1,297 research outputs found

    Quenched chirality in RbNiCl3_3

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    The critical behaviour of stacked-triangular antiferromagnets has been intensely studied since Kawamura predicted new universality classes for triangular and helical antiferromagnets. The new universality classes are linked to an additional discrete degree of freedom, chirality, which is not present on rectangular lattices, nor in ferromagnets. However, the theoretical as well as experimental situation is discussed controversially, and generic scaling without universality has been proposed as an alternative scenario. Here we present a careful investigation of the zero-field critical behaviour of RbNiCl3_3, a stacked-triangular Heisenberg antiferromagnet with very small Ising anisotropy. From linear birefringence experiments we determine the specific heat exponent α\alpha as well as the critical amplitude ratio A+/A−A^+/A^-. Our high-resolution measurements point to a single second order phase transition with standard Heisenberg critical behaviour, contrary to all theoretical predictions. From a supplementary neutron diffraction study we can exclude a structural phase transition at TN_N. We discuss our results in the context of other available experimental results on RbNiCl3_3 and related compounds. We arrive at a simple intuitive explanation which may be relevant for other discrepancies observed in the critical behaviour of stacked-triangular antiferromagnets. In RbNiCl3_3 the ordering of the chirality is suppressed by strong spin fluctuations, yielding to a different phase diagram, as compared to e.g.\@ CsNiCl3_3, where the Ising anisotropy prevents these fluctuations

    Haydeeite: a spin-1/2 kagome ferromagnet

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    The mineral haydeeite, alpha-MgCu3(OD)6Cl2, is a S=1/2 kagome ferromagnet that displays long-range magnetic order below TC=4.2 K with a strongly reduced moment. Our inelastic neutron scattering data show clear spin-wave excitations that are well described by a Heisenberg Hamiltonian with ferromagnetic nearest-neighbor exchange J1=-38 K and antiferromagnetic exchange Jd=+11 K across the hexagons of the kagome lattice. These values place haydeeite very close to the quantum phase transition between ferromagnetic order and non-coplanar twelve-sublattice cuboc2 antiferromagnetic order. Diffuse dynamic short-range ferromagnetic correlations observed above TC persist well into the ferromagnetically ordered phase with a behavior distinct from critical scattering

    Low dimensional ordering and fluctuations in methanol-β\beta-hydroquinone-clathrate studied by X-ray and neutron diffraction

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    Methanol-β\beta-hydroquinone-clathrate has been established as a model system for dielectric ordering and fluctuations and is conceptually close to magnetic spin systems. In X-ray and neutron diffraction experiments, we investigated the ordered structure, the one-dimensional (1D) and the three-dimensional (3D) critical scattering in the paraelectric phase, and the temperature dependence of the lattice constants. Our results can be explained by microscopic models of the methanol pseudospin in the hydroquinone cage network, in consistency with previous dielectric investigations

    Magnetic Order and Dynamics in Stripe-Ordered La2-xSrxNiO4

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    We have studied magnetic correlations in several compositions of stripe-ordered La2-xSrxNiO4. In this paper we show how polarized-neutron scattering has helped uncover important features of the magnetic ordering and spin dynamics. In particular, polarization analysis has enabled us (1) to characterize a spin reorientation transition, (2) to identify anisotropy gaps in the spin excitation spectrum, and (3) to investigate an anomalous dip in the spin-wave intensity suggestive of coupling between collective spin and charge excitations.Comment: 4 pages, 3 figs. Presented at PNSXM, Venice. To appear in Physica

    Spin correlations among the charge carriers in an ordered stripe phase

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    We have observed a diffuse component to the low-energy magnetic excitation spectrum of stripe-ordered La5/3Sr1/3NiO4 probed by neutron inelastic scattering. The diffuse scattering forms a square pattern with sides parallel and perpendicular to the stripe directions. The signal is dispersive, with a maximum energy of ~10 meV. Probed at 2 meV the scattering decreases in strength with increasing temperature, and is barely visible at 100 K. We argue that the signal originates from dynamic, quasi- one-dimensional, antiferromagnetic correlations among the stripe electrons.Comment: 4 pages, 4 figures. To be published in Physical Review Letter

    Electronic structure and magnetic properties of the spin-1/2 Heisenberg system CuSe2O5

