Photoemission view of electron fractionalization in quasi-one dimensional metal Li0.9_{0.9}Mo6_6O17_{17}

We report Luttinger liquid line shapes better revealed by new angle resolved photoemission data taken with a much improved angle resolution on a quasi-1-dimensional metal Li$_{0.9}$Mo$_6$O$_{17}$. The new data indicate a larger spinon velocity than our previous lower resolution data indicated.Comment: submitted to SCES '0

ARPES Study of X-Point Band Overlaps in LaB6_6 and SmB6_6 - Contrast to SrB6_6 and EuB6_6

In contrast to our recent finding of an X-point band gap in divalent hexaborides, we report here that angle resolved photoemission spectroscopy (ARPES) data shows that the gap is absent for trivalent LaB$_6$ and is absent or nearly so for mixed valent SmB$_6$. This finding demonstrates a nontrivial evolution of the band structure from divalent to trivalent hexaborides.Comment: submitted to SCES '0

Direct visualization of coexisting channels of interaction in CeSb

Our understanding of correlated electron systems is vexed by the complexity of their interactions. Heavy fermion compounds are archetypal examples of this physics, leading to exotic properties that weave magnetism, superconductivity and strange metal behavior together. The Kondo semimetal CeSb is an unusual example where different channels of interaction not only coexist, but have coincident physical signatures, leading to decades of debate about the microscopic picture describing the interactions between the f moments and the itinerant electron sea. Using angle-resolved photoemission spectroscopy, we resonantly enhance the response of the Ce f electrons across the magnetic transitions of CeSb and find there are two distinct modes of interaction that are simultaneously active, but on different kinds of carriers. This study reveals how correlated systems can reconcile the coexistence of different modes on interaction-by separating their action in momentum space, they allow their coexistence in real space.11Ysciescopu

Generalized Spectral Signatures of Electron Fractionalization in Quasi-One and -Two Dimensional Molybdenum Bronzes and Superconducting Cuprates

We establish the quasi-one-dimensional Li purple bronze as a photoemission paradigm of Luttinger liquid behavior. We also show that generalized signatures of electron fractionalization are present in the angle resolved photoemission spectra for quasi-two-dimensional purple bronzes and certain cuprates. An important component of our analysis for the quasi-two-dimensional systems is the proposal of a ``melted holon'' scenario for the k-independent background that accompanies but does not interact with the peaks that disperse to define the Fermi surface.Comment: 7 pages, 8 figure

Momentum dependent dxz/yz band splitting in LaFeAsO

The nematic phase in iron based superconductors (IBSs) has attracted attention with a notion that it may provide important clue to the superconductivity. A series of angle-resolved photoemission spectroscopy (ARPES) studies were performed to understand the origin of the nematic phase. However, there is lack of ARPES study on LaFeAsO nematic phase. Here, we report the results of ARPES studies of the nematic phase in LaFeAsO. Degeneracy breaking between the dxz and dyz hole bands near the Γ and M point is observed in the nematic phase. Different temperature dependent band splitting behaviors are observed at the Γ and M points. The energy of the band splitting near the M point decreases as the temperature decreases while it has little temperature dependence near the Γ point. The nematic nature of the band shift near the M point is confirmed through a detwin experiment using a piezo device. Since a momentum dependent splitting behavior has been observed in other iron based superconductors, our observation confirms that the behavior is a universal one among iron based superconductors

Electronic transport in EuB6_6

EuB$_6$ is a magnetic semiconductor in which defects introduce charge carriers into the conduction band with the Fermi energy varying with temperature and magnetic field. We present experimental and theoretical work on the electronic magnetotransport in single-crystalline EuB$_6$. Magnetization, magnetoresistance and Hall effect data were recorded at temperatures between 2 and 300 K and in magnetic fields up to 5.5 T. The negative magnetoresistance is well reproduced by a model in which the spin disorder scattering is reduced by the applied magnetic field. The Hall effect can be separated into an ordinary and an anomalous part. At 20 K the latter accounts for half of the observed Hall voltage, and its importance decreases rapidly with increasing temperature. As for Gd and its compounds, where the rare-earth ion adopts the same Hund's rule ground state as Eu$^{2+}$ in EuB$_{6}$, the standard antisymmetric scattering mechanisms underestimate the $size$ of this contribution by several orders of magnitude, while reproducing its $shape$ almost perfectly. Well below the bulk ferromagnetic ordering at $T_C$ = 12.5 K, a two-band model successfully describes the magnetotransport. Our description is consistent with published de Haas van Alphen, optical reflectivity, angular-resolved photoemission, and soft X-ray emission as well as absorption data, but requires a new interpretation for the gap feature deduced from the latter two experiments.Comment: 35 pages, 12 figures, submitted to PR

Electronic Structure of Calcium Hexaboride within the Weighted Density Approximation

We report calculations of the electronic structure of CaB$_6$ using the weighted density approximation (WDA) to density functional theory. We find a semiconducting band structure with a sizable gap, in contrast to local density approximation (LDA) results, but in accord with recent experimental data. In particular, we find an $X$-point band gap of 0.8 eV. The WDA correction of the LDA error in describing the electronic structure of CaB$_6$ is discussed in terms of the orbital character of the bands and the better cancelation of self-interactions within the WDA.Comment: 1 figur

Angle-resolved photoemission study of quasi-one-dimensional superconductor β\beta-Na0.33_{0.33}V2_2O5_5

We have studied the electronic structure of $\beta$-Na$_{0.33}$V$_2$O$_5$, which becomes a superconductor under pressure, by angle-resolved photoemission spectroscopy. Clear band dispersions is observed only along the chain direction, indicating the quasi-one-dimensional (1D) electronic structure. The spectra of the V 3d band are dominated by a Gaussian-like broad feature at $\sim$ 1 eV below the Fermi level ($E_F$) with negligible intensity at $E_F$, which we attribute to strong electron-phonon coupling as in other 1D polaronic metals. In the momentum space, the spectra show a maximum intensity at $k \sim \pm \pi/4b$, where $b$ is the V-V distance along the b-axis, reflecting the band filling of the chain and/or ladder.Comment: 4 pages, 4 figure