Application of LaBr3 detector for neutron resonance densitometry

A method to determine the amount of nuclear materials in melted fuel resulting from a nuclear accident such as the one occurred at the Fukushima Daiichi nuclear power plants has not yet been established. The problem is complex due to the expected presence of 10B and other strong neutron absorbing impurities. For this reason, neutron resonance densitometry, combining neutron resonance transmission analysis and neutron capture analysis, is proposed and a feasibility study has been defined. In this contribution a method to account for the presence of 10B is presented and investigated. The study includes GEANT4 simulations to study the performance of a new well type gamma-ray detector based on LaBr3 scintillators. In the design of the detector the main emphasis was on the capability to separate the full energy peak corresponding to the 478-keV gamma ray resulting from the 10B(n,αγ) reaction from the contribution of the 662-keV gamma ray due to the decay of 137Cs. In addition, experiments have been carried out at the time-of-flight facility GELINA of the EC-JRC-IRMM to test the capabilities of a LaBr3 detector for NRCA applications, in particular to determine impurities present in the melted fuel. A neutron resonance capture gamma-ray experiment with a natSe sample was performed using a LaBr3 scintillator in parallel with a Ge-detector. The results of these measurements demonstrate that a LaBr3 detector is suitable for NRCA as a part of neutron resonance densitometry.JRC.D.4-Standards for Nuclear Safety, Security and Safeguard

Proposal of neutron resonance densitometry for particle like debris of melted fuel using NRTA and NRCA

Neutron resonance densitometry (NRD) has been proposed to quantify nuclear materials in particle-like debris of melted fuel formed in a severe accident of nuclear reactors such as the Fukushima Daiichi nuclear power plants. NRD is a method that combines NRTA (neutron resonance transmission analysis) and NRCA (neutron resonance capture analysis) using a pulsed neutron generator and the TOF (time of flight) technique. NRTA is used to quantify the amount of Pu and U isotopes. NRCA is used to identify matrix materials, such as B and Fe, which are present in the melted fuel. A special gamma-ray spectrometer has been designed to apply NRCA in the presence of highly radioactive materials. The applicability of the NRD method has been studied using Monte Carlo simulations and neutron TOF experiments at the GELINA facility of the EC-JRC-IRMM. We conclude that NRD has a potential to determine the quantities of Pu and U isotopes in particle-like debris of melted fuel with counting statistics uncertainties less than 1%, even in the presence of 2.5 w% natB and 9 w% 56Fe.JRC.D.4-Standards for Nuclear Safety, Security and Safeguard

First Direct Mass Measurements of Nuclides around Z=100 with a Multireflection Time-of-Flight Mass Spectrograph

The masses of 246Es, 251Fm, and the transfermium nuclei 249−252Md and 254No, produced by hot- and cold-fusion reactions, in the vicinity of the deformed N=152 neutron shell closure, have been directly measured using a multireflection time-of-flight mass spectrograph. The masses of 246Es and 249,250,252Md were measured for the first time. Using the masses of 249,250Md as anchor points for α decay chains, the masses of heavier nuclei, up to 261Bh and 266Mt, were determined. These new masses were compared with theoretical global mass models and demonstrated to be in good agreement with macroscopic-microscopic models in this region. The empirical shell gap parameter δ2n derived from three isotopic masses was updated with the new masses and corroborates the existence of the deformed N=152 neutron shell closure for Md and Lr

Effect of thrombin peptide 508 (TP508) on bone healing during distraction osteogenesis in rabbit tibia

Thrombin-related peptide 508 (TP508) accelerates bone regeneration during distraction osteogenesis (DO). We have examined the effect of TP508 on bone regeneration during DO by immunolocalization of Runx2 protein, a marker of osteoblast differentiation, and of osteopontin (OPN) and bone sialoprotein (BSP), two late markers of the osteoblast lineage. Distraction was performed in tibiae of rabbits over a period of 6 days. TP508 (30 or 300 μg) or vehicle was injected into the distraction gap at the beginning and end of the distraction period. Two weeks after active distraction, tissue samples were harvested and processed for immunohistochemical analysis. We also tested the in vitro effect of TP508 on Runx2 mRNA expression in osteoblast-like (MC3T3-E1) cells by polymerase chain reaction analysis. Runx2 and OPN protein were observed in preosteoblasts, osteoblasts, osteocytes of newly formed bone, blood vessel cells and many fibroblast-like cells of the soft connective tissue. Immunostaining for BSP was more restricted to osteoblasts and osteocytes. Significantly more Runx2- and OPN-expressing cells were seen in the group treated with 300 μg TP508 than in the control group injected with saline or with 30 μg TP508. However, TP508 failed to increase Runx2 mRNA levels significantly in MC3T3-E1 cells after 2–3 days of exposure. Our data suggest that TP508 enhances bone regeneration during DO by increasing the proportion of cells of the osteoblastic lineage. Clinically, TP508 may shorten the healing time during DO; this might be of benefit when bone regeneration is slow

kaonic atom experiments at j parc

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