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    A microscopic magnetic model for the spin-1/2 Heisenberg chain compound CuSe2O5 is developed based on the results of a joint experimental and theoretical study. Magnetic susceptibility and specific heat data give evidence for quasi-1D magnetism with leading antiferromagnetic (AFM) couplings and an AFM ordering temperature of 17 K. For microscopic insight, full-potential DFT calculations within the local density approximation (LDA) were performed. Using the resulting band structure, a consistent set of transfer integrals for an effective one-band tight-binding model was obtained. Electronic correlations were treated on a mean-field level starting from LDA (LSDA+U method) and on a model level (Hubbard model). In excellent agreement of experiment and theory, we find that only two couplings in CuSe2O5 are relevant: the nearest-neighbour intra-chain interaction of 165 K and a non-frustrated inter-chain coupling of 20 K. From a comparison with structurally related systems (Sr2Cu(PO4)2, Bi2CuO4), general implications for a magnetic ordering in presence of inter-chain frustration are made.Comment: 20 pages, 8 figures, 3 table

    Root cortex development is fine-tuned by the interplay of MIGs, SCL3 and DELLAs during arbuscular mycorrhizal symbiosis

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    Root development is a crucial process that determines the ability of plants to acquire nutrients, adapt to the substrate and withstand changing environmental conditions. Root plasticity is controlled by a plethora of transcriptional regulators that allow, in contrast to tissue development in animals, post-embryonic changes that give rise to new tissue and specialized cells. One of these changes is the accommodation in the cortex of hyperbranched hyphae of symbiotic arbuscular mycorrhizal (AM) fungi, called arbuscules. Arbuscule-containing cells undergo massive reprogramming to coordinate developmental changes with transport processes. Here we describe a novel negative regulator of arbuscule development, MIG3. MIG3 induces and interacts with SCL3, both of which modulate the activity of the central regulator DELLA, restraining cortical cell growth. As in a tug-of-war, MIG3-SCL3 antagonizes the function of the complex MIG1-DELLA, which promotes the cell expansion required for arbuscule development, adjusting cell size during the dynamic processes of the arbuscule life cycle. Our results in the legume plant Medicago truncatula advance the knowledge of root development in dicot plants, showing the existence of additional regulatory elements not present in Arabidopsis that fine-tune the activity of conserved central modules

    The critical behavior of frustrated spin models with noncollinear order

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    We study the critical behavior of frustrated spin models with noncollinear order, including stacked triangular antiferromagnets and helimagnets. For this purpose we compute the field-theoretic expansions at fixed dimension to six loops and determine their large-order behavior. For the physically relevant cases of two and three components, we show the existence of a new stable fixed point that corresponds to the conjectured chiral universality class. This contradicts previous three-loop field-theoretical results but is in agreement with experiments.Comment: 4 pages, RevTe

    Surgical smoke: modern mobile smoke evacuation systems improve occupational safety in the operating theatre.

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    OBJECTIVES Evaluation of smoke capture efficiency of different mobile smoke evacuation devices with respect to volatile organic compounds and their noise emission. METHODS Electrosurgical incisions were performed on fresh porcine liver in an operating room with vertical laminar flow. The generated surgical smoke was analysed with proton-transfer-reaction mass spectrometry with and without the use of a mobile smoke evacuation system consisting of a smoke evacuator machine, a suction hose and a handpiece. The inlet of the mass spectrometer was positioned 40 cm above the specimen. Various devices were compared: a hard plastic funnel, a flexible foam funnel, an on-tip integrated aspirator of an electrosurgical knife and a standard secretion suction (Yankauer). Also, sound levels were measured at a distance of 40 cm from the handpieces' inlet. RESULTS The smoke capture efficiency of the secretion suction was only 53%, while foam funnel, plastic funnel and integrated aspirator were all significantly more effective with a clearance of 95%, 91% and 91%, respectively. The mean sound levels were 68 and 59 A-weighted decibels with the plastic and foam funnel, respectively, 66 A-weighted decibels with the integrated aspirator and 63 A-weighted decibels with the secretion suction. CONCLUSIONS Carcinogenic, mutagenic and reprotoxic volatile organic compounds in surgical smoke can be efficiently reduced by mobile smoke evacuation system, providing improved protection for medical personnel. Devices specifically designed for smoke evacuation are more efficient than standard suction tools. Noise exposure for the surgeon was lowest with the flexible foam funnel and higher with the other handpieces tested
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