also performed, allowing us to assign spins and parities for a number of states and to determine multipolarity mixing ratios for selected γ transitions. The low-energy part of the experimental level scheme (up to about 1.4 MeV) was compared with Monte Carlo shell-model calculations, which predict spherical shapes for all states, apart from the 9/2+ and the second excited 1/2- states of oblate deformation.SCOPUS: ar.jinfo:eu-repo/semantics/publishe

High-precision spectroscopy of 65Ni via neutron capture

Detailed studies of the low-spin structures of neutron-rich Ni isotopes may help shedding light on the shape coexistence phenomenon. Of particular interest is the 65Ni nucleus, since it lies between 64Ni and 66Ni, where shape coexistence has been reported earlier. A spectroscopic investigation of 65Ni has been performed at Institut Laue-Langevin via the reaction64Ni(n,γ)65Ni, using the FIPPS HPGe array. Several new gamma transitions have been observed and angular correlation analyses have been performed. A comparison with Monte Carlo shell-model calculations pointed to a dominance of spherical states up to 1.5 MeV excitation energy, together with the appearance of two states of oblate character.SCOPUS: ar.jinfo:eu-repo/semantics/publishe

Testing the predictive power of realistic shell model calculations via lifetime measurement of the 11/2+ state in 131Sb

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Multifaceted Quadruplet of Low-Lying Spin-Zero States in Ni 66: Emergence of Shape Isomerism in Light Nuclei

A search for shape isomers in the Ni66 nucleus was performed, following old suggestions of various mean-field models and recent ones, based on state-of-the-art Monte Carlo shell model (MCSM), all considering Ni66 as the lightest nuclear system with shape isomerism. By employing the two-neutron transfer reaction induced by an O18 beam on a Ni64 target, at the sub-Coulomb barrier energy of 39 MeV, all three lowest-excited 0+ states in Ni66 were populated and their γ decay was observed by γ-coincidence technique. The 0+ states lifetimes were assessed with the plunger method, yielding for the 02+, 03+, and 04+ decay to the 21+ state the B(E2) values of 4.3, 0.1, and 0.2 Weisskopf units (W.u.), respectively. MCSM calculations correctly predict the existence of all three excited 0+ states, pointing to the oblate, spherical, and prolate nature of the consecutive excitations. In addition, they account for the hindrance of the E2 decay from the prolate 04+ to the spherical 21+ state, although overestimating its value. This result makes Ni66 a unique nuclear system, apart from U236,238, in which a retarded γ transition from a 0+ deformed state to a spherical configuration is observed, resembling a shape-isomerlike behavior.SCOPUS: ar.jinfo:eu-repo/semantics/publishe

Dynamical Dipole and Equation of State in N/Z Asymmetric Fusion Reactions

In heavy ion reactions, in the case of N/Z asymmetry between projectile and target, the process leading to complete fusion is expected to produce pre-equilibrium dipole γ-ray emission. It is generated during the charge equilibration process and it is known as Dynamical Dipole. A new measurement of the dynamical dipole emission was performed by studying 16O + 116Sn at 12 MeV/u. These data, together with those measured at 8.1 MeV/u and 15.6 MeV/u for the same reaction, provide the dependence on the Dynamical Dipole total emission yield with beam energy and they can be compared with theoretical expectations. The experimental results show a weak increase of the Dynamical Dipole total yield with beam energies and are in agreement with the prediction of a theoretical model based on the Boltzmann–Nordheim–Vlasov (BNV) approach. The measured trend with beam energy does not confirm the rise and fall behavior previously reported for the same fused compound but with a much higher dipole moment

Shape Coexistence at Zero Spin in 64Ni driven by the Monopole Tensor Interaction

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